arXiv subjects

Zong-Quan Zhou

Publications and source records attributed to Zong-Quan Zhou.

At least 19 recordsLinked to original sources

arXiv2026

A Metropolitan-scale Multiplexed Quantum Repeater with Bell Nonlocality

Quantum repeaters can overcome exponential photon loss in optical fibers, enabling heralded entanglement between distant quantum memories. The definitive benchmark for this entanglement is Bell nonlocality; however, recent metropolitan-scale demonstrations based on single-photon interference (SPI) schemes have been limited to generating low-quality entanglement, falling short of Bell nonlocality certification. Here, we introduce a multiplexed quantum repeater protocol based on time measurements (MQR-TM), successfully combining the high heralding rate of SPI schemes with the phase robustness of two-photon interference (TPI) schemes. This approach achieves heralded entanglement distribution between two solid-state quantum memories over a record 14.5~km separation, generating a Bell state with a fidelity of $78.6 \pm 2.0\%$. We observe a CHSH-Bell inequality violation by 3.7 standard deviations, marking the first certification of Bell nonlocality in metropolitan-scale quantum repeaters. Our architecture supports autonomous quantum node operation without fiber channel phase stabilization, offering a practical framework for scalable quantum-repeater networks.

quant-ph↗

arXiv2026

Heterogeneous entanglement between a trapped ion and a solid-state quantum memory

Hybrid quantum networks offer a promising architecture for scalable quantum information processing and a future quantum internet, as they can combine the complementary strengths of disparate physical platforms. While single-atom systems provide deterministic quantum logic gates, atomic ensembles enable large-capacity quantum storage. However, generating entanglement between such heterogeneous systems has remained an open challenge, primarily due to fundamental spectral mismatches and system complexity. Here, we demonstrate a hybrid quantum network that entangles a single trapped $\mathrm{^{171}Yb^{+}}$ ion and a quantum memory based on $\rm ^{153}Eu^{3+}\colon\!Y_2SiO_5$ crystal over a 75-m separation. Using polarization-maintaining quantum frequency conversion, we map spin-photon entanglement onto a hybrid entanglement between a single spin qubit and a collective excitation of the quantum memory. The resulting entangled state achieves a fidelity of $(89.21 \pm 2.23)\%$ and violates the CHSH-Bell inequality by 6 standard deviations ($S = 2.328 \pm 0.055$), confirming nonlocality between two heterogeneous nodes. This work establishes entanglement between a quantum processing module with a multiplexed quantum memory node, representing a key step toward a scalable, multifunctional quantum internet.

quant-ph↗

arXiv2026

Global-scale quantum networking using hybrid-channel quantum repeaters with relays based on a chain of balloons

Global-scale entanglement distribution has been a formidable challenge due to the unavoidable losses in communication channels. Here, we propose a novel backbone channel for quantum network based on balloon-based aerial relays. We demonstrate for the first time that the atmospheric disturbances in balloon-based channels can be almost eliminated through optimizing beam waist positions and employing a series of adaptive optics systems, which boosts the channel efficiency to -21 dB over a 10,000 km distance, outperforming satellite-based relays by 12 dB with same device parameters. We then propose a global-scale quantum networking scheme based on hybrid-channel quantum repeaters that combine ground-based quantum repeaters and balloon-based aerial relays. Servers are interconnected globally via a chain of balloons, while clients link to local servers through fiber connections, facilitating rapid client switching and network scalability. Our simulations, employing state-of-the-art Eu$^{3+}$:Y$_2$SiO$_5$ quantum memories and mature entanglement sources based on spontaneous parametric down-conversion, demonstrate an entanglement distribution rate in the sub-Hertz range between clients separated by 10,000 km. This approach offers a practical path toward global quantum networking in the near future.

quant-ph↗

arXiv2025

Minute-Scale Photonic Quantum Memory

Long-lived storage of single photons is a fundamental requirement for enabling quantum communication and foundational tests of quantum physics over extended distances. While the implementation of a global-scale quantum network requires quantum storage times on the order of seconds to minutes, existing photonic quantum memories have so far been limited to subsecond lifetimes. Although $^{151}$Eu$^{3+}$:Y$_2$SiO$_5$ crystals exhibit substantially extended spin coherence times at the `magic' magnetic field, the concomitant weak optical absorption has until now prevented single-photon storage. Here, we overcome this challenge by integrating a noiseless photon echo protocol--which makes full use of the crystal's natural absorption for photonic storage--with a universally robust dynamical decoupling sequence incorporating adiabatic pulses to efficiently protect delocalized spin-wave excitation, enabling long-lived quantum storage at the `magic' magnetic field. At a storage time of 5.6 s, we achieve a time-bin qubit storage fidelity of 88.0 $\pm$ 2.1%, surpassing the maximum fidelity attainable via classical strategies. Our device reaches a $1/e$ storage lifetime of 27.6 $\pm$ 0.5 s, enabling single-photon-level storage for 42 s with a signal-to-noise ratio greater than unity. This work establishes photonic quantum memory in the minute-scale regime, laying a solid foundation for global-scale quantum network and deep-space quantum experiments.

quant-ph↗

arXiv2025

Efficient integrated quantum memory for light

Scalable implementation of quantum networks and photonic processors require integrated photonic memories with high efficiency, yet current integrated systems have been limited to storage efficiencies below 27.8%. Here, we demonstrate highly efficient integrated quantum memories based on rare-earth-iondoped crystals coupled with impedance-matched microcavities, realized in two novel architectures: 200-micrometer-thin membranes of Eu3+:Y2SiO5 integrated with fiber-based microcavities, and waveguide-based cavities fabricated using femtosecond lasers. Our approach achieves reliable integrated quantum storage with record efficiencies of 80.3(7)% for weak coherent pulses and 69.8(1.6)% for telecom-heralded single photons, alongside the storage of 20 temporal modes with an average efficiency of 51.3(2)%. Moreover, the thin-membrane Eu3+:Y2SiO5 architecture enables spectrally tunable efficient quantum storage via variable strain, providing a flexible interface for quantum networks. By combining high efficiency, large multimode capacity, and tunability, our devices establish a versatile hardware foundation for scalable quantum repeaters and chip-scale photonic processors.

quant-ph↗

arXiv2025

Multichannel and high dimensional integrated photonic quantum memory

Integrated photonic quantum memories are essential components for scalable quantum networks and photonic information processors. However, prior implementations have been confined to single-channel operation, limiting their capacity to manipulate multiple photonic pulses and support high-dimensional information. In this work, we introduce an 11-channel integrated quantum memory based on laser-written waveguide arrays in $^{151}$Eu$^{3+}$:Y$_2$SiO$_5$ crystals. On-chip electrode arrays enable independent control over the readout times for each channel via Stark-shift-induced atomic interference. Our device achieves random-access quantum storage of three time-bin qubits with a fidelity exceeding 99%, as well as storage of five-dimensional path-encoded quantum states with a fidelity above 96%. This multichannel integrated storage device enables versatile applications through its random access capability and lays a solid foundation for the development of high-dimensional quantum networks in integrated architectures.

quant-ph↗

arXiv2025

Remote Quantum Networks based on Quantum Memories

Quantum networks, capable of transmitting arbitrary quantum states, provide a foundation for a wide range of quantum applications, including distributed quantum computing, distributed quantum sensing, and quantum communication. Photons are the natural carrier of information in quantum networks, but the exponential loss of optical fiber channels prevents the construction of large-scale quantum networks. A potential solution is implementing quantum repeaters based on quantum memories, which can efficiently establish long-distance entanglement from short-distance entanglement. In the past decades, intense efforts have been devoted to constructing large-scale quantum networks based on various atomic quantum memories. In this Perspective, we present a concise overview of current advancements in remote quantum networks, elucidate the imminent challenges that must be addressed, and discuss the future directions.

quant-ph↗

arXiv2025

A hybrid-frequency on-chip programmable synthetic-dimension simulator with arbitrary couplings

High-performance photonic chips provide a powerful platform for analog computing, enabling the simulation of high-dimensional physical systems using low-dimensional devices with additional synthetic dimensions. The realization of large-scale complex simulations necessitates an architecture capable of arbitrary coupling configurations (encompassing symmetric, asymmetric and long-range coupling schemes) which is also crucial for scaling up. Previous approaches rely on excessive physical components to introduce asymmetric coupling, however, are restricted in reconfiguring and scaling by the relatively complicated structures. Here, to solve this problem, we propose a hybrid-frequency synthetic-dimension simulator architecture that combines both intra-resonant and inter-resonant frequency-lattice sites, and experimentally demonstrate it using the thin-film lithium niobate (TFLN) photonic chip. Employing this hybrid programmable architecture, we are able to simulate both the regular and long-range coupled forms of diverse compound-lattice models, such as the Hall ladder, Creutz ladder (symmetric) and Su-Schrieffer-Heeger (SSH, asymmetric) model, on a single chip, simultaneously reducing the experimental requirements significantly. As results, the direct readout of the bandstructure of the SSH model is able to be achieved, to be distinguished from all previous works, and important phenomena such as spin-momentum locking, topological flat band and Aharonov-Bohm cage effect are also observed with lower experimental requirements. Furthermore, applications like piecewise-continuous optical frequency shifting can be enabled by cascading our devices. Our results offer promising insights for future large-scale complex on-chip simulators with arbitrary couplings.

physics.optics↗

arXiv2025

A millisecond integrated quantum memory for photonic qubits

Quantum memories for light are essential building blocks for quantum repeaters and quantum networks. Integrated operations of quantum memories could enable scalable application with low-power consumption. However, the photonic quantum storage lifetime in integrated optical waveguide has so far been limited to tens of microseconds, falling short of the requirements for practical applications. Here, we demonstrate quantum storage of photonic qubits for 1.021 ms based on a laser-written optical waveguide fabricated in a 151Eu3+:Y2SiO5 crystal. Spin dephasing of 151Eu3+ is mitigated through dynamical decoupling applied via on-chip electric waveguides and we obtain a storage efficiency of 12.0(0.5)% at 1.021 ms, which is a demonstration of integrated quantum memories that outperforms the efficiency of a simple fiber delay line. Such long-lived waveguide-based quantum memory could support applications in quantum repeaters, and further combination with critical magnetic fields could enable potential application as transportable quantum memories.

quant-ph↗

arXiv2024

Nonlocal photonic quantum gates over 7.0 km

Quantum networks provide a prospective paradigm to connect separated quantum nodes, which relies on the distribution of long-distance entanglement and active feedforward control of qubits between remote nodes. Such approaches can be utilized to construct nonlocal quantum gates, forming building blocks for distributed quantum computing and other novel quantum applications. However, these gates have only been realized within single nodes or between nodes separated by a few tens of meters, limiting the ability to harness computing resources in large-scale quantum networks. Here, we demonstrate nonlocal photonic quantum gates between two nodes spatially separated by 7.0 km using stationary qubits based on multiplexed quantum memories, flying qubits at telecom wavelengths, and active feedforward control based on field-deployed fibers. Furthermore, we illustrate quantum parallelism by implementing the Deutsch-Jozsa algorithm and the quantum phase estimation algorithm between the two remote nodes. These results represent a proof-of-principle demonstration of quantum gates over metropolitan-scale distances and lay the foundation for the construction of large-scale distributed quantum networks relying on existing fiber channels.

quant-ph↗

arXiv2023

Realization of edge states along a synthetic orbital angular momentum dimension

The synthetic dimension is a rising method to study topological physics, which enables us to implement high-dimensional physics in low-dimensional geometries. Photonic orbital angular momentum (OAM), a degree of freedom characterized by discrete yet unbounded, serves as a suitable synthetic dimension. However, a sharp boundary along a synthetic OAM dimension has not been demonstrated, dramatically limiting the investigation of topological edge effects in an open boundary lattice system. In this work, we make a sharp boundary along a Floquet Su-Schrieffer-Heeger OAM lattice and form approximate semi-infinite lattices by drilling a pinhole on the optical elements in a cavity. The band structures with zero ($\pmπ$) energy boundary states are measured directly, benefiting from the spectra detection of the cavity. Moreover, we obtain the edge modes moving from the gap to the bulk by dynamically changing the boundary phase, and we reveal that interference near the surface leads to spectrum discretization. Our work provides a new perspective to observe edge effects and explore practical photonics tools.

physics.optics↗

arXiv2023

Counterfactual communication without a trace in the transmission channel

We report an experimental realization of a modified counterfactual communication protocol that eliminates the dominant environmental trace left by photons passing through the transmission channel. Compared to Wheeler's criterion for inferring past particle paths, as used in prior protocols, our trace criterion provide stronger support for the claim of the counterfactuality of the communication. We verify the lack of trace left by transmitted photons via tagging the propagation arms of an interferometric device by distinct frequency-shifts and finding that the collected photons have no frequency shift which corresponds to the transmission channel. As a proof of principle, we counterfactually transfer a quick response code image with sufficient fidelity to be scanned with a cell phone.

quant-ph↗

arXiv2023

Stark tuning of telecom single-photon emitters based on a single Er$^{3+}$

The implementation of scalable quantum networks requires photons at the telecom band and long-lived spin coherence. The single Er$^{3+}$ in solid-state hosts is an important candidate that fulfills these critical requirements simultaneously. However, to entangle distant Er$^{3+}$ ions through photonic connections, the emission frequency of individual Er$^{3+}$ in solid-state matrix must be the same, which is challenging because the emission frequency of Er$^{3+}$ depends on its local environment. Herein, we propose and experimentally demonstrate the Stark tuning of the emission frequency of a single Er$^{3+}$ in a Y$_2$SiO$_5$ crystal by employing electrodes interfaced with a silicon photonic crystal cavity. We obtain a Stark shift of 182.9 $\pm$ 0.8 MHz which is approximately 27 times of the optical emission linewidth, demonstrating the promising applications in tuning the emission frequency of independent Er$^{3+}$ into the same spectral channels. Our results provide a useful solution for construction of scalable quantum networks based on single Er$^{3+}$ and a universal tool for tuning emission of individual rare-earth ions.

quant-ph↗

arXiv2023

Nonclassical photon-pair source based on noiseless photon echo

The Duan-Lukin-Cirac-Zoller (DLCZ) scheme is a potential method to establish remote entanglements and realize large-scale quantum networks. Here we propose a DLCZ-like scheme based on the noiseless photon echo in rare-earth ion-doped crystals. Correlated photon pairs with a controllable delay can be created by the direct optical rephasing. Theoretical analysis indicates that the protocol is efficient in the low-optical-depth regime. This protocol could be feasibly implemented to establish long-lived quantum correlations between a photon and a spin-wave excitation in rare-earth ion-doped crystals.

quant-ph↗

arXiv2023

Laser Direct Writing of Visible Spin Defects in Hexagonal Boron Nitride for Applications in Spin-Based Technologies

Optically addressable spins in two-dimensional hexagonal boron nitride (hBN) attract widespread attention for their potential advantage in on-chip quantum devices, such as quantum sensors and quantum network. A variety of spin defects have been found in hBN, but no convenient and deterministic generation methods have been reported for other defects except negatively charged boron vacancy ($V_B^-$). Here we report that by using femtosecond laser direct writing technology, we can deterministically create spin defect ensembles with spectra range from 550 nm to 800 nm on nanoscale hBN flakes. Positive single-peak optically detected magnetic resonance (ODMR) signals are detected in the presence of magnetic field perpendicular to the substrate, and the contrast can reach 0.8%. With the appropriate thickness of hBN flakes, substrate and femtosecond laser pulse energy, we can deterministically and efficiently generate bright spin defect array. Our results provide a convenient deterministic method to create spin defects in hBN, which will motivate more endeavors for future researches and applications of spin-based technologies such as quantum magnetometer array.

physics.optics↗

arXiv2022

On-demand storage of photonic qubits at telecom wavelengths

Quantum memories at telecom wavelengths are crucial for the construction of large-scale quantum networks based on existing fiber networks. On-demand storage of telecom photonic qubits is a fundamental request for such networking applications but yet to be demonstrated. Here we demonstrate the storage and on-demand retrieval of telecom photonic qubits using a laser-written waveguide fabricated in an $^{167}$Er$^{3+}$:Y$_2$SiO$_5$ crystal. Both ends of the waveguide memory are directly connected with fiber arrays with a fiber-to-fiber efficiency of 51%. Storage fidelity of 98.3(1)% can be obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity that can be achieved with a classical measure and prepare strategy. This device features high reliability, easy scalability and can be directly integrated into fiber networks, which could play an essential role in fiber-based quantum networks.

quant-ph↗

arXiv2022

Extending the spin coherence lifetimes of ${}^{167}$Er$^{3+}$$:$Y$_2$SiO$_5$ at subkelvin temperatures

Er$^{3+}$$:$Y$_2$SiO$_5$ is a material of particular interest due to its suitability for telecom-band quantum memories and quantum transducers interfacing optical communication with quantum computers working in the microwave regime. Extending the coherence lifetimes of the electron spins and the nuclear spins is essential for implementing efficient quantum information processing based on such hybrid electron-nuclear spin systems. The electron spin coherence time of Er$^{3+}$$:$Y$_2$SiO$_5$ is so far limited to several microseconds, and there are significant challenges in optimizing coherence lifetimes simultaneously for both the electron and nuclear spins. Here we perform a pulsed-electron-nuclear-double-resonance investigation for an Er$^{3+}$-doped material at subkelvin temperatures. At the lowest working temperature, the electron spin coherence time reaches 290 $\pm$ 17 $μ$s, which has been enhanced by 40 times compared with the previous results. In the subkelvin regime, a rapid increase in the nuclear spin coherence time is observed, and the longest coherence time of 738 $\pm$ 6 $μ$s is obtained. These extended coherence lifetimes could be valuable resources for further applications of Er$^{3+}$$:$Y$_2$SiO$_5$ in fiber-based quantum networks.

quant-ph↗

arXiv2022

On-demand multimode optical storage in a laser-written on-chip waveguide

Quantum memory is a fundamental building block for large-scale quantum networks. On-demand optical storage with a large bandwidth, a high multimode capacity and an integrated structure simultaneously is crucial for practical application. However, this has not been demonstrated yet. Here, we fabricate an on-chip waveguide in a $\mathrm {^{151}Eu^{3+}:Y_2SiO_5}$ crystal with insertion losses of 0.2 dB, and propose a novel pumping scheme to enable spin-wave atomic frequency comb (AFC) storage with a bandwidth of 11 MHz inside the waveguide. Based on this, we demonstrate the storage of 200 temporal modes using the AFC scheme and conditional on-demand storage of 100 temporal modes using the spin-wave AFC scheme. The interference visibility between the readout light field and the reference light field is $99.0\% \pm 0.6\%$ and $97\% \pm 3\%$ for AFC and spin-wave AFC storage, respectively, indicating the coherent nature of this low-loss, multimode and integrated storage device.

physics.optics↗