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Zhicheng Pei

Publications and source records attributed to Zhicheng Pei.

2 recordsLinked to original sources

Field re-entrant superconductivity in Eu-doped infinite-layer nickelates

Intertwined superconducting and magnetic orders may give rise to exotic quantum phases, including field-induced and re-entrant superconductivity. However, such magnetism-enhanced superconductivity has remained elusive in superconductors with higher transition temperatures. While infinite-layer nickelates represent a new class of unconventional superconductors, the impact of rare-earth magnetism on superconducting properties remains largely unexplored. Here, we show that Eu-doped infinite-layer nickelate Sm$_{0.95-x}$Ca$_{0.05}$Eu$_x$NiO$_2$ exhibits a magnetic-field-induced re-entrant superconducting phase in the Eu-rich over-doped regime. Zero-resistance transport and high-field diamagnetic screening confirm the superconducting nature of this phase, which emerges after the initial suppression of low-field superconductivity and remains robust across a broad range of temperatures, fields and field orientations. In the same doping range, we observe nonlinear Hall transport and hysteretic magnetoresistance, indicating the unconventional nature of the re-entrant behaviour. While partially consistent with a compensation mechanism between the Eu-derived exchange field and the applied field, our data reveal pronounced deviations from this model at the highest-doping levels. Our findings establish infinite-layer nickelates as a fertile platform for exploring magnetically driven high-field superconductivity in strongly correlated oxides.

cond-mat.supr-con↗

Enhanced Superconductivity and Mixed-dimensional Behaviour in Infinite-layer Samarium Nickelate Thin Films

Rare-earth infinite-layer nickelates represent an emerging class of unconventional superconductors, with materials synthesis largely limited to early lanthanide compounds. Here, we report the synthesis and characterization of phase-pure superconducting samarium-based infinite-layer nickelate thin films, including the first demonstration of Sm$_{1-x}$Sr$_x$NiO$_2$, along with co-doped variants incorporating europium and calcium. These films, grown on LSAT (001) substrates, exhibit coherent lattice structures up to $\sim$ 9 nm thickness with minimal stacking faults. The co-doped compounds achieve a record-small $c$-axis parameter of 3.26 Å and display remarkable superconducting transition temperatures up to 32.5 K. These results establish a clear correlation between decreasing $c$-axis parameter and increasing critical temperature across different rare-earth systems. In addition, angle-dependent magnetoresistance investigations reveal the existence of a hybrid mixture of 2D and 3D superconductivity in this novel system with enhanced coupling between the rare-earth 5d and Ni 3d orbitals, confirmed by resonant inelastic X-ray scattering experiments. As the concentration of Eu increases, the system exhibits a clear tendency towards 3D superconductivity. Furthermore, we observe distinctive negative magnetoresistance in the europium-containing samples. These findings advocate clear materials design principles for higher transition temperatures and exotic physics in infinite-layer nickelate superconductors through structural engineering of the rare-earth site.

cond-mat.supr-con↗