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Zhouyi Yin

Publications and source records attributed to Zhouyi Yin.

5 recordsLinked to original sources

Discovery of a symmetry-driven electronic cascade in a $d$-wave altermagnet

Altermagnets host magnetic compensation together with non-relativistic spin-split bands, a coexistence enabled by crystal symmetry. Yet whether and how crystal symmetry organizes collective electronic order remains largely unexplored. Here we uncover a symmetry-driven cascade of finite-$q$ charge order in a $d$-wave altermagnet Rb$_{1-{\delta}}$V$_2$Te$_2$O, using phase-resolved scanning tunneling microscopy. A primary density-wave instability drives an initial electronic reconstruction, followed by the emergence of a nematic component and an off-axis modulation with wave vectors geometrically tied to the preceding orders. Phase-resolved spectroscopy distinguishes these components through separate contrast-inversion energies and maps out branch-selective spectral-weight redistribution within the off-axis mode. Together with doping and temperature evolution, these observations establish a highly coordinated hierarchy of coupled density-wave instabilities, consistent with successive symmetry lowering. This multi-component hierarchy can be well described in the Landau framework through sequential softening of the charge orders, where bilinear coupling to their compatible octupolar partners at the lower-symmetry stages enables mutual stabilization within an intertwined charge-multipole state. Such a transparent realization of a charge-order cascade shows how altermagnetic symmetry can extend beyond band formation to organize collective electronic order, offering a new perspective on emergent many-body states in correlated quantum materials.

cond-mat.mes-hall

Odd spin symmetry and anisotropy switching in p-wave magnet CeNiAsO

Odd-parity magnets, complementary to altermagnets, exhibit unique properties such as high efficiency in charge-spin conversion and compatibility with conventional superconductivity, of critical importance in the pursuit of energy-efficient spintronics and topological superconductors for quantum computation. For even-parity d-wave and g-wave altermagnets, the magnetic structure, spin-split band structure and physical properties are currently under intensive study. On the contrary, while hundreds of odd-parity magnets and the promising properties have been predicted in theory, experimental studies are scarce. Specifically, the magnetic structure and transport properties of candidates NiI2 and Ga3Ru4Al12 have been reported, yet the characteristic band structure and particularly the odd-parity spin symmetry remain elusive. Here we demonstrate experimentally the deterministic p-wave spin symmetry and resistance anisotropy switching for the prototype odd-parity magnet, CeNiAsO. Angle-resolved photoemission spectroscopy (ARPES) reveals two cleaved terminations with distinct surface band structure. By compensating the polar surface, we achieve intrinsic bulk band structure, for which the spin splitting can be well described by the p-wave magnetic structure through first-principles calculation. The bulk spin polarization measured by spin-resolved ARPES exhibits symmetry with only one degenerate plane, fingerprint of p-wave magnetism. We further demonstrate giant resistance anisotropy and switching between high-resistance and low-resistance states through modest field-induced domain selection, highlighting its potential for antiferromagnetic spin memory devices. The structural similarity between CeNiAsO and 1111-type Fe-based superconductors stimulates further exploration on the interplay between p-wave magnetism, superconductivity and band topology.

cond-mat.str-el

Crystal-symmetry-paired spin-valley locking in a layered room-temperature antiferromagnet

Recent theoretical efforts predicted a type of unconventional antiferromagnet characterized by the crystal symmetry C (rotation or mirror), which connects antiferromagnetic sublattices in real space and simultaneously couples spin and momentum in reciprocal space. This results in a unique C-paired spin-valley locking (SVL) and corresponding novel properties such as piezomagnetism and noncollinear spin current even without spin-orbit coupling. However, the unconventional antiferromagnets reported thus far are not layered materials, limiting their potential in spintronic applications. Additionally, they do not meet the necessary symmetry requirements for nonrelativistic spin current. Here, we report the realization of C-paired SVL in a layered room-temperature antiferromagnetic compound, Rb1-{\delta}V2Te2O. Spin resolved photoemission measurements directly demonstrate the opposite spin splitting between C-paired valleys. Quasi-particle interference patterns reveal the suppression of inter-valley scattering due to the spin selection rules, as a direct consequence of C-paired SVL. All these experiments are well consistent with the results obtained from first-principles calculations. Our observations represent the first realization of layered antiferromagnets with C-paired SVL, enabling both the advantages of layered materials and possible control through crystal symmetry manipulation. These results hold significant promise and broad implications for advancements in magnetism, electronics, and information technology.

cond-mat.str-el

Phonon promoted charge density wave in topological kagome metal ScV$_{6}$Sn$_{6}$

Charge density wave (CDW) orders in vanadium-based kagome metals have recently received tremendous attention due to their unique properties and intricate interplay with exotic correlated phenomena, topological and symmetry-breaking states. However, the origin of the CDW order remains a topic of debate. The discovery of ScV$_{6}$Sn$_{6}$, a vanadium-based bilayer kagome metal exhibiting an in-plane $\sqrt{3}$ x $\sqrt{3} $ $\textit{R}$30$°$ CDW order with time-reversal symmetry breaking, provides a novel platform to explore the underlying mechanism behind the unconventional CDW. Here, we combine high-resolution angle-resolved photoemission spectroscopy, Raman scattering measurements and density functional theory to investigate the electronic structures and phonon modes of ScV$_{6}$Sn$_{6}$ and their evolution with temperature. We identify topologically nontrivial Dirac surface states and multiple van Hove singularities (VHSs) in the vicinity of the Fermi level, with one VHS near the K point exhibiting nesting wave vectors in proximity to the $\sqrt{3}$ x $\sqrt{3}$ $\textit{R}$30$°$ CDW wave vector. Additionally, Raman measurements indicate a strong intrinsic electron-phonon coupling in ScV$_{6}$Sn$_{6}$, as evidenced by the presence of a two-phonon mode and a large frequency amplitude mode. Our findings highlight the fundamental role of lattice degrees of freedom in promoting the CDW in ScV$_{6}$Sn$_{6}$ and provide important insights into the fascinating correlation phenomena observed in kagome metals.

cond-mat.str-el

Spectroscopic signature of obstructed surface states in SrIn$_2$P$_2$

The century-long development of surface sciences has witnessed the discoveries of a variety of quantum states. In the recently proposed "obstructed atomic insulators", insulators with symmetric charges pinned at virtual sites where no real atoms reside, the cleavage through these sites could lead to a set of obstructed surface states with partial occupation. Here, utilizing scanning tunneling microscopy, angle-resolved photoemission spectroscopy and first-principles calculations, we observe spectroscopic signature of obstructed surface states in SrIn$_2$P$_2$. We find a pair of surface states originated from the pristine obstructed surface states split by a unique surface reconstruction. The upper branch is marked with a striking differential conductance peak followed by negative differential conductance, signaling its localized nature, while the lower branch is found to be highly dispersive. This pair of surface states is in consistency with our calculational results. Our finding not only demonstrates a surface quantum state induced by a new type of bulk-boundary correspondence, but also provides a platform for exploring efficient catalysts and related surface engineering.

cond-mat.mtrl-sci