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Zoe Z. Yan

Publications and source records attributed to Zoe Z. Yan.

14 recordsLinked to original sources

Quantum science with arrays of metastable helium-3 atoms

The motion of atoms in programmable optical tweezer arrays offers many new opportunities for neutral atom quantum science. These include inter- and intra-site atom motion for resource-efficient implementations of fermionic and bosonic modes, respectively, as well as tweezer transport for efficient compilation of arbitrary circuits. However, the exploitation of atomic motion for all three purposes and others is limited by the inertia of the atoms. We present a comprehensive architectural blueprint for the use of fermionic metastable helium-3 ($^3$He$^*$) atoms -- the lightest trappable atomic species -- in programmable optical tweezer arrays. This includes a concrete analysis of atomic structure considerations as well as Rydberg-mediated interactions. We show that inter-tweezer hopping of $^3$He$^*$ atoms can be $\gtrsim3\times$ faster than previous demonstrations with lithium-6. We also demonstrate a new toolbox for encoding and manipulating qubits directly in the tweezer trap potential, uniquely enabled by the light mass of $^3$He$^*$. Finally, we provide several examples of new opportunities for fermionic quantum simulation and computation that leverage the transport and inter-tweezer hopping of $^3$He$^*$ atom arrays. These tools present new methods to improve the resource efficiency of neutral atom quantum science that may also enable quantum simulations of lattice gauge theories and quantum chemistry outside the Born-Oppenheimer approximation

quant-ph

Exact quantum scars from kinetic frustration for cross-platform realizations

Quantum many-body scars are nonthermal states exhibiting persistent revivals in an otherwise ergodic, nonintegrable quantum system. Here we leverage the phenomenon of kinetic frustration -- the destructive interference of multiple quantum paths -- to create exact scars. The simplicity makes these models directly suitable for implementation on multiple existing quantum simulation platforms. In particular, we show how frustrated hardcore bosons in cold atom Bose-Hubbard simulators and polar molecule or Rydberg atom tweezer arrays have persistent oscillations whose lifetimes can be tuned with experimentally accessible parameters, like the Hubbard interaction or a Floquet drive. Second, we propose an experimentally realizable scar within a non-integrable Fermi-Hubbard model where the frustration arises from the fermionic exchange statistics, which admits a one-to-one mapping with the bosonic model in the scar subspace. Finally, we introduce a practical heuristic based on the energy distribution of eigenstates for systematically predicting and optimizing quantum many-body scar lifetimes. Their cross-platform realizability and long lifetimes make them well-suited for benchmarking coherence and exploring nonergodic dynamics in current and near-term quantum devices.

quant-ph

A magneto-optical trap of silver and potassium atoms

We demonstrate a dual magneto-optical trap of $^{109}$Ag and $^{39}$K. For silver, a decreasing-field Zeeman slower loads a MOT of $1.5{\times}10^8$ atoms at a temperature of 0.74(5) mK, with laser cooling occurring primarily on the $D_2$ line of $4d^{10}5s\; {}^2S_{1/2}\rightarrow 5p\; {}^2P_{3/2}$ at 328 nm. We create a novel Ag "dark spot MOT," where shelving the atoms in a dark state enhances the captured atom number by a factor of two and the lifetime by a factor of four. For potassium, we obtain $2{\times}10^8$ trapped atoms, and further cooling on the $D_1$ transition via grey molasses results in a cloud of $1.2{\times} 10^8$ atoms at 7(1) $μ$K. We observe evidence of photoionization loss of the K MOT in the presence of Ag laser-cooling light, with implications for optimal dual species loading strategies. Our results on Ag point to simple and general laser cooling strategies for other coinage metals (Au, Cu). Furthermore, this work lays the foundation for the production of alkali-coinage metal degenerate quantum mixtures and highly polar molecules.

physics.atom-ph

Directly imaging spin polarons in a kinetically frustrated Hubbard system

The emergence of quasiparticles in quantum many-body systems underlies the rich phenomenology in many strongly interacting materials. In the context of doped Mott insulators, magnetic polarons are quasiparticles that usually arise from an interplay between the kinetic energy of doped charge carriers and superexchange spin interactions. However, in kinetically frustrated lattices, itinerant spin polarons - bound states of a dopant and a spin-flip - have been theoretically predicted even in the absence of superexchange coupling. Despite their important role in the theory of kinetic magnetism, a microscopic observation of these polarons is lacking. Here we directly image itinerant spin polarons in a triangular lattice Hubbard system realised with ultracold atoms, revealing enhanced antiferromagnetic correlations in the local environment of a hole dopant. In contrast, around a charge dopant, we find ferromagnetic correlations, a manifestation of the elusive Nagaoka effect. We study the evolution of these correlations with interactions and doping, and use higher-order correlation functions to further elucidate the relative contributions of superexchange and kinetic mechanisms. The robustness of itinerant spin polarons at high temperature paves the way for exploring potential mechanisms for hole pairing and superconductivity in frustrated systems. Furthermore, our work provides microscopic insights into related phenomena in triangular lattice moiré materials.

cond-mat.quant-gas

Collective flow of fermionic impurities immersed in a Bose-Einstein Condensate

Interacting mixtures of bosons and fermions are ubiquitous in nature. They form the backbone of the standard model of physics, provide a framework for understanding quantum materials and are of technological importance in helium dilution refrigerators. However, the description of their coupled thermodynamics and collective behaviour is challenging. Bose-Fermi mixtures of ultracold atoms provide a platform to investigate their properties in a highly controllable environment, where the species concentration and interaction strength can be tuned at will. Here we characterize the collective oscillations of spin-polarized fermionic impurities immersed in a Bose-Einstein condensate as a function of the interaction strength and temperature. For strong interactions, the Fermi gas perfectly mimics the superfluid hydrodynamic modes of the condensate, from low-energy quadrupole modes to high-order Faraday excitations. With an increasing number of bosonic thermal excitations, the dynamics of the impurities cross over from the collisionless to the hydrodynamic regime, reminiscent of the emergence of hydrodynamics in two-dimensional electron fluids.

cond-mat.quant-gas

Accelerating analysis of Boltzmann equations using Gaussian mixture models: Application to quantum Bose-Fermi mixtures

The Boltzmann equation is a powerful theoretical tool for modeling the collective dynamics of quantum many-body systems subject to external perturbations. Analysis of the equation gives access to linear response properties including collective modes and transport coefficients, but often proves intractable due to computational costs associated with multidimensional integrals describing collision processes. Here, we present a method to resolve this bottleneck, enabling the study of a broad class of many-body systems that appear in fundamental science contexts and technological applications. Specifically, we demonstrate that a Gaussian mixture model can accurately represent equilibrium distribution functions, thereby allowing efficient evaluation of collision integrals. Inspired by cold atom experiments, we apply this method to investigate the collective behavior of a quantum Bose-Fermi mixture of cold atoms in a cigar-shaped trap, a system that is particularly challenging to analyze. We focus on monopole and quadrupole collective modes above the Bose-Einstein transition temperature, and find a rich phenomenology that spans interference effects between bosonic and fermionic collective modes, dampening of these modes, and the emergence of hydrodynamics in various parameter regimes. These effects are readily verifiable experimentally.

cond-mat.quant-gas

Probing site-resolved correlations in a spin system of ultracold molecules

Synthetic quantum systems with interacting constituents play an important role in quantum information processing and in elucidating fundamental phenomena in many-body physics. Following impressive advances in cooling and trapping techniques, ensembles of ultracold polar molecules have emerged as a promising synthetic system that combines several advantageous properties. These include a large set of internal states for encoding quantum information, long nuclear and rotational coherence times and long-range, anisotropic interactions. The latter are expected to allow the exploration of intriguing phases of correlated quantum matter, such as topological superfluids, quantum spin liquids, fractional Chern insulators and quantum magnets. Probing correlations in these phases is crucial to understand their microscopic properties, necessitating the development of new experimental techniques. Here we use quantum gas microscopy to measure the site-resolved dynamics of quantum correlations in a gas of polar molecules in a two-dimensional optical lattice. Using two rotational states of the molecules, we realize a spin-1/2 system where the particles are coupled via dipolar interactions, producing a quantum spin-exchange model. Starting with the synthetic spin system prepared far from equilibrium, we study the evolution of correlations during the thermalization process for both spatially isotropic and anisotropic interactions. Furthermore, we study the correlation dynamics in a spin-anisotropic Heisenberg model engineered from the native spin-exchange model using Floquet techniques. These experiments push the frontier of probing and controlling interacting systems of ultracold molecules, with prospects for exploring new regimes of quantum matter and characterizing entangled states useful for quantum computation and metrology.

cond-mat.quant-gas

Observation of the Hanbury Brown and Twiss Effect with Ultracold Molecules

Measuring the statistical correlations of individual quantum objects provides an excellent way to study complex quantum systems. Ultracold molecules represent a powerful platform for quantum science due to their rich and controllable internal degrees of freedom. However, the detection of correlations between single molecules in an ultracold gas has yet to be demonstrated. Here we observe the Hanbury Brown and Twiss effect in a gas of bosonic $^{23}$Na$^{87}$Rb, enabled by the realization of a quantum gas microscope for molecules. We detect the characteristic bunching correlations in the density fluctuations of a 2D molecular gas released from and subsequently recaptured in an optical lattice. The quantum gas microscope allows us to extract the positions of individual molecules with single-site resolution. As a result, we obtain a high-contrast two-molecule interference pattern with a visibility of $54(13)\%$. While these measured correlations arise purely from the quantum statistics of the molecules, the demonstrated capabilities pave the way toward site-resolved studies of interacting molecular gases in optical lattices.

cond-mat.quant-gas

A Fermi-Hubbard Optical Tweezer Array

We use lithium-6 atoms in an optical tweezer array to realize an eight-site Fermi-Hubbard chain near half filling. We achieve single site detection by combining the tweezer array with a quantum gas microscope. By reducing disorder in the energy offsets to less than the tunneling energy, we observe Mott insulators with strong antiferromagnetic correlations. The measured spin correlations allow us to put an upper bound on the entropy of 0.26(4)$k_\mathrm{B}$ per atom, comparable to the lowest entropies achieved with optical lattices. Additionally, we establish the flexibility of the tweezer platform by initializing atoms on one tweezer and observing tunneling dynamics across the array for different 1D geometries.

cond-mat.quant-gas

Resonant and first-order dipolar interactions between ultracold molecules in static and microwave electric fields

We theoretically study collisions between ultracold polar molecules that are polarized by microwave or static electric fields. We systematically study the dependence on field strength, microwave polarization, and detuning from rotational transitions. We calculate the loss in two-body collisions that is observable experimentally and compare to the results expected for purely first-order dipolar interactions. For ground state molecules polarized by a static electric field, the dynamics are accurately described by first-order dipolar interactions. For microwave dressing, instead, resonant dipolar collisions dominate the collision process, in which molecules reorient along the intermolecular axis and interact with the full strength of the transition dipole. For red detuning, reorientation can only be suppressed at extreme Rabi frequencies. For blue detuned microwaves, resonant dipolar interactions dominate even for high Rabi frequencies, leading to microwave shielding for circular polarization and structured losses due to resonances for linear polarization. The results are presented numerically for fermionic $^{23}$Na$^{40}$K and bosonic $^{23}$Na$^{39}$K molecules.

physics.atom-ph

Resonant dipolar collisions of ultracold molecules induced by microwave dressing

We demonstrate microwave dressing on ultracold, fermionic ${}^{23}$Na${}^{40}$K ground-state molecules and observe resonant dipolar collisions with cross sections exceeding three times the $s$-wave unitarity limit. The origin of these collisions is the resonant alignment of the approaching molecules' dipoles along the intermolecular axis, which leads to strong attraction. We explain our observations with a conceptually simple two-state picture based on the Condon approximation. Furthermore, we perform coupled-channels calculations that agree well with the experimentally observed collision rates. While collisions are observed here as laser-induced loss, microwave dressing on chemically stable molecules trapped in box potentials may enable the creation of strongly interacting dipolar gases of molecules.

cond-mat.quant-gas

Bose polarons near quantum criticality

The emergence of quasiparticles in strongly interacting matter represents one of the cornerstones of modern physics. However, when different phases of matter compete near a quantum critical point, the very existence of quasiparticles comes under question. Here we create Bose polarons near quantum criticality by immersing atomic impurities in a Bose-Einstein condensate (BEC) with near-resonant interactions. Using locally-resolved radiofrequency spectroscopy, we probe the energy, spectral width, and short-range correlations of the impurities as a function of temperature. Far below the superfluid critical temperature, the impurities form well-defined quasiparticles. However, their inverse lifetime, given by their spectral width, is observed to increase linearly with temperature at the Planckian scale $\frac{k_B T}{\hbar}$, a hallmark of quantum critical behavior. Close to the BEC critical temperature, the spectral width exceeds the binding energy of the impurities, signaling a breakdown of the quasiparticle picture.

cond-mat.quant-gas

Second-Scale Nuclear Spin Coherence Time of Trapped Ultracold $^{23}$Na$^{40}$K Molecules

Coherence, the stability of the relative phase between quantum states, lies at the heart of quantum mechanics. Applications such as precision measurement, interferometry, and quantum computation are enabled by physical systems that have quantum states with robust coherence. With the creation of molecular ensembles at sub-$μ$K temperatures, diatomic molecules have become a novel system under full quantum control. Here, we report on the observation of stable coherence between a pair of nuclear spin states of ultracold fermionic NaK molecules in the singlet rovibrational ground state. Employing microwave fields, we perform Ramsey spectroscopy and observe coherence times on the scale of one second. This work opens the door for the exploration of single molecules as a versatile quantum memory. Switchable long-range interactions between dipolar molecules can further enable two-qubit gates, allowing quantum storage and processing in the same physical system. Within the observed coherence time, $10^4$ one- and two-qubit gate operations will be feasible.

cond-mat.quant-gas

Coherent Microwave Control of Ultracold $^{23}$Na$^{40}$K Molecules

We demonstrate coherent microwave control of rotational and hyperfine states of trapped, ultracold, and chemically stable $^{23}$Na$^{40}$K molecules. Starting with all molecules in the absolute rovibrational and hyperfine ground state, we study rotational transitions in combined magnetic and electric fields and explain the rich hyperfine structure. Following the transfer of the entire molecular ensemble into a single hyperfine level of the first rotationally excited state, $J{=}1$, we observe collisional lifetimes of more than $3\, \rm s$, comparable to those in the rovibrational ground state, $J{=}0$. Long-lived ensembles and full quantum state control are prerequisites for the use of ultracold molecules in quantum simulation, precision measurements and quantum information processing.

cond-mat.quant-gas