arXiv subjects

Zongzhi Zhang

Publications and source records attributed to Zongzhi Zhang.

5 recordsLinked to original sources

arXiv2026

Strain-controlled sign reversal of the anomalous Hall effect in Ru/[Co/Ni]$_N$ multilayers

The anomalous Hall effect (AHE) is a hallmark transport phenomenon in ferromagnets arising from relativistic spin-orbit interaction. Here, we report an unexpected sign reversal of the AHE in Ru/[Co/Ni]$_N$ multilayers controlled by the stacking sequence of the Ru layer. When Ru is placed beneath, rather than atop, the Co/Ni multilayers, the anomalous Hall signal switches from positive to negative. By systematically varying the multilayer repeat number N and combining transport measurements with first-principles calculations, we show that this reversal originates from in-plane tensile strain imposed by the Ru underlayer, which reshapes the electronic structure and redistributes Berry curvature near the Fermi level. Our findings establish interfacial strain as an effective knob for tuning Berry-curvature-driven transport and suggest a pathway toward strain-controlled topological transport phenomena in magnetic multilayers.

cond-mat.mtrl-sci↗

arXiv2026

Unveiling Orbital-mediated Ultrafast Demagnetization in Rare Earth-Transition-Metal Ferrimagnets

The ultimate speed limit of magnetic recording and spintronic devices is set by the efficiency of angular-momentum transfer during ultrafast demagnetization, yet its microscopic pathway in Rare-Earth-Transition-Metal (RE-TM) ferrimagnets remains debated. Here, we establish an orbital-mediated framework in which 3d spin-orbit coupling (SOC) governs angular momentum (AM) dissipation. Strong 3d-SOC in RE-Co enables sub-picosecond, single-step demagnetization via direct orbital-to-lattice transfer, whereas weak 3d-SOC in RE-Fe redirects AM into 4f orbitals, producing slower two-step dynamics. The second-stage rate scales with 4f-SOC strength, revealing a distinct orbital-mediated dissipation channel. Using time-resolved magneto-optical Kerr measurements, supported by an extended four-temperature model, corroborate this picture across diverse RE-TM systems (RE = Sm, Gd, Tb, Dy, Ho and TM = Fe, Co, CoNi). Our results identify the SOC-driven competition between 3d and 4f orbital channels as the universal mechanism governing ultrafast demagnetization in RE-TM ferrimagnets, enabling rational design of the switching speed for next-generation spintronic devices.

cond-mat.mtrl-sci↗

arXiv2020

Strongly modulated ultrafast demagnetization and magnetization precession dynamics in ferrimagnetic Gdx(CoFe)1-x alloys via 3d-4f intersublattice exchange coupling

Manipulation of the intersublattice interaction strengh (JRE-TM) in rare earth (RE)-transition metal (TM) alloys is a key issue to understand how efficiently the laser-induced angular momentum transfers from 3d to 4f spins and to have a better control of the ultrafast spin dynamics. In this work, the relationships between laser-induced demagnetization process and the intersublattice 3d-4f interaction for the GdCoFe alloys were systematically studied. The ultrafast two-stage demagnetization process could change into a one-stage mode as the angular momentum transferring channel between 3d and 4f spins is switched off, which could be modulated by JRE-TM. Furthermore, both the effective g-factor and damping constant deduced by the subsequently laser-induced magnetization precession process diverge at the angular momentum compensation point based on the ferromagnetic resonance method with the LLG equations. The results provide an alternative way to efficiently manipulate the ultrafast demagnetization time for practical applications.

cond-mat.mtrl-sci↗

arXiv2019

Picosecond spin-orbit torque switching of ferrimagnets

Spintronics provides an efficient platform for realizing non-volatile memory and logic devices. In these systems, data is stored in the magnetization of magnetic materials, and magnetization is switched in the writing process. In conventional spintronic devices, ferromagnetic materials are used which have a magnetization dynamics timescale of around the nanoseconds, setting a limit for the switching speed. Increasing the magnetization switching speed has been one of the challenges in spintronic research. In this work we take advantage of the ultrafast magnetization dynamics in ferrimagnetic materials instead of ferromagnets, and we use femtosecond laser pulses and a photoconductive Auston switch to create picosecond current pulses for switching the ferrimagnet. By anomalous Hall and magneto-optic Kerr (MOKE) measurement, we demonstrate the robust picosecond SOT driven magnetization switching of ferrimagnetic GdFeCo. The time-resolved MOKE shows more than 50 GHz magnetic resonance frequency of GdFeCo, indicating faster than 20 ps spin dynamics and tens of picosecond SOT switching speed. Our work provides a promising route to realize picosecond operation speed for non-volatile magnetic memory and logic applications.

physics.app-ph↗

arXiv2017

Influence of heavy metal materials on magnetic properties of Pt/Co/heavy metal tri-layered structures

Pt/Co/heavy metal (HM) tri-layered structures with interfacial perpendicular magnetic anisotropy (PMA) are currently under intensive research for several emerging spintronic effects, such as spinorbit torque, domain wall motion, and room temperature skyrmions. HM materials are used as capping layers to generate the structural asymmetry and enhance the interfacial effects. For instance, the Pt/Co/Ta structure attracts a lot of attention as it may exhibit large Dzyaloshinskii-Moriya interaction. However, the dependence of magnetic properties on different capping materials has not been systematically investigated. In this paper, we experimentally show the interfacial PMA and damping constant for Pt/Co/HM tri-layered structures through time-resolved magneto-optical Kerr effect measurements as well as magnetometry measurements, where the capping HM materials are W, Ta, and Pd. We found that the Co/HM interface plays an important role on the magnetic properties. In particular, the magnetic multilayers with a W capping layer features the lowest effective damping value, which may be attributed to the different spin-orbit coupling and interfacial hybridization between Co and HM materials. Our findings allow a deep understanding of the Pt/Co/HM tri-layered structures. Such structures could lead to a better era of data storage and processing devices.

cond-mat.mes-hall↗