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Zhirong Huang

Publications and source records attributed to Zhirong Huang.

At least 37 records · Page 2Linked to original sources

Active Q-switched X-Ray Regenerative Amplifier Free-Electron Laser

Despite tremendous progress in x-ray free-electron laser (FEL) science over the last decade, future applications still demand fully coherent, stable x-rays that have not been demonstrated in existing X-ray FEL facilities. In this Letter, we describe an active Q-switched x-ray regenerative amplifier FEL scheme to produce fully coherent, high-brightness, hard x rays at a high-repetition rate. By using simple electron-beam phase space manipulation, we show this scheme is flexible in controlling the x-ray cavity quality factor Q and hence the output radiation. We report both theoretical and numerical studies on this scheme with a wide range of accelerator, x-ray cavity, and undulator parameters.

physics.acc-ph↗

Multiplexed Photoinjector Optimization for High-Repetition-Rate Free-Electron Lasers

The multiplexing capabilities of superconducting X-ray free-electron lasers (FELs) have gained much attention in recent years. The demanding requirements for photon properties from multiple undulator lines necessitate more flexible beam manipulation techniques to achieve the goal of "beam on demand". In this paper, we investigate a multiplexed configuration for the photoinjector of high-repetition-rate FELs that aims to simultaneously provide low-emittance electron beams of different charges. A parallel, multi-objective genetic algorithm is implemented for the photoinjector parameter optimization. The proposed configuration could drastically enhance the flexibility of beam manipulation to improve multiplexing capabilities and realize the full potential of the facility.

physics.acc-ph↗

Ultra-compact attosecond X-ray free-electron lasers utilizing unique beams from plasma-based acceleration and an optical undulator

Accelerator-based X-ray free-electron lasers (XFELs) are the latest addition to the revolutionary tools of discovery for the 21st century. The two major components of an XFEL are an accelerator-produced electron beam and a magnetic undulator which tend to be kilometer-scale long and expensive. Here, we present an ultra-compact scheme to produce 10s of attosecond X-ray pulses with several GW peak power utilizing a novel aspect of the FEL instability using a highly chirped, pre-bunched and ultra-bright electron beam from a plasma-based accelerator interacting with an optical undulator. The self-selection of electrons from the combination of a highly chirped and pre-bunched beam leads to the stable generation of attosecond X-ray pulses. Furthermore, two-color attosecond pulses with sub-femtosecond separation can be produced by adjusting the energy distribution of the electron beam so that multiple FEL resonances occur at different locations within the beam. Such a tunable coherent attosecond X-ray sources may open up a new area of attosecond science enabled by X-ray attosecond pump/probe techniques.

physics.plasm-ph↗

Femtosecond-Terawatt Hard X Ray Pulse Generation with Chirped Pulse Amplification on a Free Electron Laser

Advances of high intensity lasers have opened up the field of strong field physics and led to a broad range of technological applications. Recent x ray laser sources and optics development makes it possible to obtain extremely high intensity and brightness at x ray wavelengths. In this paper, we present a system design that implements chirped pulse amplification for hard x ray free electron lasers. Numerical modeling with realistic experimental parameters show that near-transform-limit single-femtosecond hard x ray laser pulses with peak power exceeding 1 TW and brightness exceeding $4\times10^{35}~$s$^{-1}$mm$^{-2}$mrad$^{-2}$0.1\%bandwdith$^{-1}$ can be consistently generated. Realization of such beam qualities is essential for establishing systematic and quantitative understanding of strong field x-ray physics and nonlinear x ray optics phenomena.

physics.optics↗

XCC: An X-ray FEL-based $γγ$ Collider Higgs Factory

This report describes the design of a $γγ$ Higgs factory in which 62.8 GeV electron beams collide with 1 keV X-ray free electron laser (XFEL) beams to produce colliding beams of 62.5 GeV photons. The Higgs boson production rate is 34,000 Higgs bosons per $10^7$ second year, roughly the same as the ILC Higgs rate. The electron accelerator is based on cold copper distributed coupling (C$^3$) accelerator technology. The 0.7 J pulse energy of the XFEL represents a 300-fold increase over the pulse energy of current soft x-ray FEL's. Design challenges are discussed, along with the R\&D to address them, including demonstrators.

hep-ex↗

Field Analysis for a Highly-Overmoded Iris Line, with Application to THz Radiation Transport at LCLS

Vector field analysis is presented for a highly overmoded iris-line structure that can act as a medium of transportation for THz radiation. The axisymmetric structure is capable of supporting hybrid modes with desirable features such as low propagation loss, uniformly linear polarization and approximately-Gaussian intensity profile across the iris. A specific application that can benefit from these features is the transportation of THz undulator radiation over hundreds of meters to reach the experimental halls at the LCLS facility, SLAC, Stanford. Such a structure has been modelled before as a boundary-value problem using Vainstein's impedance boundary condition and assuming infinitely-thin screens. Given that physical realizations of such screens must have finite thickness and that the THz wavelength in the 3-15 THz range is expected to be smaller than convenient screen thicknesses in practice, the question of the impact of finite screen thickness on propagation performance becomes rather pressing. To address this question, we present a mode-matching analysis of the structure, with finite screen thickness and perturbatively clustered (localized) field expansions, for computational feasibility. The effect of screen thickness is seen to lower the attenuation constant on the iris line, which is dominated by diffraction loss. The propagation loss predictions based on the Vainstein-model are compared with the numerical results from mode-matching for infinitely-thin screens, where the former method is observed to agree with the numerical results better at higher Fresnel numbers (highly-overmoded structures). The properties of the dominant mode fields are formally derived from first principles and a recommended approach is discussed for the inclusion of screen-thickness effects into propagation loss estimations.

physics.acc-ph↗

C$^3$: A "Cool" Route to the Higgs Boson and Beyond

We present a proposal for a cold copper distributed coupling accelerator that can provide a rapid route to precision Higgs physics with a compact 8 km footprint. This proposal is based on recent advances that increase the efficiency and operating gradient of a normal conducting accelerator. This technology also provides an $e^{+}e^{-}$ collider path to physics at multi-TeV energies. In this article, we describe our vision for this technology and the near-term R&D program needed to pursue it.

hep-ex↗

Attosecond Coherent Electron Motion in Auger-Meitner Decay

In quantum systems, coherent superpositions of electronic states evolve on ultrafast timescales (few femtosecond to attosecond, 1 as = 0.001 fs = 10^{-18} s), leading to a time dependent charge density. Here we exploit the first attosecond soft x-ray pulses produced by an x-ray free-electron laser to induce a coherent core-hole excitation in nitric oxide. Using an additional circularly polarized infrared laser pulse we create a clock to time-resolve the electron dynamics, and demonstrate control of the coherent electron motion by tuning the photon energy of the x-ray pulse. Core-excited states offer a fundamental test bed for studying coherent electron dynamics in highly excited and strongly correlated matter.

physics.chem-ph↗

A self-consistent refractive index model for fast simulation of free-electron lasers

Modern x-ray free-electron lasers (XFELs) produce x-ray pulses of exceptional transverse coherence. This is due largely to the process of optical guiding by which the radiation is both refractively guided by the bunched electron beam and gain guided by the preferential amplification of on-axis radiation. These effects may be summarized by an effective index of refraction, which has been used in the past to study the transverse dynamics of the FEL process with significant simplifications and approximations, but never fully self-consistently. We present here a self-consistent method for studying high gain FELs in the linear regime by approximating the FEL equations to second-order in the lateral displacement from the nominal electron beam axis. This is made possible by casting the FEL equations in the language of optical fibers with an appropriately chosen refractive index. We demonstrate that this approach is both fast and highly accurate, indicating that the most important FEL dynamics are inherently second-order. In its full form our method can capture the effects of transverse offsets in both the x-ray beam and the electron beam, making it a versatile tool for studying non-ideal effects in seeded FELs, regenerative amplifier XFELs, and even self-amplified spontaneous emission (SASE) FELs.

physics.acc-ph↗

Measurements of undulator radiation power noise and comparison with $\textit{ab initio}$ calculations

Generally, turn-to-turn fluctuations of synchrotron radiation power in a storage ring depend on the 6D phase-space distribution of the electron bunch. This effect is related to the interference of fields radiated by different electrons. Changes in the relative electron positions and velocities inside the bunch result in fluctuations in the total emitted energy per pass in a synchrotron radiation source. This effect has been previously described assuming constant and equal electron velocities before entering the synchrotron radiation source. In this paper, we present a generalized formula for the fluctuations with a non-negligible beam divergence. Further, we corroborate this formula in a dedicated experiment with undulator radiation in the Integrable Optics Test Accelerator (IOTA) storage ring at Fermilab. Lastly, possible applications in beam instrumentation are discussed.

physics.acc-ph↗

Transverse beam emittance measurement by undulator radiation power noise

Generally, turn-to-turn power fluctuations of incoherent spontaneous synchrotron radiation in a storage ring depend on the 6D phase-space distribution of the electron bunch. In some cases, if only one parameter of the distribution is unknown, this parameter can be determined from the measured magnitude of these power fluctuations. In this Letter, we report an absolute measurement (no free parameters or calibration) of a small vertical emittance (5--15 nm rms) of a flat beam by this method, under conditions, when it is unresolvable by a conventional synchrotron light beam size monitor.

physics.acc-ph↗

Site-specific Interrogation of an Ionic Chiral Fragment During Photolysis Using an X-ray Free-Electron Laser

Short-wavelength free-electron lasers with their ultrashort pulses at high intensities have originated new approaches for tracking molecular dynamics from the vista of specific sites. X-ray pump X-ray probe schemes even allow to address individual atomic constituents with a 'trigger'-event that preludes the subsequent molecular dynamics while being able to selectively probe the evolving structure with a time-delayed second X-ray pulse. Here, we use a linearly polarized X-ray photon to trigger the photolysis of a prototypical chiral molecule, namely trifluoromethyloxirane (C$_3$H$_3$F$_3$O), at the fluorine K-edge at around 700 eV. The evolving fluorine-containing fragments are then probed by a second, circularly polarized X-ray pulse of higher photon energy in order to investigate the chemically shifted inner-shell electrons of the ionic motherfragment for their stereochemical sensitivity. We experimentally demonstrate and theoretically support how two-color X-ray pump X-ray probe experiments with polarization control enable XFELs as tools for chiral recognition.

physics.chem-ph↗

Temporal X-ray Reconstruction using Temporal and Spectral Measurements at LCLS

Transverse deflecting structures (TDS) are widely used in accelerator physics to measure the longitudinal density of particle bunches. When used in combination with a dispersive section, the whole longitudinal phase space density can be imaged. At the Linac Coherent Light Source (LCLS), the installation of such a device downstream of the undulators enables the reconstruction of the X-ray temporal intensity profile by comparing longitudinal phase space distributions with lasing on and lasing off. However, the resolution of this TDS is limited to around 1 fs rms (root mean square), and therefore, it is not possible to resolve single self-amplified spontaneous emission (SASE) spikes within one X-ray photon pulse. By combining the power spectrum from a high resolution photon spectrometer and the temporal structure from the TDS, the overall resolution is enhanced, thus allowing the observation of temporal, single SASE spikes. The combined data from the spectrometer and the TDS is analyzed using an iterative algorithm to obtain the actual intensity profile. In this paper, we present some improvements to the reconstruction algorithm as well as real data taken at LCLS.

physics.acc-ph↗

Statistical properties of undulator radiation in the IOTA storage ring

We study turn-by-turn fluctuations in the number of spontaneously emitted photons from an undulator, installed in the Integrable Optics Test Accelerator (IOTA) electron storage ring at Fermilab. A theoretical model is presented, showing the relative contributions due to the discrete nature of light emission and to the incoherent sum of fields from different electrons in the bunch. The model is compared with a previous experiment at Brookhaven and with new experiments we carried out at IOTA. Our experiments focused on the case of a large number of longitudinal and transverse radiation modes, a regime where photon shot noise is significant and the total magnitude of the fluctuations is very small. The experimental and data analysis techniques, required to reach the desired sensitivity, are detailed. We discuss how the model and the experiment provide insights into this emission regime, enable diagnostics of small beam sizes, and improve our understanding of beam lifetime in IOTA.

physics.acc-ph↗

Attosecond Transient Absorption Spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the resultant photoproducts. The spectral bandwidth inherent to attosecond pulses is wide compared to the resonant features typically probed, which generally precludes the application of this technique in the attosecond regime. In this paper we propose and demonstrate a new technique to conduct transient absorption spectroscopy with broad bandwidth attosecond pulses with the aid of ghost imaging, recovering sub-bandwidth resolution in photoproduct-based absorption measurements.

physics.chem-ph↗

Phase-stable self-modulation of an electron-beam in a magnetic wiggler

Electron-beams with a sinusoidal energy modulation have the potential to emit sub-femtosecond x-ray pulses in a free-electron laser. The energy modulation can be generated by overlapping a powerful infrared laser with an electron-beam in a magnetic wiggler. Here we report on a new infrared source for this modulation, coherent radiation from the electron-beam itself. In this self-modulation process, the current spike on the tail of the electron-beam radiates coherently at the resonant wavelength of the wiggler, producing a six-period carrier-envelope-phase (CEP) stable infrared field with gigawatt power. This field creates a few MeV, phase-stable modulation in the electron-beam core. The modulated electron-beam is immediately useful for generating sub-femtosecond x-ray pulses at any machine repetition rate, and the CEP-stable infrared field may find application as an experimental pump or timing diagnostic.

physics.acc-ph↗

Tunable Isolated Attosecond X-ray Pulses with Gigawatt Peak Power from a Free-Electron Laser

The quantum mechanical motion of electrons in molecules and solids occurs on the sub-femtosecond timescale. Consequently, the study of ultrafast electronic phenomena requires the generation of laser pulses shorter than 1 fs and of sufficient intensity to interact with their target with high probability. Probing these dynamics with atomic-site specificity requires the extension of sub-femtosecond pulses to the soft X-ray spectral region. Here we report the generation of isolated GW-scale soft X-ray attosecond pulses with an X-ray free-electron laser. Our source has a pulse energy that is six orders of magnitude larger than any other source of isolated attosecond pulses in the soft X-ray spectral region, with a peak power in the tens of gigawatts. This unique combination of high intensity, high photon energy and short pulse duration enables the investigation of electron dynamics with X-ray non-linear spectroscopy and single-particle imaging.

physics.optics↗

Transverse forces in planar symmetric dielectric laser-driven accelerators

The use of dielectric microstructures driven by solid state lasers to accelerate charged particles or to transversely deflect them is a growing area of scientific interest with an international collaboration of researchers working to develop this concept. Many experimental efforts and new designs use a planar symmetric geometry with sub-micron apertures for the particle beam. We provide a general theoretical framework for the electromagnetic fields in this type of geometry, including derivation of the TE and TM modes supported, and examine the transverse force components exerted on the beam, which may be used for focusing or for deflection of the particles.

physics.acc-ph↗