arXiv subjects

Zi Yang Meng

Publications and source records attributed to Zi Yang Meng.

At least 163 records · Page 9Linked to original sources

arXiv2019

Antiferromagnetism in kagome $α$-Cu$_{3}$Mg(OH)$_6$Br$_2$

The antiferromagnetism in $α$-Cu$_3$Mg(OH)$_6$Br$_2$ was studied by magnetic-susceptibility, specific-heat and neutron-diffraction measurements. The crystal structure consists of Cu$^{2+}$ kagome layers with Mg$^{2+}$ ions occupying the centers of the hexagons, separated by Br$^{1-}$ ions. The magnetic system orders antiferromagnetically at 5.4 K with the magnetic moments aligned ferromagnetically within the kagome planes. The ordered moment is 0.94 $μ_B$, suggesting little quantum and geometrical fluctuations. By comparing the magnetic and specific-heat properties with those of the haydeeite, we suggest that $α$-Cu$_3$Mg(OH)$_6$Br$_2$ may be described by the two-dimensional spin-$1/2$ Heisenberg kagome model and is in the region of the ferromagnetic-order side of the phase diagram.

cond-mat.str-el↗

arXiv2019

Emergent Symmetry and Conserved Current at a One Dimensional Incarnation of Deconfined Quantum Critical Point

The deconfined quantum critical point (DQCP) was originally proposed as a continuous transition between two spontaneous symmetry breaking phases in 2D spin-1/2 systems. While great efforts have been spent on the DQCP for 2D systems, both theoretically and numerically, ambiguities among the nature of the transition are still not completely clarified. Here we shift the focus to a recently proposed 1D incarnation of DQCP in a spin-1/2 chain. By solving it with the variational matrix product state in the thermodynamic limit, a continuous transition between a valence-bond solid phase and a ferromagnetic phase is discovered. The scaling dimensions of various operators are calculated and compared with those from field theoretical description. At the critical point, two emergent O(2) symmetries are revealed, and the associated conserved current operators with exact integer scaling dimensions are determined with scrutiny. Our findings provide the low-dimensional analog of DQCP where unbiased numerical results are in perfect agreement with the controlled field theoretical predictions and have extended the realm of the unconventional phase transition as well as its identification with the advanced numerical methodology.

cond-mat.str-el↗

arXiv2019

Charge-Density-Wave Transitions of Dirac Fermions Coupled to Phonons

The spontaneous generation of charge-density-wave order in a Dirac fermion system via the natural mechanism of electron-phonon coupling is studied in the framework of the Holstein model on the honeycomb lattice. Using two independent and unbiased quantum Monte Carlo methods, the phase diagram as a function of temperature and coupling strength is determined. It features a quantum critical point as well as a line of thermal critical points. Finite-size scaling appears consistent with fermionic Gross-Neveu-Ising universality for the quantum phase transition, and bosonic Ising universality for the thermal phase transition. The critical temperature has a maximum at intermediate couplings. Our findings motivate experimental efforts to identify or engineer Dirac systems with sufficiently strong and tunable electron-phonon coupling.

cond-mat.str-el↗

arXiv2018

From Claringbullite to a new spin liquid candidate Cu$_3$Zn(OH)$_6$FCl

The search for quantum spin liquid (QSL) materials has attracted significant attention in the field of condensed matter physics in recent years, but until now only a handful of them are considered as candidates hosting QSL ground state. Owning to their geometrically frustrated structure, Kagome materials are ideal system to realize QSL. In this study, we synthesized the kagome structured material Claringbullite (Cu$_4$(OH)$_6$FCl) and then performed Zn doping to form Cu$_3$Zn(OH)$_6$FCl. Comprehensive measurements reveal that doping Zn$^{2+}$ ions transforms magnetically ordered Cu$_4$(OH)$_6$FCl into a non-magnetic QSL candidate Cu$_3$Zn(OH)$_6$FCl. Therefore, the successful syntheses of Cu$_4$(OH)$_6$FCl and Cu$_3$Zn(OH)$_6$FCl not only provide a new platform for the study of QSL but also a novel pathway of investigating the transition between QSL and magnetically ordered systems.

cond-mat.str-el↗

arXiv2018

EMUS-QMC: Elective Momentum Ultra-Size Quantum Monte Carlo Method

One bottleneck of quantum Monte Carlo (QMC) simulation of strongly correlated electron systems lies at the scaling relation of computational complexity with respect to the system sizes. For generic lattice models of interacting fermions, the best methodology at hand still scales with $βN^3$ where $β$ is the inverse temperature and $N$ is the system size. Such scaling behavior has greatly hampered the accessibility of the universal infrared (IR) physics of many interesting correlated electron models at (2+1)D, let alone (3+1)D. To reduce the computational complexity, we develop a new QMC method with inhomogeneous momentum-space mesh, dubbed elective momentum ultra-size quantum Monte Carlo (EQMC) method. Instead of treating all fermionic excitations on an equal footing as in conventional QMC methods, by converting the fermion determinant into the momentum space, our method focuses on fermion modes that are directly associated with low-energy (IR) physics in the vicinity of the so-called hot-spots, while other fermion modes irrelevant for universal properties are ignored. As shown in the manuscript, for any cutoff-independent quantities, e.g. scaling exponents, this method can achieve the same level of accuracy with orders of magnitude increase in computational efficiency. We demonstrate this method with a model of antiferromagnetic itinerant quantum critical point, realized via coupling itinerant fermions with a frustrated transverse-field Ising model on a triangle lattice. The system size of $48 \times 48 \times 32$ ($L\times L\timesβ$, almost 3 times of previous investigations) are comfortably accessed with EQMC. With much larger system sizes, the scaling exponents are unveiled with unprecedentedly high accuracy, and this result sheds new light on the open debate about the nature and the universality class of itinerant quantum critical points.

cond-mat.str-el↗

arXiv2018

Dynamical Signature of Fractionalization at the Deconfined Quantum Critical Point

Deconfined quantum critical points govern continuous quantum phase transitions at which fractionalized (deconfined) degrees of freedom emerge. Here we study dynamical signatures of the fractionalized excitations in a quantum magnet (the easy-plane J-Q model) that realize a deconfined quantum critical point with emergent O(4) symmetry. By means of large-scale quantum Monte Carlo simulations and stochastic analytic continuation of imaginary-time correlation functions, we obtain the dynamic spin structure factors in the $S^{x}$ and $S^{z}$ channels. In both channels, we observe broad continua that originate from the deconfined excitations. We further identify several distinct spectral features of the deconfined quantum critical point, including the lower edge of the continuum and its form factor on moving through the Brillouin Zone. We provide field-theoretical and lattice model calculations that explain the overall shapes of the computed spectra, which highlight the importance of interactions and gauge fluctuations to explaining the spectral-weight distribution. We make further comparisons with the conventional Landau O(2) transition in a different quantum magnet, at which no signatures of fractionalization are observed. The distinctive spectral signatures of the deconfined quantum critical point suggest the feasibility of its experimental detection in neutron scattering and nuclear magnetic resonance experiments.

cond-mat.str-el↗

arXiv2018

Bosonic SET to SPT Transition under Dyonic LSM Theorem

Employing large-scale quantum Monte Carlo simulatoins, we study the phase diagram of a quantum spin model which is subject to the recently developed dyonic Lieb-Shultz-Mattis (LSM) theorem. The theorem predicts there are symmetry enriched/protected topological (SET/SPT) phases in the phase diagram. Our numerical results reveal a first order quantum phase transition between SET and SPT phases, consistent with an anyon condensation mechanism that enforces SPT phase according to the theorem. Also there exists in the phase diagram a symmetry-breaking phase in the form of superfluid (SF). The transition between SET and SF is continuous and that between SPT and SF is first order. Interestingly, the SET, SPT and SF phases meet at a critical endpoint, whose presence can be universally explained via theory contains emergent gauge field coupled to vortex fields, and consequently reveals the exotic feature of our model even beyond the realm of dyonic LSM.

cond-mat.str-el↗

arXiv2018

Effect of Zn doping on the antiferromagnetism in kagome Cu$_{4-x}$Zn$_x$(OH)$_6$FBr

Barlowite Cu$_4$(OH)$_6$FBr shows three-dimensional (3D) long-range antiferromagnetism, which is fully suppressed in Cu$_3$Zn(OH)$_6$FBr with a kagome quantum spin liquid ground state. Here we report systematic studies on the evolution of magnetism in the Cu$_{4-x}$Zn$_x$(OH)$_{6}$FBr system as a function of $x$ to bridge the two limits of Cu$_4$(OH)$_6$FBr ($x$=0) and Cu$_3$Zn(OH)$_6$FBr ($x$=1). Neutron-diffraction measurements reveal a hexagonal-to-orthorhombic structural change with decreasing temperature in the $x$ = 0 sample. While confirming the 3D antiferromagnetic nature of low-temperature magnetism, the magnetic moments on some Cu$^{2+}$ sites on the kagome planes are found to be vanishingly small, suggesting strong frustration already exists in barlowite. Substitution of interlayer Cu$^{2+}$ with Zn$^{2+}$ with gradually increasing $x$ completely suppresses the bulk magnetic order at around $x$ = 0.4, but leaves a local secondary magnetic order up to $x\sim 0.8$ with a slight decrease in its transition temperature. The high-temperature magnetic susceptibility and specific heat measurements further suggest that the intrinsic magnetic properties of kagome spin liquid planes may already appear from $x>0.3$ samples. Our results reveal that the Cu$_{4-x}$Zn$_x$(OH)$_6$FBr may be the long-thought experimental playground for the systematic investigations of the quantum phase transition from a long-range antiferromagnet to a topologically ordered quantum spin liquid.

cond-mat.str-el↗

arXiv2018

Quantum Spin Liquid with Even Ising Gauge Field Structure on Kagome Lattice

Employing large-scale quantum Monte Carlo simulations, we study the extended $XXZ$ model on the kagome lattice. A $\mathbb Z_2$ quantum spin liquid phase with effective even Ising gauge field structure emerges from the delicate balance among three symmetry-breaking phases including stripe solid, staggered solid and ferromagnet. This $\mathbb{Z}_2$ spin liquid is stabilized by an extended interaction related to the Rokhsar-Kivelson potential in the quantum dimer model limit. The phase transitions from the staggered solid to a spin liquid or ferromagnet are found to be first order and so is the transition between the stripe solid and ferromagnet. However, the transition between a spin liquid and ferromagnet is found to be continuous and belongs to the 3D $XY^*$ universality class associated with the condensation of spinons. The transition between a spin liquid and stripe solid appears to be continuous and associated with the condensation of visons.

cond-mat.str-el↗

arXiv2018

Dynamical Signature of Symmetry Fractionalization in Frustrated Magnets

The nontrivialness of quantum spin liquid (QSL) typically manifests in the non-local observables that signifies their existence, however, this fact actually casts shadow on detecting QSL with experimentally accessible probes. Here, we provide a solution by unbiasedly demonstrating dynamical signature of anyonic excitations and symmetry fractionalization in QSL. Employing large-scale quantum Monte Carlo simulation and stochastic analytic continuation, we investigate the extended XXZ model on the kagome lattice, and find out that across the phase transitions from Z2 QSLs to different symmetry breaking phases, spin spectral functions can reveal the presence and condensation of emergent anyonic spinon and vison excitations, in particular the translational symmetry fractionalization of the latter, which can be served as the unique dynamical signature of the seemingly ephemeral QSLs in spectroscopic techniques such as inelastic neutron or resonance (inelastic) X-ray scatterings.

cond-mat.str-el↗

arXiv2018

Itinerant quantum critical point with frustration and non-Fermi-liquid

Employing the self-learning quantum Monte Carlo algorithm, we investigate the frustrated transverse-field triangle-lattice Ising model coupled to a Fermi surface. Without fermions, the spin degrees of freedom undergoes a second-order quantum phase transition between paramagnetic and clock-ordered phases. This quantum critical point (QCP) has an emergent U(1) symmetry and thus belongs to the (2+1)D XY universality class. In the presence of fermions, spin fluctuations introduce effective interactions among fermions and distort the bare Fermi surface towards an interacting one with hot spots and Fermi pockets. Near the QCP, non-Fermi-liquid behavior are observed at the hot spots, and the QCP is rendered into a different universality with Hertz-Millis type exponents. The detailed properties of this QCP and possibly related experimental systems are also discussed.

cond-mat.str-el↗

arXiv2018

Symmetry Enforced Self-Learning Monte Carlo Method Applied to the Holstein Model

Self-learning Monte Carlo method (SLMC), using a trained effective model to guide Monte Carlo sampling processes, is a powerful general-purpose numerical method recently introduced to speed up simulations in (quantum) many-body systems. In this work, we further improve the efficiency of SLMC by enforcing physical symmetries on the effective model. We demonstrate its effectiveness in the Holstein Hamiltonian, one of the most fundamental many-body descriptions of electron-phonon coupling. Simulations of the Holstein model are notoriously difficult due to the combination of the typical cubic scaling of fermionic Monte Carlo and the presence of extremely long autocorrelation times. Our method addresses both bottlenecks. This enables simulations on large lattices in the most difficult parameter regions, and evaluation of the critical point for the charge density wave transition at half-filling with high precision. We argue that our work opens a new research area of quantum Monte Carlo (QMC), providing a general procedure to deal with ergodicity in situations involving Hamiltonians with multiple, distinct low energy states.

cond-mat.str-el↗

arXiv2018

Dynamics of Topological Excitations in a Model Quantum Spin Ice

We study the quantum spin dynamics of a frustrated XXZ model on a pyrochlore lattice by using large-scale quantum Monte Carlo simulation and stochastic analytic continuation. In the low-temperature quantum spin ice regime, we observe signatures of coherent photon and spinon excitations in the dynamic spin structure factor. As the temperature rises to the classical spin ice regime, the photon disappears from the dynamic spin structure factor, whereas the dynamics of the spinon remain coherent in a broad temperature window. Our results provide experimentally relevant, quantitative information for the ongoing pursuit of quantum spin ice materials.

cond-mat.str-el↗

arXiv2017

Nearly deconfined spinon excitations in the square-lattice spin-1/2 Heisenberg antiferromagnet

We study the dynamic spin structure factor of the spin-$1/2$ square-lattice Heisenberg antiferromagnet and of the $J$-$Q$ model (with 4-spin interactions $Q$ and Heisenberg exchange $J$). Using an improved method for stochastic analytic continuation of imaginary-time correlation functions computed with QMC simulations, we can treat the sharp ($δ$-function) contribution from spinwaves (magnons) and a continuum at higher energy. The results for the Heisenberg model agree with neutron scattering experiments on Cu(DCOO)$_2$$\cdot$4D$_2$O, where a broad spectral-weight continuum at $q=(π,0)$ was interpreted as deconfined spinons. Our results at $(π,0)$ show a similar reduction of the magnon weight and a large continuum, while the continuum is much smaller at $q=(π/2,π/2)$ (as also seen experimentally). Turning on $Q$, we observe a rapid reduction of the $(π,0)$ magnon weight to zero, well before the deconfined quantum phase transition into a spontaneously dimerized state. We re-interpret the picture of deconfined spinons at $(π,0)$ in the experiments as nearly deconfined spinons---a precursor to deconfined quantum criticality. To further elucidate the picture of a fragile $(π,0)$-magnon in the Heisenberg model and its depletion in the $J$-$Q$ model, we introduce an effective model in which a magnon can split into two spinons that do not separate but fluctuate in and out of the magnon space (in analogy with the resonance between a photon and a particle-hole pair in the exciton-polariton problem). The model reproduces the $(π,0)$ and $(π/2,π/2)$ features of the Heisenberg model. It can also account for the rapid loss of the $(π,0)$ magnon with increasing $Q$ and a remarkable persistence of a large magnon pole at $q=(π/2,π/2)$ even at the deconfined critical point.

cond-mat.str-el↗

arXiv2017

Unified phase diagram for iron-based superconductors

High-temperature superconductivity is closely adjacent to a long-range antiferromagnet, which is called a parent compound. In cuprates, all parent compounds are alike and carrier doping leads to superconductivity, so a unified phase diagram can be drawn. However, the properties of parent compounds for iron-based superconductors show significant diversity and both carrier and isovalent dopings can cause superconductivity, which casts doubt on the idea that there exists a unified phase diagram for them. Here we show that the ordered moments in a variety of iron pnictides are inversely proportional to the effective Curie constants of their nematic susceptibility. This unexpected scaling behavior suggests that the magnetic ground states of iron pnictides can be achieved by tuning the strength of nematic fluctuations. Therefore, a unified phase diagram can be established where superconductivity emerges from a hypothetical parent compound with a large ordered moment but weak nematic fluctuations, which suggests that iron-based superconductors are strongly correlated electron systems.

cond-mat.supr-con↗

arXiv2017

Unifying static and dynamic properties in 3D quantum antiferromagnets

Quantum Monte Carlo simulations offer an unbiased means to study the static and dynamic properties of quantum critical systems, while quantum field theory provides direct analytical results. We study three dimensional, critical quantum antiferromagnets by performing a combined analysis using both quantum field theory calculations and quantum Monte Carlo data. Explicitly, we analyze the order parameter (staggered magnetization), Néel temperature, quasiparticle gaps, and the susceptibilities in the scalar and vector channels. We connect the two approaches by deriving descriptions of the quantum Monte Carlo observables in terms of the quasiparticle excitations of the field theory. The remarkable agreement not only unifies the description of the static and dynamic properties of the system, but also constitutes a thorough test of perturbative O(3) quantum field theory and opens new avenues for the analytical guidance of detailed numerical studies.

cond-mat.str-el↗

arXiv2017

Topological Spin Liquid with Symmetry-Protected Edge States

Topological spin liquids are robust quantum states of matter with long-range entanglement and possess many exotic properties such as the fractional statistics of the elementary excitations. Yet these states, short of local parameters like all topological states, are elusive for conventional experimental probes. In this work, we combine theoretical analysis and quantum Monte Carlo numerics on a frustrated spin model which hosts a $\mathbb Z_2$ topological spin liquid ground state, and demonstrate that the presence of symmetry-protected gapless edge modes is a characteristic feature of the state, originating from the nontrivial symmetry fractionalization of the elementary excitations. Experimental observation of these modes on the edge would directly indicate the existence of the topological spin liquids in the bulk, analogous to the fact that the observation of Dirac edge states confirmed the existence of topological insulators.

cond-mat.str-el↗

arXiv2017

Non-Fermi-liquid at (2+1)d ferromagnetic quantum critical point

We construct a two-dimensional lattice model of fermions coupled to Ising ferromagnetic critical fluctuations. Using extensive sign-problem-free quantum Monte Carlo simulations, we show that the model realizes a continuous itinerant quantum phase transition. In comparison with other similar itinerant quantum critical points (QCPs), our QCP shows much weaker superconductivity tendency with no superconducting state down to the lowest temperature investigated, hence making the system a good platform for the exploration of quantum critical fluctuations. Remarkably, clear signatures of non-Fermi-liquid behavior in the fermion propagators are observed at the QCP. The critical fluctuations at the QCP partially resemble Hertz-Millis-Moriya behavior. However, careful scaling analysis reveals that the QCP belongs to a different universality class, deviating from both (2+1)d Ising and Hertz-Millis-Moriya predictions.

cond-mat.str-el↗