arXiv subjects

Zhiliang Yuan

Publications and source records attributed to Zhiliang Yuan.

At least 19 recordsLinked to original sources

arXiv2026

Transmitter-device-independent quantum key distribution

Transmitter-side device dependence is a longstanding yet implicit problem in quantum key distribution (QKD), in contrast to the thoroughly addressed measurement-side case. Quantum steering, which intrinsically distinguishes the roles of sender and receiver in entanglement certification, offers a natural route to lifting trust assumptions on the transmitter. Existing one-sided device-independent (1sDI) protocols primarily exploit steering as a security resource, and provoke a signaling loophole in the transmitter-receiver architecture. Here we formalize transmitter-device-independence on the basis of faithful quantum steering and propose a transmitter-device-independent (TDI) QKD protocol within 1sDI framework that closes this loophole through introducing a photon storage, thereby eliminating transmitter-side device vulnerabilities. In a proof-of-principle experiment we validate the feasibility of the TDI protocol, achieving a key-rate in the asymptotic limit of 410~bps over 27~km spool fiber. By delivering TDI security while retaining strong loss tolerance, our approach helps bridge the gap between security and practicality for real-world QKD deployments.

quant-ph↗

arXiv2026

Fiber-integrated Quantum Frequency Conversion for Long-distance Quantum Networking

Signal photons emitted by quantum nodes typically fall outside the low-loss telecom window of optical fibers, leading to severe transmission losses. Quantum frequency conversion (QFC) offers an effective optical interface that bridges quantum nodes with telecom-band channels, enabling long-distance quantum communication. In this work, we demonstrate a compact, fiber-integrated QFC system with low noise and a high signal-to-noise ratio (SNR). Using a periodically poled lithium niobate (PPLN) waveguide, input photons at 637.2 nm are down-converted to telecom photons at 1588.3 nm. Our system achieves a total conversion efficiency of approximately 9%, with pump-induced noise suppressed to 154 Hz. For input photon rates of 32.7, 118.0, and 327.7 kHz, the corresponding SNRs are 12.3, 43.9, and 117.8, respectively. We further develop a theoretical model to simulate the entanglement fidelity between nitrogen-vacancy (NV) center spins and the frequency-converted telecom photons. At the emission rate of an NV center, our QFC system maintains an expected fidelity exceeding 52% over a transmission distance of 100 km. These findings highlight the potential of our QFC system for scalable, long-distance quantum networking.

quant-ph↗

arXiv2026

Engineering energy-time entanglement from resonance fluorescence

Resonance fluorescence from a coherently driven two-level emitter is a minimal quantum optical field that combines phase coherence with single-photon-level nonlinearity. Here we show that it can be engineered, using only passive linear interferometry, into energy-time entanglement. By injecting resonance fluorescence from a single quantum dot into an asymmetric Mach--Zehnder interferometer operated near destructive interference of the single-photon component, we generate an output field whose coincidence statistics are dominated by the simultaneous two-photon contribution |2> and the temporally separated photon-pair contribution |11>. In a Franson geometry, these two sectors are resolved on the coincidence-delay axis, and both exhibit high-visibility nonlocal interference fringes and violate the Clauser--Horne--Shimony--Holt Bell inequality. Our results reveal a general route for engineering entanglement from resonance fluorescence using passive optics.

quant-ph↗

arXiv2025

Broadband telecom single-photon emissions from InAs/InP quantum dots grown by MOVPE droplet epitaxy

The development of quantum materials for single-photon emission is crucial for the advancement of quantum information technology. Although significant advancement has been witnessed in recent years for single photon sources in near infrared band (λ~700-1000 nm), several challenges have yet to be addressed for ideal single photon emission at the telecommunication band. In this study, we present a droplet-epitaxy strategy for O-band to C-band single-photon source based semiconductor quantum dots (QDs) using metal-organic vapor-phase epitaxy (MOVPE). Via investigating the growth conditions of the epitaxial process, we have successfully synthesized InAs/InP QDs with narrow emission lines spanning a broad spectral range of λ~1200-1600 nm. The morphological and optical properties of the samples were characterized using atomic force microscopy and micro photoluminescence spectroscopy. The recorded single-photon purity of a plain QD structure reaches (g(2)(0) = 0.16), with a radiative recombination lifetime as short as 1.5 ns. This work provides a crucial platform for future research on integrated microcavity enhancement techniques and coupled QDs with other quantum photonics in the telecom bands, offering significant prospects for quantum network applications.

physics.optics↗

arXiv2025

Bell Inequality Violation with Vacuum-One-Photon Number Superposition States

Entanglement is a central resource in quantum technologies, and the realization of photonic entanglement necessarily relies on interaction with matter. Resonance fluorescence (RF), originating from the coherent interaction between a driving field and a two-level system, plays a pivotal role in quantum optics. Here, we demonstrate a novel route to entanglement generation based on RF from a single quantum dot. Rather than relying on generation of multiphoton states, our approach directly exploits vacuum-one-photon number superposition states created under resonant excitation. By delocalizing this superposition via a beam splitter, we realize time-bin entanglement and observe a clear violation of the Clauser-Horn-Shimony-Holt Bell inequality using Franson-type interferometry. Our scheme removes the need for multiphoton generation, simplifies the experimental requirements, and establishes a scalable pathway toward solid-state entangled photon sources.

quant-ph↗

arXiv2025

Two-photon interference between mutually-detuned resonance fluorescence signals scattered off a semiconductor quantum dot

The radiative linewidth of a two-level emitter (TLE) fundamentally limits the bandwidth available for quantum information processing. Despite its importance, no prior experiment has systematically examined how driving detuning affects the indistinguishability of photons scattered from a TLE - a parameter critical for photonic quantum computing. Here, we perform post-selective two-photon interference measurements between mutually detuned resonance fluorescence signals from an InAs quantum dot embedded in a micropillar cavity. At small mutual laser detunings (<=0.5GHz), the results are accurately described by the pure-state model [Nat. Commun. 16, 6453 (2025)], which treats all resonance-fluorescence photons as spontaneous emission. At larger detunings, we uncover an anomalous feature in the two-photon interference, where the normalised second-order correlation function under orthogonal polarisations yields g2_vert(0) < 0.5.

quant-ph↗

arXiv2025

High-Performance Fully Passive Discrete-State Continuous-Variable Quantum Key Distribution With Local Local Oscillator

We propose and demonstrate a fully passive discrete-state continuous-variable quantum key distribution (CV-QKD), which can eliminate all modulator side channels on the source side, using a local local oscillator (LLO). The CV-QKD system achieves a maximum transmission length of 100 km with a repetition rate of 1 GHz using specially designed phase rotation and discretization methods, and the corresponding secret key bit rate is 127 kbps, as estimated based on the amplitude of prepared states at the transmitter, as well as the first- and second-order moments of quadratures at the receiver by employing the convex optimization without imposing any assumptions on the quantum channel. The performance of the protocol is similar to that of modulated CV LLO protocols and better than those of passive discrete-variable and CV protocols. Our protocol is expected to play an important role in the quantum metropolitan area networks and quantum access networks with high realistic security.

quant-ph↗

arXiv2025

Steering nonlocality in high-speed telecommunication system without detection loophole

Nonlocal correlation represents the key feature of quantum mechanics, and is an exploitable resource in quantum information processing. However, the loophole issues and the associated applicability compromises hamper the practical applications. We report the first time-bin entangled detection-loophole-free steering nonlocality demonstration in a fully chip-fiber telecommunication system, with an ultra-fast measurement switching rate (1.25~GHz). In this endeavor, we propose the phase-encoding measurement scheme to adapt the system to time-bin degree of freedom, and design and fabricate a low-loss silicon chip for efficient entanglement generation. An asymmetric configuration is introduced to mimic the active measurement implementation at the steering party thus bypassing the phase modulation loss. Consequently, we build a fiber-optic setup that can overcome the detection efficiency required by conclusive quantum steering with multiple actively switched measurement settings. Our setup presents an immediate platform for exploring applications based on steering nonlocality, especially for quantum communication.

quant-ph↗

arXiv2025

Bright Heralded Single-Photon Source Saturating Theoretical Single-photon Purity

Single-photon source is the cornerstone for modern quantum information processing. The present work derives the theoretical limit of single-photon purity for general parametric heralded single-photon sources, and subsequently demonstrates a bright, gigahertz-pulsed heralded source with the purity saturating the limit. By stimulating spontaneous four-wave mixing effect in the silicon spiral waveguide, this on-chip source is measured to have a coincidence rate exceeding 1.5~MHz at a coincidence-to-accidental ratio (CAR) of 16.77 in the photon pair correlation experiment. The single-photon purity of this source, quantified by the heralded auto-correlation function $g^{(2)}_\text{h}(0)$, is measured by a heralded Hanbury Brown--Twiss setup to reach the theoretical limit with the lowest value of $0.00094 \pm 0.00002$ obtained at a coincidence rate of 0.8~kHz and a CAR of 2220. The performance improvements are attributed to effective spectral filtering suppressing the noise as well as the coherent pump condition helped by optical injection locking. The reported results provide a reliable standard for benchmarking heralded single-photon sources and present a state-of-the-art heralded source for quantum information processing.

quant-ph↗

arXiv2025

Coherence in resonance fluorescence

Resonance fluorescence of a two-level emitter displays persistently anti-bunching irrespective of the excitation intensity, but inherits the driving laser's linewidth under weak monochromatic excitation. These properties are commonly explained in terms of two disjoined pictures, i.e., the emitter's single photon saturation or passively scattering light. Here, we propose a unified model that treats all fluorescence photons as spontaneous emission, one at a time, and can explain simultaneously both the spectral and correlation properties of the emission. We theoretically derive the excitation power dependencies, measurable at the single-photon incidence level, of the first-order coherence of the whole resonance fluorescence and super-bunching of the spectrally filtered, followed by experimental confirmation on a semiconductor quantum dot micro-pillar device. Furthermore, our model explains peculiar coincidence bunching observed in phase-dependent two-photon interference experiments. Our work provides an intuitive understanding of coherent light-matter interaction and may stimulate new applications.

quant-ph↗

arXiv2024

Independent Optical Frequency Combs Powered 546 km Field Test of Twin-Field Quantum Key Distribution

Owing to its repeater-like rate-loss scaling, twin-field quantum key distribution (TF-QKD) has repeatedly exhibited in laboratory its superiority for secure communication over record fiber lengths. Field trials pose a new set of challenges however, which must be addressed before the technology's roll-out into real-world. Here, we verify in field the viability of using independent optical frequency combs -- installed at sites separated by a straight-line distance of 300~km -- to achieve a versatile TF-QKD setup that has no need for optical frequency dissemination and thus enables an open and network-friendly fiber configuration. Over 546 and 603 km symmetric links, we record a finite-size secure key rate (SKR) of 0.53~bit/s and an asymptotic SKR of 0.12 bit/s, respectively. Of practical importance, the setup is demonstrated to support 44~km fiber asymmetry in the 452 km link. Our work marks an important step towards incorporation of long-haul fiber links into large quantum networks.

quant-ph↗

arXiv2024

Post-Measurement Pairing Quantum Key Distribution with Local Optical Frequency Standard

The idea of post-measurement coincidence pairing simplifies substantially long-distance, repeater-like quantum key distribution (QKD) by eliminating the need for tracking the differential phase of the users' lasers. However, optical frequency tracking remains necessary and can become a severe burden in future deployment of multi-node quantum networks. Here, we resolve this problem by referencing each user's laser to an absolute frequency standard and demonstrate a practical post-measurement pairing QKD with excellent long-term stability. We confirm the setup's repeater-like behavior and achieve a finite-size secure key rate (SKR) of 15.94 bit/s over 504 km fiber, which overcomes the absolute repeaterless bound by 1.28 times. Over a fiber length 100 km, the setup delivers an impressive SKR of 285.68 kbit/s. Our work paves the way towards an efficient muti-user quantum network with the local frequency standard.

quant-ph↗

arXiv2023

Experimental Quantum Communication Overcomes the Rate-loss Limit without Global Phase Tracking

Secure key rate (SKR) of point-point quantum key distribution (QKD) is fundamentally bounded by the rate-loss limit. Recent breakthrough of twin-field (TF) QKD can overcome this limit and enables long distance quantum communication, but its implementation necessitates complex global phase tracking and requires strong phase references which not only add to noise but also reduce the duty cycle for quantum transmission. Here, we resolve these shortcomings, and importantly achieve even higher SKRs than TF-QKD, via implementing an innovative but simpler measurement-device-independent QKD which realizes repeater-like communication through asynchronous coincidence pairing. Over 413 and 508 km optical fibers, we achieve finite-size SKRs of 590.61 and 42.64 bit/s, which are respectively 1.80 and 4.08 times of their corresponding absolute rate limits. Significantly, the SKR at 306 km exceeds 5 kbit/s and meets the bitrate requirement for live one-time-pad encryption of voice communication. Our work will bring forward economical and efficient intercity quantum-secure networks.

quant-ph↗

arXiv2023

The Mollow triplets under few-photon excitation

Resonant excitation is an essential tool in the development of semiconductor quantum dots (QDs) for quantum information processing. One central challenge is to enable a transparent access to the QD signal without post-selection information loss. A viable path is through cavity enhancement, which has successfully lifted the resonantly scattered field strength over the laser background under \emph{weak} excitation. Here, we extend this success to the \emph{saturation} regime using a QD-micropillar device with a Purcell factor of 10.9 and an ultra-low background cavity reflectivity of just 0.0089. We achieve a signal to background ratio of 50 and an overall system responsivity of 3~\%, i.e., we detect on average 0.03 resonantly scattered single photons for every incident laser photon. Raising the excitation to the few-photon level, the QD response is brought into saturation where we observe the Mollow triplets as well as the associated cascade single photon emissions, without resort to any laser background rejection technique. Our work offers a new perspective toward QD cavity interface that is not restricted by the laser background.

quant-ph↗

arXiv2023

Suppression of patterning effect using IQ modulator for high-speed quantum key distribution systems

Quantum key distribution (QKD) is an attractive technology for distributing secret encryption keys between distant users. The decoy-state technique has drastically improved its practicality and performance, and has been widely adopted in commercial systems. However, conventional intensity modulators can introduce security side channels in high speed QKD systems because of their non-stationary working points for decoy-state generation. Here, we analyze the transfer function of an in-phase/quadrature (IQ) modulator and reveal its superiority for stable decoy-state generation, followed by an experimental demonstration. Thanks to their convenient two-level modulation and inherent high speed, IQ modulators are ideal for use in high-speed decoy-state QKD systems.

quant-ph↗

arXiv2023

Controlled entanglement source for quantum cryptography

Quantum entanglement has become an essential resource in quantum information processing. Existing works employ entangled quantum states to perform various tasks, while little attention is paid to the control of the resource. In this work, we propose a simple protocol to upgrade an entanglement source with access control through phase randomization at the optical pump. The enhanced source can effectively control all users in utilizing the entanglement resource to implement quantum cryptography. In addition, we show this control can act as a practical countermeasure against memory attack on device-independent quantum key distribution at a negligible cost. To demonstrate the feasibility of our protocol, we implement an experimental setup using just off-the-shelf components and characterize its performance accordingly.

quant-ph↗

arXiv2023

Twin-field quantum key distribution without optical frequency dissemination

Twin-field (TF) quantum key distribution (QKD) has rapidly risen as the most viable solution to long-distance secure fibre communication thanks to its fundamentally repeater-like rate-loss scaling. However, its implementation complexity, if not successfully addressed, could impede or even prevent its advance into real-world. To satisfy its requirement for twin-field coherence, all present setups adopted essentially a gigantic, resource-inefficient interferometer structure that lacks scalability that mature QKD systems provide with simplex quantum links. Here we introduce a novel technique that can stabilise an open channel without using a closed interferometer and has general applicability to phase-sensitive quantum communications. Using locally generated frequency combs to establish mutual coherence, we develop a simple and versatile TF-QKD setup that does not need service fibre and can operate over links of 100 km asymmetry. We confirm the setup's repeater-like behaviour and obtain a finite-size rate of 0.32 bit/s at a distance of 615.6 km.

quant-ph↗

arXiv2023

Ultra-narrowband interference circuits enable low-noise and high-rate photon counting for InGaAs/InP avalanche photodiodes

Afterpulsing noise in InGaAs/InP single photon avalanche photodiodes (APDs) is caused by carrier trapping and can be suppressed successfully through limiting the avalanche charge via sub-nanosecond gating. Detection of faint avalanches requires an electronic circuit that is able to effectively remove the gate-induced capacitive response while keeping photon signals intact. Here we demonstrate a novel ultra-narrowband interference circuit (UNIC) that can reject the capacitive response by up to 80 dB per stage with little distortion to avalanche signals. Cascading two UNIC's in a readout circuit, we were able to enable high count rate of up to 700 MC/s and low afterpulsing of 0.5 % at a detection efficiency of 25.3 % for 1.25 GHz sinusoidally gated InGaAs/InP APDs. At -30 degree C, we measured 1 % afterpulsing at a detection efficiency of 21.2 %.

quant-ph↗