arXiv subjects

Zilong Wu

Publications and source records attributed to Zilong Wu.

4 recordsLinked to original sources

arXiv2025

Electrically tunable quantum interference of atomic spins on surfaces

Controlling quantum interference near avoided energy-level crossings is crucial for fast and reliable coherent manipulation in quantum information processing. However, achieving tunable quantum interference in atomically-precise engineered structures remains challenging. Here, we demonstrate electrical control of quantum interference using atomic spins on an insulating film in a scanning tunneling microscope. Using bias voltages applied across the tunnel junction, we modulate the atomically-confined magnetic interaction between the probe tip and surface atoms with a strong electric field, and drive the spin state rapidly through the energy-level anticrossing. This all-electrical manipulation allows us to achieve Landau-Zener-Stückelberg-Majorana (LZSM) interferometry on both single spins and pairs of interacting spins. The LZSM pattern exhibits multiphoton resonances, and its asymmetry suggests that the spin dynamics is influenced by spin-transfer torque of tunneling electrons. Multi-level LZSM spectra measured on coupled spins with tunable interactions show distinct interference patterns depending on their many-body energy landscapes. These results open new avenues for all-electrical quantum manipulation in spin-based quantum processors in the strongly driven regime.

cond-mat.mes-hall↗

arXiv2024

Enhancing Cross-lingual Sentence Embedding for Low-resource Languages with Word Alignment

The field of cross-lingual sentence embeddings has recently experienced significant advancements, but research concerning low-resource languages has lagged due to the scarcity of parallel corpora. This paper shows that cross-lingual word representation in low-resource languages is notably under-aligned with that in high-resource languages in current models. To address this, we introduce a novel framework that explicitly aligns words between English and eight low-resource languages, utilizing off-the-shelf word alignment models. This framework incorporates three primary training objectives: aligned word prediction and word translation ranking, along with the widely used translation ranking. We evaluate our approach through experiments on the bitext retrieval task, which demonstrate substantial improvements on sentence embeddings in low-resource languages. In addition, the competitive performance of the proposed model across a broader range of tasks in high-resource languages underscores its practicality.

cs.CL↗

arXiv2023

Light-driven C-H bond activation mediated by 2D transition metal dichalcogenides

C-H bond activation enables the facile synthesis of new chemicals. While C-H activation in short-chain alkanes has been widely investigated, it remains largely unexplored for long-chain organic molecules. Here, we report light-driven C-H activation in complex organic materials mediated by 2D transition metal dichalcogenides (TMDCs) and the resultant solid-state synthesis of luminescent carbon dots in a spatially-resolved fashion. We unravel the efficient H adsorption and a lowered energy barrier of C-C coupling mediated by 2D TMDCs to promote C-H activation. Our results shed light on 2D materials for C-H activation in organic compounds for applications in organic chemistry, environmental remediation, and photonic materials.

cond-mat.mtrl-sci↗

arXiv2019

Dark-Exciton-Mediated Fano Resonance from a Single Gold Nanostructure Deposited on Monolayer WS2 at Room Temperature

Strong spatial confinement and highly reduced dielectric screening provide monolayer transition metal dichalcogenides (TMDCs) with strong many-body effects, thereby possessing optically forbidden excitonic states (i.e., dark excitons) at room temperature. Herein, we explore the interaction of surface plasmons with dark excitons in hybrid systems consisting of stacked gold nanotriangles (AuNTs) and monolayer WS2. We observe a narrow Fano resonance when the hybrid system is surrounded by water, and we attribute the narrowing of the spectral Fano linewidth to the plasmon-enhanced decay of dark K-K excitons. Our results reveal that dark excitons in monolayer WS2 can strongly modify Fano resonances in hybrid plasmon-exciton systems and can be harnessed for novel optical sensors and active nanophotonic devices.

physics.optics↗