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the n_TOF Collaboration

Publications and source records attributed to the n_TOF Collaboration.

8 recordsLinked to original sources

Direct Experiments of Neutron Capture on Stable and Unstable Isotopes for Stellar Nucleosynthesis Studies

Neutron-capture reactions provide essential nuclear-physics input for modeling the synthesis of heavy elements in stars. The growing precision of stellar spectroscopy and isotopic measurements in presolar SiC grains now demands cross sections with improved accuracy over the full energy range, and access to unstable nuclei relevant to slow (s-) process branchings and the intermediate (i-) process. This article reviews recent progress in direct neutron-capture measurements, focusing on time-of-flight (TOF) experiments at CERN n_TOF and complementary activation techniques. Substantial advances have been achieved for stable s-only and bottleneck isotopes, significantly improving constraints on s-process models. In parallel, the combination of high instantaneous neutron fluxes and advanced detector systems has facilitated first-time measurements of several radioactive branching-point nuclei. Feasibility studies, however, reveal current limitations related to sample availability, background conditions, and restricted energy coverage. In this context, the complementarity between TOF and activation emerges as a central strategy. Future developments, including high-flux facilities and novel inverse-kinematics experiments in ion storage rings, are expected to extend the boundaries of neutron-capture measurements, overcoming current limitation

nucl-ex

Characterisation of the neutron beam in the n_TOF-EAR2 experimental area at CERN following the spallation target upgrade

The n_TOF facility at CERN has undergone a major upgrade after the installation of a new spallation target, designed to improve the features of both neutron beamlines at the experimental areas 1 and 2 (EAR1 and EAR2) and the commissioning of a new experimental area (NEAR). Due to improved coupling of the spallation target with the EAR2 beamline, the upgrade resulted in a significantly increased neutron flux and improved neutron energy resolution. This paper presents the results of the commissioning phase that followed to characterise the EAR2 neutron beamline and validate the FLUKA Monte Carlo simulations of the facility. The main features of the neutron beam, namely the neutron flux, spatial profile and energy resolution, are evaluated and compared to the previous target. The neutron flux presents a general increase of 20% below 1 eV, 40% between 1 eV and 100 keV and 50% between 100 keV and 10 MeV. The measured width of the beam profile was 3 cm (FWHM) at the reference position for neutron capture measurements. The energy resolution with the new spallation target shows a significant improvement compared to the previous one. Moreover, FLUKA Monte Carlo simulations present a good agreement with the measured neutron flux and profile within uncertainties, and a remarkable reproduction of the energy resolution.

physics.ins-det

New measurement of $^{50}$Cr and $^{53}$Cr (n,$\gamma$) cross sections at n_TOF: a call for chromium nuclear data revision

$^{50}$Cr and $^{53}$Cr are very relevant in criticality safety benchmarks related to nuclear reactors. The discrepancies of up to 30% between the neutron capture cross section evaluations have an important effect on the $k_{eff}$ and $k_{\infty}$ in criticality benchmarks particularly sensitive to chromium. In this work, the $^{50,53}$Cr(n,$\gamma$) cross sections are to be determined between 1 and 100 keV with an 8-10% accuracy following the requirements of the NEA High Priority Request List (HPRL) to solve the current discrepancies. We have measured these reactions by the time-of-flight technique at the EAR1 experimental area of the n_TOF facility, using an array of four C$_6$D$_6$ detectors with very low neutron sensitivity. The highly-enriched samples used are significantly thinner than in previous measurements, thus minimizing the multiple-scattering effects. We have produced, and analysed with the R-matrix analysis code SAMMY, capture yields featuring 33 resonances of $^{50}$Cr and 51 of $^{53}$Cr with an accuracy between 5% and 9%, hence fulfilling the requirements made by the NEA. The differential and integral cross sections have been compared to previous data and evaluations. The new measured $^{50,53}$Cr(n,$\gamma$) cross sections provide a valuable input for upcoming evaluations, which are deemed necessary given that the results presented herein do not support the increase in both cross sections proposed in the recent INDEN evaluation.

nucl-ex

Recent highlights and prospects on (n,$γ$) measurements at the CERN n_TOF facility

Neutron capture cross-section measurements are fundamental in the study of the slow neutron capture (s-) process of nucleosynthesis and for the development of innovative nuclear technologies. One of the best suited methods to measure radiative neutron capture (n,$γ$) cross sections over the full stellar range of interest for all the applications is the time-of-flight (TOF) technique. Overcoming the current experimental limitations for TOF measurements, in particular on low mass unstable samples, requires the combination of facilities with high instantaneous flux, such as the CERN n_TOF facility, with detection systems with an enhanced detection sensitivity and high counting rate capabilities. This contribution presents a summary about the recent highlights in the field of (n,$γ$) measurements at n_TOF. The recent upgrades in the facility and in new detector concepts for (n,\g) measurements are described. Last, an overview is given on the existing limitations and prospects for TOF measurements involving unstable targets and the outlook for activation measurements at the brand new high-flux n_TOF-NEAR station.

nucl-ex

New detection systems for an enhanced sensitivity in key stellar (n,$γ$) measurements

Neutron capture cross-section measurements are fundamental in the study of astrophysical phenomena, such as the slow neutron capture (s-) process of nucleosynthesis operating in red-giant and massive stars. However, neutron capture measurements via the time-of-flight (TOF) technique on key $s$-process nuclei are often challenging. Difficulties arise from the limited mass ($\sim$mg) available and the high sample-related background in the case of the unstable $s$-process branching points. Measurements on neutron magic nuclei, that act as $s$-process bottlenecks, are affected by low (n,$γ$) cross sections and a dominant neutron scattering background. Overcoming these experimental challenges requires the combination of facilities with high instantaneous flux, such as n\_TOF-EAR2, with detection systems with an enhanced detection sensitivity and high counting rate capabilities. This contribution reviews some of the latest detector developments in detection systems for (n,$γ$) measurements at n\_TOF, such as i-TED, an innovative detection system which exploits the Compton imaging technique to reduce the dominant neutron scattering background and s-TED, a highly segmented total energy detector intended for high flux facilities. The discussion will be illustrated with results of the first measurement of key the $s$-process branching-point reaction $^{79}$Se(n,$γ$).

nucl-ex

New perspectives for neutron capture measurements in the upgraded CERN-n_TOF Facility

The n_TOF facility has just undergone in 2021 a major upgrade with the installation of its third generation spallation target that has been designed to optimize the performance of the two n_TOF time-of-flight lines. This contribution describes the key features and limitations for capture measurements in the two beam lines prior to the target upgrade and presents first results of (n,$γ$) measurements carried out as part of the commissioning of the upgraded facility. In particular, the energy resolution, a key factor for both increasing the signal-to-background ratio and obtaining accurate resonance parameters, has been clearly improved for the 20 m long vertical beam-line with the new target design while keeping the remarkably high resolution of the long beamline n_TOF-EAR1. The improvements in the n_TOF neutron beam-lines need to be accompanied by improvements in the instrumentation. A review is given on recent detector R&D projects aimed at tackling the existing challenges and further improving the capabilities of this facility.

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Measurement of the $^{154}$Gd(n,$γ$) cross section and its astrophysical implications

The neutron capture cross section of $^{154}$Gd was measured from 1 eV to 300 keV in the experimental area located 185 m from the CERN n\_TOF neutron spallation source, using a metallic sample of gadolinium, enriched to 67$\%$ in $^{154}$Gd. The capture measurement, performed with four C$_{6}$D$_{6}$ scintillation detectors, has been complemented by a transmission measurement performed at the GELINA time-of-flight facility (JRC-Geel), thus minimising the uncertainty related to sample composition. An accurate Maxwellian averaged capture cross section (MACS) was deduced over the temperature range of interest for s process nucleosynthesis modeling. We report a value of 880(50) mb for the MACS at $kT=30$ keV, significantly lower compared to values available in literature. The new adopted $^{154}$Gd(n,$γ$) cross section reduces the discrepancy between observed and calculated solar s-only isotopic abundances predicted by s-process nucleosynthesis models.

nucl-ex

First tests of the applicability of $γ$-ray imaging for background discrimination in time-of-flight neutron capture measurements

In this work we explore for the first time the applicability of using $γ$-ray imaging in neutron capture measurements to identify and suppress spatially localized background. For this aim, a pinhole gamma camera is assembled, tested and characterized in terms of energy and spatial performance. It consists of a monolithic CeBr$_3$ scintillating crystal coupled to a position-sensitive photomultiplier and readout through an integrated circuit AMIC2GR. The pinhole collimator is a massive carven block of lead. A series of dedicated measurements with calibrated sources and with a neutron beam incident on a $^{197}$Au sample have been carried out at n_TOF, achieving an enhancement of a factor of two in the signal-to-background ratio when selecting only those events coming from the direction of the sample.

physics.ins-det