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Zhihuan Dong

Publications and source records attributed to Zhihuan Dong.

13 recordsLinked to original sources

Imaging Interacting Two-Dimensional Anisotropic Electrons

We directly visualize a two-dimensional anisotropic Wigner crystal and its quantum melting in monolayer 1T-ReSe2 using non-invasive scanning tunnelling microscopy. In crystals with anisotropic effective mass, an electron's quantum wavefunction becomes elongated along the light-mass direction to reduce kinetic energy. At low electron density, such anisotropic electrons are predicted to form an oblique Wigner crystal rather than the familiar triangular lattice of isotropic systems. Despite longstanding theoretical interest, this physics has been little explored experimentally. Here we first image the anisotropic shape of individual electrons in gated monolayer ReSe2, whose wavefunctions are strongly elongated along the light-mass direction. At low density, these electrons crystallize into an oblique Wigner lattice. As the density increases, quantum fluctuations grow more rapidly along the light-mass direction than along the heavy-mass direction, driving a one-dimensional melting of the crystal. The resulting state retains order along one direction but melts along the other, consistent with a smectic electron liquid crystal between the electron solid and Fermi liquid phases. Our work establishes monolayer ReSe2 as a platform for studying anisotropic correlated electrons, quantum melting, and coupled one-dimensional electron chains.

cond-mat.str-el

Anyon superfluidity of excitons in quantum Hall bilayers

The charged anyons of a fractional quantum Hall fluid are necessarily dispersionless due to the continuous magnetic translation symmetry. Neutral anyons, however, can disperse, resulting in a much richer space of possible ``daughter'' states when doped to finite density. We discuss a natural realization of such physics in quantum Hall bilayers, where a finite density of excitons with fractional statistics is argued to give rise to `anyonic exciton superfluidity,' the charge-neutral analog of anyon superconductivity. In a balanced bilayer of two Laughlin $ν= 1/3$ states, the minimal interlayer exciton carries anyonic exchange statistics. A finite density of these excitons is argued to yield an exciton superfluid stitched to a specific bulk topological order and edge spectrum. Such superfluidity should be most robust near the direct transition into the Halperin $(112)$ state, and near analogous transitions in the bilayer Jain sequence at total filling $ν_\text{T} = 2\times \frac{n}{2n+1}$. These topological transitions can be described by Chern-Simons QED$_3$, from which we derive several novel and general properties of anyon superfluidity near such transitions, including an anomalously large superfluid stiffness of $κ_\text{s} \propto |δν|^{1/2}$ at layer imbalance fraction $δν$. A notable feature of the phase diagrams we construct is the prevalence of spatial symmetry breaking, driven by an underlying composite Fermi surface. Our results can be directly tested with currently available experimental techniques. We compare our theory with existing data and make concrete predictions for future measurements, including higher-pseudospin exciton superfluids when doping higher Jain fractions.

cond-mat.str-el

Self-doped Crystal from Preempted Band-inversion Transitions

Recent experiments in rhombohedral graphene find evidence for a "self-doped" Wigner crystal (SDC) in which a slightly incommensurate Wigner crystal (WC) coexists with a small Fermi sea. We provide non-perturbative arguments that such SDCs generically arise from preempted band-inversion transitions between commensurate crystals, which motivates simple band-theory criteria for their appearance. Self-consistent Hartree-Fock calculations establish the existence of a SDC consistent with this mechanism in both the $λ$-jellium model and rhombohedral pentalayer graphene (R5G). In the $λ$-jellium model, we identify a SDC phase located between a "halo"-WC and an anomalous Hall crystal (AHC), which would otherwise be connected via a Dirac transition when pinned to commensuration; this contrasts with the WC-AHC transition, which we show cannot be connected by a continuous transition due to a mismatch of symmetry indices. In R5G, we predict a SDC phase located between a WC and a "disqualified" halo anomalous Hall crystal. We discuss in general how the Berry curvature distribution in the parent band affects the appearance of SDC, revealing a novel role of quantum geometry in inducing exotic quantum phases of matter.

cond-mat.str-el

Imaging Electron-Hole Asymmetry in the Quantum Melting of Generalized Wigner Crystals

Two-dimensional moiré materials provide a versatile platform to explore phase transitions in strongly correlated systems. Using scanning tunneling microscopy (STM) we have imaged the density-driven melting of generalized Wigner crystals (GWCs) and Mott insulators (MIs) in electron-doped, near-60° twisted MoSe2 bilayers featuring a triangular moiré superlattice. We observe striking electron-hole asymmetry in GWC melting: hole-doped GWCs yield interaction-driven disordered states whereas electron-doped GWCs melt into delocalized liquid-like states. This asymmetry arises from the broken particle-hole symmetry of the moiré superlattice, which produces electron and hole Fermi pockets with different momentum geometries upon GWC condensation. MI states melt without such asymmetry, consistent with the absence of a symmetry-breaking density modulation. This work provides direct visualization of the novel emergent phases that appear as GWCs undergo quantum melting transitions.

cond-mat.str-el

Theory of quantum anomalous Hall phases in pentalayer rhombohedral graphene moiré structures

Remarkable recent experiments on the moiré structure formed by pentalayer rhombohedral graphene aligned with a hexagonal Boron-Nitride substrate report the discovery of a zero field fractional quantum hall effect. These "(Fractional) Quantum Anomalous Hall" ((F)QAH) phases occur for one sign of a perpendicular displacement field, and correspond, experimentally, to full or partial filling of a valley polarized Chern-$1$ band. Such a band is absent in the non-interacting band structure. Here we show that electron-electron interactions play a crucial role, and present microscopic theoretical calculations demonstrating the emergence of a nearly flat, isolated, Chern-$1$ band and FQAH phases in this system. We also study the four and six-layer analogs and identify parameters where a nearly flat isolated Chern-$1$ band emerges which may be suitable to host FQAH physics.

cond-mat.str-el

Extended quantum anomalous Hall effect in moiré structures: phase transitions and transport

Recent experiments on multilayer rhombohedral graphene have unearthed a number of interesting phenomena in the regime where Integer and Fractional Quantum Anomalous Hall phenomena were previously reported. Specifically at low temperature ($T$) and low applied currents, an "Extended" Integer Quantum Anomalous Hall (EIQAH) is seen over a wide range of the phase diagram. As the current is increased, at low $T$, the EIQAH undergoes a phase transition to a metallic state at generic fillings, and to the fractional quantum anomalous Hall (FQAH) state at the Jain fillings. Increasing temperature at the Jain fillings also leads to an evolution out of the EIQAH to the Jain state. Here we provide an interpretation of many of these observations. We describe the EIQAH as a crystalline state (either of holes doped into the $ν= 1$ state, or an Anomalous Hall Crystal of electrons) that breaks moiré translation symmetry. At generic fillings, we show how an electric current-induced depinning transition of the crystalline order leads to peculiar non-linear current-voltage curves consistent with the experiment. At Jain fillings, we propose that the depinning transition is pre-empted by an equilibrium transition between EIQAH and Jain FQAH states. This transition occurs due to the large polarizability of the Jain FQAH states which enables them to lower their energy effectively in an applied electric field compared to the crystal states. We also discuss the finite temperature evolution in terms of the relative entropies of the crystalline and FQAH states.

cond-mat.str-el

Excitonic quantum criticality: from bilayer graphene to narrow Chern bands

We study a family of excitonic quantum phase transitions describing the evolution of a bilayer metallic state to an inter-layer coherent state where excitons condense. We argue that such transitions can be continuous and exhibit a non-Fermi liquid counterflow response ${ρ_{\mathrm{counterflow}}(ω)\simω^{2/z}}$ that directly encodes the dynamical critical exponent $z$. Our calculations are performed within a controlled expansion around $z = 2$. This physics is relevant to any system with spin, valley, or layer degrees of freedom. We consider two contexts for excitonic quantum criticality: (1) a weakly interacting graphene bilayer, and (2) a system of two narrow, half-filled Chern bands at zero external magnetic field, with total Chern number $C_{\mathrm{tot}}=0$, which may soon be realizable in moiré materials. The latter system hosts a time-reversed pair of composite Fermi liquid states, and the condensation of excitons of the composite fermions leads to an exotic exciton insulator* state with a charge neutral Fermi surface. Our work sheds new light on the physics of inter-layer coherence transitions in 2D materials.

cond-mat.str-el

Stability of Anomalous Hall Crystals in multilayer rhombohedral graphene

Recent experiments showing an integer quantum anomalous Hall effect in pentalayer rhombohedral graphene have been interpreted in terms of a valley-polarized interaction-induced Chern band. The resulting many-body state can be viewed as an Anomalous Hall Crystal (AHC), with a further coupling to a weak moiré potential. We explain the origin of the Chern band and the corresponding AHC in the pentalayer system. To describe the competition between AHC and Wigner Crystal (WC) phases, we propose a simplified low-energy description that predicts the Hartree-Fock phase diagram to good accuracy. This theory can be fruitfully viewed as `superconducting ring' in momentum space, where the emergence of Chern number is analogous to the flux quantization in a Little-Parks experiment. We discuss the possible role of the moiré potential, and emphasize that even if in the moiré-less limit, the AHC is not favored (beyond Hartree-Fock) over a correlated Fermi liquid, the moiré potential will push the system into a `moiré-enabled AHC'. We also suggest that there is a range of alignment angles between R5G and hBN where a $C = 2$ insulator may be found at integer filling.

cond-mat.str-el

Excitonic Chern insulator and kinetic ferromagnetism in MoTe$_2$/WSe$_2$ moiré bilayer

We propose a new mechanism for quantum anomalous Hall (QAH) effect in the AB stacked MoTe$_2$/WSe$_2$ system. Based on the observation that the inter-layer tunneling is suppressed in the AB stacking, we consider a model with two layers coupled through the Coulomb interaction. The moiré lattices of the two layers are shifted to form a honeycomb lattice together. Initially, the system is in a layer-polarized Mott insulator at $ν_T=1$. But with a displacement field, an equal number of holes and electrons are doped into the two layers respectively and they form inter-layer exciton condensation. Through mean field theory, we find p$\pm$ip exciton condensation in a certain parameter regime, which leads to a Chern insulator with Chern number $C=\pm 1$. The valleys are polarized due to the kinetic energy instead of interaction. But the polarization in the two layers can be either the same or opposite depending on small perturbations away from a symmetric point. As a result, both valley polarized and inter-valley coherent (IVC) Chern insulator phases are possible. The latter has the same spin $S_z$ in the two layers.

cond-mat.str-el

Evolution between quantum Hall and conducting phases: simple models and some results

Quantum many particle systems in which the kinetic energy, strong correlations, and band topology are all important pose an interesting and topical challenge. Here we introduce and study particularly simple models where all of these elements are present. We consider interacting quantum particles in two dimensions in a strong magnetic field such that the Hilbert space is restricted to the Lowest Landau Level (LLL). This is the familiar quantum Hall regime with rich physics determined by the particle filling and statistics. A periodic potential with a unit cell enclosing one flux quantum broadens the LLL into a Chern band with a finite bandwidth. The states obtained in the quantum Hall regime evolve into conducting states in the limit of large bandwidth. We study this evolution in detail for the specific case of bosons at filling factor $ν= 1$. In the quantum Hall regime the ground state at this filling is a gapped quantum hall state (the "bosonic Pfaffian") which may be viewed as descending from a (bosonic) composite fermi liquid. At large bandwidth the ground state is a bosonic superfluid. We show how both phases and their evolution can be described within a single theoretical framework based on a LLL composite fermion construction. Building on our previous work on the bosonic composite fermi liquid, we show that the evolution into the superfluid can be usefully described by a non-commutative quantum field theory in a periodic potential.

cond-mat.str-el

Non-commutative field theory and composite Fermi Liquids in some quantum Hall systems

Composite Fermi liquid metals arise at certain special filling fractions in the quantum Hall regime and play an important role as parent states of gapped states with quantized Hall response. They have been successfully described by the Halperin-Lee-Read (HLR) theory of a Fermi surface of composite fermions coupled to a $U(1)$ gauge field with a Chern-Simons term. However, the validity of the HLR description when the microscopic system is restricted to a single Landau has not been clear. Here for the specific case of bosons at filling $ν= 1$, we build on earlier work from the 1990s to formulate a low energy description that takes the form of a {\em non-commutative} field theory. This theory has a Fermi surface of composite fermions coupled to a $U(1)$ gauge field with no Chern-Simons term but with the feature that all fields are defined in a non-commutative spacetime. An approximate mapping of the long wavelength, small amplitude gauge fluctuations yields a commutative effective field theory which, remarkably, takes the HLR form but with microscopic parameters correctly determined by the interaction strength. Extensions to some other composite fermi liquids, and to other related states of matter are discussed.

cond-mat.str-el

Ferromagnetism in narrow bands of moiré superlattices

Many graphene moiré superlattices host narrow bands with non-zero valley Chern numbers. We provide analytical and numerical evidence for a robust spin and/or valley polarized insulator at total integer band filling in nearly flat bands of several different moiré materials. In the limit of a perfectly flat band, we present analytical arguments in favor of the ferromagnetic state substantiated by numerical calculations. Further, we numerically evaluate its stability for a finite bandwidth. We provide exact diagonalization results for models appropriate for ABC trilayer graphene aligned with hBN, twisted double bilayer graphene, and twisted bilayer graphene aligned with hBN. We also provide DMRG results for a honeycomb lattice with a quasi-flat band and non-zero Chern number, which extend our results to larger system sizes. We find a maximally spin and valley polarized insulator at all integer fillings when the band is sufficiently flat. We also show that interactions may induce effective dispersive terms strong enough to destabilize this state. These results still hold in the case of zero valley Chern number (for example, trivial side of TLG/hBN). We give an intuitive picture based on extended Wannier orbitals, and emphasize the role of the quantum geometry of the band, whose microscopic details may enhance or weaken ferromagnetism in moiré materials.

cond-mat.str-el

Bosonic Integer Quantum Hall States without Landau Levels on Square Lattice

We study an interacting two-component hard-core bosons on square lattice for which, in the presence of staggered magnetic flux, the ground state is a bosonic integer quantum Hall (BIQH) state. Using a coupled-wire bosonization approach, we analytically show this model exhibits a BIQH state at total charge half filling associated with a symmetry-protected topological phase under $U(1)$ charge conservation. These theoretical expectations are verified, using the infinite density matrix renormalization group method, by providing numerical evidences for: (i) a quantized Hall conductance $σ_{xy}=\pm2$, and (ii) two counter-propagating gapless edge modes. Our model is a bosonic cousin of the fermionic Haldane model and serves as an additional case of analogy between bosonic and fermionic quantum Hall states.

cond-mat.quant-gas