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Zhongchen Xu

Publications and source records attributed to Zhongchen Xu.

7 recordsLinked to original sources

Fractional phase slips across the charge-density-wave domain walls in 1-T TiSe2

The microscopic origin of the charge density wave (CDW) in 1\textit{T}-TiSe$_2$ remains controversial, with competing scenarios based on phonon-driven lattice instability and electronically driven excitonic correlations. Here, we combine low-temperature scanning tunneling microscopy with two-dimensional lock-in phase analysis to directly resolve the local CDW phase in real space and track its evolution across individual domain walls. In homogeneous regions, the CDW phase remains uniform; by contrast, across domain walls we uncover a robust and reproducible $2\pi/3$ phase shift that occurs collectively in all three symmetry-related CDW components. This nontrivial and correlated phase-slip configuration places stringent constraints on the order-parameter manifold and challenges the simplest purely phonon-driven commensurate lock-in picture, which would instead predict a $\pi$ phase shift. A minimal free-energy model incorporating both electron-phonon and electron-hole interactions reproduces the observed phase behavior and indicates that electronic interactions play an important role in shaping the local phase structure of the CDW order. These results establish domain walls as direct real-space probes of the microscopic interactions underlying multicomponent order and provide a general phase-resolved framework for constraining competing ordering mechanisms in correlated materials.

cond-mat.str-el

Quantum fluctuations associated with first-order magnetic transition in a frustrated kagome lattice antiferromagnet

Intense quantum fluctuations arising from geometrical frustrations in kagome-lattice magnets provide a feasible approach to exotic quantum states. Here, we document an unexpected isosymmetric first-order magnetic transition in the recently synthesized frustrated kagome-lattice antiferromagnet Nd3ScBi5, which is characterized by significant latent heat and a pronounced magnetocaloric effect, as well as discontinuous Raman shifts and negligible hysteresis. Employing the magnetocaloric effect as a detection method, in conjunction with systematical field-dependent physical properties, we uncover a distinctive 1/2 magnetization plateau phase with significant quantum fluctuations. Our study unveils Nd3ScBi5 as a prototypical model with an emerging phase of enhanced quantum fluctuations triggered by first-order magnetic transitions.

cond-mat.str-el

Quasi-linear magnetoresistance and paramagnetic singularity in Hypervalent Bismuthide

Materials featuring hypervalent bismuth motifs have generated immense interest due to their extraordinary electronic structure and exotic quantum transport. In this study, we synthesized high-quality single crystals of La3ScBi5 characterized by one-dimensional hypervalent bismuth chains and performed a systematic investigation of the magnetoresistive behavior and quantum oscillations. The metallic La3ScBi5 exhibits a low-temperature plateau of electrical resistivity and quasi-linear positive magnetoresistance, with anisotropic magnetoresistive behaviors suggesting the presence of anisotropic Fermi surfaces. This distinctive transport phenomenon is perfectly elucidated by first-principles calculations utilizing the semiclassical Boltzmann transport theory. Furthermore, the nonlinear Hall resistivity pointed towards a multiband electronic structure, characterized by the coexistence of electron and hole carriers, which is further supported by our first-principles calculations. Angle-dependent de Haas-van Alphen oscillations are crucial for further elucidating its Fermiology and topological characteristics. Intriguingly, magnetization measurements unveiled a notable paramagnetic singularity at low fields, which might suggest the nontrivial nature of the surface states. Our findings underscore the interplay between transport phenomena and the unique electronic structure of hypervalent bismuthide La3ScBi5, opening avenues for exploring novel electronic applications.

cond-mat.mtrl-sci

Stability Frontiers and Mixed-dimensional physics in the Kagome Intermetallics Ln3ScBi5 (Ln = La-Nd, Sm)

Low-dimensional physics provides profound insights into strongly correlated interactions, leading to enhanced quantum effects and the emergence of exotic quantum states. The Ln3ScBi5 family stands out as a chemically versatile kagome platform with mixed low-dimensional structural framework and tunable physical properties. Our research initiates with a comprehensive evaluation of the currently known Ln3ScBi5 (Ln = La-Nd, Sm) materials, providing a robust methodology for assessing their stability frontiers within this system. Focusing on Pr3ScBi5, we investigate the influence of the zigzag chains of quasi-one-dimensional (Q1D) motifs and the distorted kagome layers of quasi-two-dimensional (Q2D) networks in the mixed-dimensional structure on the intricate magnetic ground states and unique spin fluctuations. Our study reveals that the noncollinear antiferromagnetic (AFM) moments of Pr3+ ions are confined within the Q2D kagome planes, displaying minimal in-plane anisotropy. In contrast, a strong AFM coupling is observed within the Q1D zigzag chains, significantly constraining spin motion. Notably, the magnetic frustration is partially the consequence of coupling to conduction electrons via the Ruderman-Kittel-Kasuya Yosida (RKKY) interaction, highlighting a promising framework for future investigations into mixed-dimensional frustration in Ln3ScBi5 systems.

cond-mat.str-el

Magnetization plateau and anisotropic magnetoresistance in the frustrated Kondo-lattice compound Ce3ScBi5

Kondo metals with geometric frustration offer fertile ground for exploring exotic states of matter with a field-induced fractional magnetization platform and nonsaturating magnetoresistance. Herein, a Ce3ScBi5 single crystal with anti-Hf5Sn3Cu hexagonal structure was successfully synthesized via the bismuth self-flux method, leading to the formation of cerium cations arranged in a frustrated structure within a distorted kagome lattice. Magnetic measurements exhibit two distinct antiferromagnetic transitions at 4.1 and 5.9 K. Specifically, the occurrence of multiple metamagnetic transitions between magnetization plateaus is evidenced upon applying magnetic fields perpendicular to the c axis. Transport measurements highlight remarkable Kondo-lattice characteristics and anisotropic magnetoresistance in Ce3ScBi5. The anomalous Hall contributions are observed at low temperatures under critical fields, suggesting Fermi surface reconstruction in a subset of the metamagnetic transitions. We have constructed a temperature-field phase diagram to provide comprehensive information on the complex magnetic structures arising from competitive interactions. Our work establishes Ce3ScBi5 and related materials as a unique platform for exploring low-dimensional quantum fluctuations in bulk crystals, and analyzes the critical role of geometric frustration in Kondo and Ruderman-Kittel-Kasuya-Yosida physical frameworks.

cond-mat.str-el

A non-invasive dry-transfer method for fabricating mesoscopic devices on sensitive materials

Many materials with novel or exotic properties are highly sensitive to environmental factors such as air, solvents, and heat, which complicates device fabrication and limits their potential applications. Here, we present a universal submicron fabrication method for mesoscopic devices using a dry-transfer technique, tailored specifically for sensitive materials. This approach utilizes PMMA masks, combined with a water-dissoluble coating as a sacrificial layer, to ensure that sensitive materials are processed without exposure to harmful environmental conditions. The entire fabrication process is carried out in a glove box, employing dry techniques that avoid air, solvents, and heat exposure, culminating in an encapsulation step. We demonstrate the utility of this method by fabricating and characterizing K2Cr3As3 and WTe2 devices, a one- and two-dimensional material, respectively. The results show that our technique preserves the integrity of the materials, provides excellent contact interfaces, and is broadly applicable to a range of sensitive materials.

cond-mat.mes-hall

Evidence of P-wave Pairing in K$_2$Cr$_3$As$_3$ Superconductors from Phase-sensitive Measurement

P-wave superconductors hold immense promise for both fundamental physics and practical applications due to their unusual pairing symmetry and potential topological superconductivity. However, the exploration of the p-wave superconductors has proved to be a complex endeavor. Not only are they rare in nature but also the identification of p-wave superconductors has been an arduous task in history. For example, phase-sensitive measurement, an experimental technique which can provide conclusive evidence for unconventional pairing, has not been implemented successfully to identify p-wave superconductors. Here, we study a recently discovered family of superconductors, A$_2$Cr$_3$As$_3$ (A = K, Rb, Cs), which were proposed theoretically to be a candidate of p-wave superconductors. We fabricate superconducting quantum interference devices (SQUIDs) on exfoliated K$_2$Cr$_3$As$_3$, and perform the phase-sensitive measurement. We observe that such SQUIDs exhibit a pronounced second-order harmonic component sin(2$π$) in the current-phase relation, suggesting the admixture of 0- and $π$-phase. By carefully examining the magnetic field dependence of the oscillation patterns of critical current and Shapiro steps under microwave irradiation, we reveal a crossover from 0- to $π$-dominating phase state and conclude that the existence of the $π$-phase is in favor of the p-wave pairing symmetry in K$_2$Cr$_3$As$_3$.

cond-mat.supr-con