arXiv subjects

Zhong Shi

Publications and source records attributed to Zhong Shi.

10 recordsLinked to original sources

arXiv2025

Ferromagnetic interface engineering of spin-charge conversion in RuO$_2$

Spin-orbit torque efficiency is conventionally fixed by bulk materials. $D$-wave altermagnets introduce an additional nonrelativistic spin-charge conversion channel beyond inverse spin-Hall effect. Using prototypical candidate RuO$_2$ as an example, we show that the adjacent ferromagnet alone can dictate both the magnitude and sign of spin-charge conversion. Spin-pumping measurements on RuO$_2$/Y$_3$Fe$_5$O$_{12}$ (YIG) and RuO$_2$/Ni$_{80}$Fe$_{20}$ (Py) bilayers yield opposite effective spin-Hall angles that persist across crystalline and polycrystalline RuO$_2$. Inserting an ultrathin Au spacer at the RuO$_2$/YIG interface reverses the signal, envidencing a dominant interfacial inverse Rashba-Edelstein effect, whereas RuO$_2$/Py is governed by bulk inverse spin-Hall effect. First-principles calculations trace this dichotomy to interface-selective band hybridization: Rashba surface states survive at the insulating YIG contact yet are quenched by metallic Py. Our findings establish ferromagnetic interfacing as a deterministic knob for tailoring spin-charge conversion in altermagnetic oxides, paving the way to field-free, low-dissipation spintronic memory devices.

cond-mat.mtrl-sci↗

arXiv2024

Unveiling the nonrelativistic spin current polarization in an altermagnet

Spin current plays a central role in spintronics for driving exotic spin-dependent phenomena and high-performance device applications. Recently, a magnetic spin Hall effect has been discovered in spin-split antiferromagnets including noncollinear antiferromagnets and altermagnets, allowing the efficient generation of unconventional spin currents even in the absence of spin-orbit coupling. However, although such nonrelativistic spin currents are proposed to have a magnetic origin, the direct connection between the Neel vector and the spin current polarization is still missing. Here, using the altermagnetic RuO2 as a representative example, we unveil the spin current polarization by disentangling the conventional and magnetic spin Hall effects using a technique we developed based on the spin Hall magnetoresistance measurement. The results suggest that the nonrelativistic spin current hosts a polarization very close to the Neel vector. Our work offers unambiguous evidence of the magnetic origin of the nonrelativistic spin current in altermagnetic RuO2, and paves a straightforward route to understand the unconventional spin currents that are crucial in spintronics.

cond-mat.mes-hall↗

arXiv2023

Strain-Tunable Magnetic Compensation Temperature of Epitaxial Tb$_3$Fe$_5$O$_{12}$ Thin Films

High-quality rare-earth iron garnet (ReIG) Tb$_3$Fe$_5$O$_{12}$ (TbIG) thin films are epitaxially grown on a series of (111)-oriented garnet substrates with various lattice constants. The coherent growth induces a substrate-dependent in-plane tensile or compressive strain in the TbIG film. Measurements of the anomalous Hall-like effect (AHLE) in TbIG/Pt heterostructures show that the compensation temperature of TbIG films monotonically changes with the film strain. The strain results in a variation of the distances between magnetic atoms in the TbIG crystal and therefore the corresponding exchange interactions. The latter is explicitly calculated as a function of the lattice strain based on density functional theory, reproducing the observed experimental results. This work provides a versatile way to optimize ReIG-based spin-orbit torque devices.

cond-mat.mtrl-sci↗

arXiv2022

Twisting the near-field radiative heat switch in hyperbolic antiferromagnets

We study the twisted control of the near-field radiative heat transfer between two hyperbolic antiferromagnetic insulators under external magnetic fields. We show that the near-field heat flux can be affected by both the twist angle $θ$ and the magnitude of the applied magnetic field with different broken symmetries. Irrespective of twist angle, the external magnetic field causes the radiative heat flux to change nonmonotonically, and the minimum heat flux can be found with the magnetic fields of about 1.5 T. Such nonmonotonic behavior is due to the fact that the magnetic field can radically change the nature of the magnon polaritons with time reversal symmetry breaking. The field not only affects the topological structure of surface magnon polaritons, but also induces the volume magnon polaritons that progressively dominate the heat transfer as the field increases. We further propose a twist-induced thermal switch device with inversion symmetry breaking, which can severely regulate radiative heat flux through different magnetic fields. Our findings account for a characteristic modulation of radiative heat transfer with implications for applications in dynamic thermal management.

cond-mat.mes-hall↗

arXiv2021

Role of Magnon-Magnon Scattering in Magnon Polaron Spin Seebeck Effect

The spin Seebeck effect (SSE) signal of magnon polarons in bulk-Y3Fe5O12 (YIG)/Pt heterostructures is found to drastically change as a function of temperature. It appears as a dip in the total SSE signal at low temperatures, but as the temperature increases, the dip gradually decreases before turning to a peak. We attribute the observed dip-to-peak transition to the rapid rise of the four-magnon scattering rate. Our analysis provides important insights into the microscopic origin of the hybridized excitations and the overall temperature dependence of the SSE anomalies.

cond-mat.mtrl-sci↗

arXiv2020

Thermal relaxation of magnons and phonons near resonance points in magnetic insulators

We theoretically investigate the energy relaxation rate of magnons and phonons near the resonance points to clarify the underlying mechanism of heat transport in ferromagnetic materials. We find that the simple two-temperature model is valid for the one-phonon/one-magnon process, as the rate of energy exchange between magnons and phonons is proportional to the temperature difference between them, and it is independent of temperature in the high temperature limit. We found that the magnon-phonon relaxation time due to the one-phonon/one-magnon interaction could be reduced to 1.48 $μs$ at the resonance point by applying an external magnetic field. It means that the resonance effect plays a significant role in enhancing the total magnon-phonon energy exchange rate, apart from the higher order interaction processes.

cond-mat.mes-hall↗

arXiv2019

Spin Seebeck effect from antiferromagnetic magnons and critical spin fluctuations in epitaxial FeF2 films

We report a longitudinal spin Seebeck effect (SSE) study in epitaxially grown FeF2(110) antiferromagnetic (AFM) thin films with strong uniaxial anisotropy over the temperature range of 3.8 - 250 K. Both the magnetic field- and temperature-dependent SSE signals below the Néel temperature (TN=70 K) of the FeF2 films are consistent with a theoretical model based on the excitations of AFM magnons without any net induced static magnetic moment. In addition to the characteristic low-temperature SSE peak associated with the AFM magnons, there is another SSE peak at TN which extends well into the paramagnetic phase. All the SSE data taken at different magnetic fields up to 12 T near and above the critical point TN follow the critical scaling law very well with the critical exponents for magnetic susceptibility of 3D Ising systems, which suggests that the AFM spin correlation is responsible for the observed SSE near TN.

cond-mat.mtrl-sci↗

arXiv2017

Direct observation of magnon-phonon coupling in yttrium iron garnet

The magnetic insulator yttrium iron garnet (YIG) with a ferrimagnetic transition temperature of $\sim$560 K has been widely used in microwave and spintronic devices. Anomalous features in the spin Seeback effect (SSE) voltages have been observed in Pt/YIG and attributed to the magnon-phonon coupling. Here we use inelastic neutron scattering to map out low-energy spin waves and acoustic phonons of YIG at 100 K as a function of increasing magnetic field. By comparing the zero and 9.1 T data, we find that instead of splitting and opening up gaps at the spin wave and acoustic phonon dispersion intersecting points, magnon-phonon coupling in YIG enhances the hybridized scattering intensity. These results are different from expectations of conventional spin-lattice coupling, calling for new paradigms to understand the scattering process of magnon-phonon interactions and the resulting magnon-polarons.

cond-mat.str-el↗

arXiv2017

Deficiency of the Bulk Spin Hall Effect Model for Spin-Orbit Torques in Magnetic Insulator/Heavy Metal Heterostructures

Electrical currents in a magnetic insulator/heavy metal heterostructure can induce two simultaneous effects, namely, spin Hall magnetoresistance (SMR) on the heavy metal side and spin-orbit torques (SOTs) on the magnetic insulator side. Within the framework of the pure spin current model based on the bulk spin Hall effect (SHE), the ratio of the spin Hall-induced anomalous Hall effect (SH-AHE) to SMR should be equal to the ratio of the field-like torque (FLT) to damping-like torque (DLT). We perform a quantitative study of SMR, SH-AHE, and SOTs in a series of thulium iron garnet/platinum or Tm3Fe5O12/Pt heterostructures with different Tm3Fe5O12 thicknesses, where Tm3Fe5O12 is a ferrimagnetic insulator with perpendicular magnetic anisotropy. We find the ratio between measured effective fields of FLT and DLT is at least 2 times larger than the ratio of the SH-AHE to SMR. In addition, the bulk SHE model grossly underestimates the spin torque efficiency of FLT. Our results reveal deficiencies of the bulk SHE model and also address the importance of interfacial effects such as the Rashba and magnetic proximity effects in magnetic insulator/heavy metal heterostructures.

cond-mat.mtrl-sci↗

arXiv2015

Nature of magnetotransport in metal/insulating-ferromagnet heterostructures: Spin Hall magnetoresistance or magnetic proximity effect

We study the anomalous Hall-like effect (AHLE) and the effective anisotropic magnetoresistance (EAMR) in antiferromagnetic γ -IrMn3/Y3Fe5O12(YIG) and Pt/YIG heterostructures. For γ -IrMn3/YIG, the EAMR and the AHLE resistivity change sign with temperature due to the competition between the spin Hall magnetoresistance (SMR) and the magnetic proximity effect (MPE) induced by the interfacial antiferromagnetic uncompensated magnetic moment. In contrast, for Pt/YIG the AHLE resistivity changes sign with temperature whereas no sign change is observed in the EAMR. This is because the MPE and the SMR play a dominant role in the AHLE and the EAMR, respectively. As new types of galvanomagnetic property, the AHLE and the EAMR have proved vital in disentangling the MPE and the SMR in metal/insulating-ferromagnet heterostructures.

cond-mat.mtrl-sci↗