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arXiv2014

Hard x-ray emission spectroscopy: a powerful tool for the characterization of magnetic semiconductors

This review aims to introduce the x-ray emission spectroscopy (XES) and resonant inelastic x-ray scattering (RIXS) techniques to the materials scientist working with magnetic semiconductors (e.g. semiconductors doped with 3d transition metals) for applications in the field of spin-electronics. We focus our attention on the hard part of the x-ray spectrum (above 3 keV) in order to demonstrate a powerful element- and orbital-selective characterization tool in the study of bulk electronic structure. XES and RIXS are photon-in/photon-out second order optical processes described by the Kramers-Heisenberg formula. Nowadays, the availability of third generation synchrotron radiation sources permits applying such techniques also to dilute materials, opening the way for a detailed atomic characterization of impurity-driven materials. We present the Kβ XES as a tool to study the occupied valence states (directly, via valence-to-core transitions) and to probe the local spin angular momentum (indirectly, via intra-atomic exchange interaction). The spin sensitivity is employed, in turn, to study the spin-polarized unoccupied states. Finally, the combination of RIXS with magnetic circular dichroism (RIXS-MCD) extends the possibilities of standard magnetic characterization tools.

cond-mat.mtrl-sci↗

arXiv2013

Dynamics and equilibration of Rydberg excitations in dissipative atomic ensembles

We study resonant optical excitations of strongly-interacting Rydberg states of atoms in the presence of relaxations. We employ the quantum stochastic (Monte Carlo) wavefunctions to simulate the dissipative dynamics of tens of atoms in two-dimensional lattices. We show that under typical experimental conditions involving slow Rydberg state decay and sizable relaxation of atomic coherences, on the time scale of several microseconds the atomic ensemble approaches a stationary state in which much of the quantum correlations between the atoms have decayed away. The steady state, however, exhibits strong classical correlations of Rydberg excitation probabilities.

quant-ph↗

arXiv2012

Spin-orbit coupling induced separation and hidden spin textures in spin-1 Bose-Einstein condensates

We analytically and numerically investigate the ground state of the spin-orbit coupled spin-1 Bose-Einstein condensates in an external parabolic potential. When the spin-orbit coupling strength $κ$ is comparable with that of the trapping potential, the density distribution centers of different components of the spinor condensate deviate evidently from the trap center in the plane wave and stripe phases. When $κ\gg1$, the magnitude of this deviation decreases as $κ$ is getting larger and larger. Correspondingly, periphery half-skyrmions textures arise. This deviation can be reflected by the non-uniform magnetic moment in the $z$ direction, $\mathcal{F}_z$. With the manipulation of the external trap, the local magnitude of $\mathcal{F}_z$ can be increased evidently. This kind of increase of $\mathcal{F}_z$ is also observed in the square vortex lattice phase of the condensate.

physics.atom-ph↗

arXiv2013

Accelerated Thermalisation of 39K atoms in a Magnetic Trap with Superimposed Optical Potential

We report the rapid accelerated thermalisation of Potassium 39 K atoms loaded in a magnetic trap, in the presence of a single dipole trap beam. More than an order of magnitude reduction in the thermalisation time, to less than a second, is observed with the focused off- resonant beam occupying only 0.01% of the volume of the magnetic trap. The cold atoms are loaded from a Magneto-Optical Trap(MOT) of 39 K that has gone through a compressed MOT and sub-Doppler cooling stage. The atoms are prepared in the magnetically stretched |F = 2, mF = 2> state prior to loading into the hybrid trap. We also report a direct loading of 39 K atoms, prepared in the state |F = 1>, into a single beam dipole trap.

physics.atom-ph↗

arXiv2013

Multidimensional high harmonic spectroscopy: A semi-classical perspective on measuring multielectron rearrangement upon ionization

High harmonic spectroscopy has the potential to combine attosecond temporal with sub-Angstrom spatial resolution of the early nuclear and multielectron dynamics in molecules. It involves strong field ionization of the molecule by the IR laser field followed by time-delayed recombination of the removed electron with the molecular ion. The time-delay is controlled on the attosecond time scale by the oscillation of the IR field and is mapped into the harmonic number, providing a movie of molecular dynamics between ionization and recombination. One of the challenges in the analysis of high harmonic signal stems from the fact that the complex dynamics of both ionization and recombination with their multiple observables are entangled in the harmonic signal. Disentangling this information requires multidimensional approach, capable of mapping ionization and recombination dynamics into different independent parameters. We suggest multidimensional high harmonic spectroscopy as a tool for characterizing of ionization and recombination processes separately allowing for simultaneous detection of both the ionization delays and sub-cycle ionization rates. Our method extends the capability of the two dimensional (2D) set-up suggested recently by Shafir et al on reconstructing ionization delays, while keeping the reconstruction procedure as simple as in the original proposal. The scheme is based on the optimization of the high harmonic signal in orthogonally polarized strong fundamental and relatively weak multicolour control fields.

physics.atom-ph↗

arXiv2013

Coherent and incoherent processes responsible for various characteristics of nonlinear magneto-optical signals in rubidium atoms

We present the results of an investigation of the different physical processes that influence the shape of the nonlinear magneto-optical signals both at small magnetic field values (~ 100 mG) and at large magnetic field values (several tens of Gauss). We used a theoretical model that provided an accurate description of experimental signals for a wide range of experimental parameters. By turning various effects "on" or "off" inside this model, we investigated the origin of different features of the measured signals. We confirmed that the narrowest structures, with widths on the order of 100 mG, are related mostly to coherences among ground-state magnetic sublevels. The shape of the curves at other scales could be explained by taking into account the different velocity groups of atoms that come into and out of resonance with the exciting laser field. Coherent effects in the excited state can also play a role, although they mostly affect the polarization components of the fluorescence. The results of theoretical calculations are compared with experimental measurements of laser induced fluorescence from the D2 line of atomic rubidium as a function of magnetic field.

physics.atom-ph↗

arXiv2013

α-Decay in Ultra-Intense Laser Fields

We investigate the α-decay of a spherical nucleus under the influence of an ultra-intense laser field for the case when the radius vector joining the center-of-masses of the α-particle and the daughter is aligned with the direction of the external field. The time-independent part of the α-daughter interaction is taken from elastic scattering compilations whereas the time-varying part describes the interaction between the decaying system with the laser field. The time-dependent Schrödinger equation is solved numerically by appealing to a modified scheme of the Crank-Nicolson type where an additional first-order time derivative appears compared to the field-free case. The tunneling probability of the α-cluster, and derived quantities (decay rate, total flux) is determined for various laser intensities and frequencies for either continous waves or few-cycle pulses of envelope function F(t)=1. We show that in the latter case pulse sequences containing an odd number of half-cycles determine an enhancement of the tunneling probability compared to the field-free case and the continuous wave case. The present study is carried out taking as example the alpha decaying nucleus $^{106}$Te.

nucl-th↗

arXiv2012

ICP polishing of silicon for high quality optical resonators on a chip

Miniature concave hollows, made by wet etching silicon through a circular mask, can be used as mirror substrates for building optical micro-cavities on a chip. In this paper we investigate how ICP polishing improves both shape and roughness of the mirror substrates. We characterise the evolution of the surfaces during the ICP polishing using white-light optical profilometry and atomic force microscopy. A surface roughness of 1 nm is reached, which reduces to 0.5 nm after coating with a high reflectivity dielectric. With such smooth mirrors, the optical cavity finesse is now limited by the shape of the underlying mirror.

physics.optics↗

arXiv2018

Phase- and intensity-resolved measurements of above threshold ionization by few-cycle pulses

We investigate the carrier-envelope phase and intensity dependence of the longitudinal momentum distribution of photoelectrons resulting from above-threshold ionization of argon by few-cycle laser pulses. The intensity of the pulses with a center wavelength of 750\,nm is varied in a range between $0.7 \times 10^{14}$ and $\unit[5.5 \times 10^{14}]{W/cm^2}$. Our measurements reveal a prominent maximum in the carrier-envelope phase-dependent asymmetry at photoelectron energies of 2\,$U_\mathrm{P}$ ($U_\mathrm{P}$ being the ponderomotive potential), that is persistent over the entire intensity range. Further local maxima are observed at 0.3 and 0.8\,$U_\mathrm{P}$. The experimental results are in good agreement with theoretical results obtained by solving the three-dimensional time-dependent Schrödinger equation (3D TDSE). We show that for few-cycle pulses, the carrier-envelope phase-dependent asymmetry amplitude provides a reliable measure for the peak intensity on target. Moreover, the measured asymmetry amplitude exhibits an intensity-dependent interference structure at low photoelectron energy, which could be used to benchmark model potentials for complex atoms.

physics.atom-ph↗

arXiv2018

Density profiles of two-component Bose-Einstein condensates interacting with a Laguerre-Gaussian Beam

The density profiles of trapped two-component Bose-Einstein condensates (BEC) and its microscopic interaction with Laguerre Gaussian (LG) beam are studied. We consider the $^{87}$Rb BEC in two hyperfine spin components. The wavelength of the LG beam is assumed to be comparable to the atomic de-Broglie wavelength. Competitions between intra- and inter-component interactions produce interesting density structures of the ground state of BEC. We demonstrate vortex-antivortex interference and its dependence on the inter-component interactions and Raman transitions.

physics.atom-ph↗

arXiv2013

Dispersive regime of the Jaynes-Cummings and Rabi lattice

Photon-based strongly-correlated lattice models like the Jaynes-Cummings and Rabi lattices differ from their more conventional relatives like the Bose-Hubbard model by the presence of an additional tunable parameter: the frequency detuning between the pseudo-spin degree of freedom and the harmonic mode frequency on each site. Whenever this detuning is large compared to relevant coupling strengths, the system is said to be in the dispersive regime. The physics of this regime is well-understood at the level of a single Jaynes-Cummings or Rabi site. Here, we extend the theoretical description of the dispersive regime to lattices with many sites, for both strong and ultra-strong coupling. We discuss the nature and spatial range of the resulting qubit-qubit and photon-photon coupling, demonstrate the emergence of photon- pairing and squeezing, and illustrate our results by exact diagonalization of the Rabi dimer.

cond-mat.mes-hall↗

arXiv2013

Polarization effects on the effective temperature of an ultracold electron source

The influence has been studied of the ionization laser polarization on the effective temperature of an ultracold electron source, which is based on near-threshold photoionization. This source is capable of producing both high-intensity and high-coherence electron pulses, with applications in for example electron diffraction experiments. For both nanosecond and femtosecond photoionization, a sinusoidal dependence of the temperature on polarization angle has been found. For most experimental conditions, the temperature is minimal when the polarization coincides with the direction of acceleration. However, surprisingly, for nanosecond ionization a regime exists when the temperature is minimal when the polarization is perpendicular to the acceleration direction. This shows that in order to create electron bunches with the highest transverse coherence length, it is important to control the polarization of the ionization laser. The general trends and magnitudes of the temperature measurements are described by a model, based on the analysis of classical electron trajectories; this model further deepens our understanding of the internal mechanisms during the photoionization process. Furthermore, for nanosecond ionization, charge oscillations as a function of laser polarization have been observed; for most situations the oscillation amplitude is small.

physics.atom-ph↗

arXiv2013

Non-adiabatic control of quantum energy transfer in ordered and disordered arrays

An elementary excitation in an aggregate of coupled particles generates a collective excited state. We show that the dynamics of these excitations can be controlled by applying a transient external potential which modifies the phase of the quantum states of the individual particles. The method is based on an interplay of adiabatic and sudden time scales in the quantum evolution of the many-body states. We show that specific phase transformations can be used to accelerate or decelerate quantum energy transfer and spatially focus delocalized excitations onto different parts of arrays of quantum particles. We consider possible experimental implementations of the proposed technique and study the effect of disorder due to the presence of impurities on its fidelity. We further show that the proposed technique can allow control of energy transfer in completely disordered systems.

quant-ph↗

arXiv2013

Direct observation of zitterbewegung in a Bose-Einstein condensate

Zitterbewegung, a force-free trembling motion first predicted for relativistic fermions like electrons, was an unexpected consequence of the Dirac equation's unification of quantum mechanics and special relativity. Though the oscillatory motion's large frequency and small amplitude have precluded its measurement with electrons, zitterbewegung is observable via quantum simulation. We engineered an environment for 87Rb Bose-Einstein condensates where the constituent atoms behaved like relativistic particles subject to the one-dimensional Dirac equation. With direct imaging, we observed the sub-micrometer trembling motion of these clouds, demonstrating the utility of neutral ultracold quantum gases for simulating Dirac particles.

cond-mat.quant-gas↗

arXiv2013

Optical wire trap for cold neutral atoms

We propose a trap for cold neutral atoms using a fictitious magnetic field induced by a nanofiber-guided light field. In close analogy to magnetic side-guide wire traps realized with current-carrying wires, a trapping potential can be formed when applying a homogeneous magnetic bias field perpendicular to the fiber axis. We discuss this scheme in detail for laser-cooled cesium atoms and find trap depths and trap frequencies comparable to the two-color nanofiber-based trapping scheme but with one order of magnitude lower powers of the trapping laser field. Moreover, the proposed scheme allows one to bring the atoms closer to the nanofiber surface, thereby enabling efficient optical interfacing of the atoms with additional light fields. Specifically, optical depths per atom, $σ_0/A_{\rm eff}$, of more than 0.4 are predicted, making this system eligible for nanofiber-based nonlinear and quantum optics experiments.

quant-ph↗

arXiv2021

Buffer gas cooling of ions in time-dependent traps using ultracold atoms

For exploration of quantum effects with hybrid atom-ion systems, reaching ultracold temperatures is the major limiting factor. In this work, we present results on numerical simulations of trapped ion buffer gas cooling using an ultracold atomic gas in a large number of experimentally realistic scenarios. We explore the suppression of micromotion-induced heating effects through optimization of trap parameters for various radio-frequency (rf) traps and rf driving schemes including linear and octupole traps, digital Paul traps, rotating traps and hybrid optical/rf traps. We find that very similar ion energies can be reached in all of them even when considering experimental imperfections that cause so-called excess micromotion. Moreover we look into a quantum description of the system and show that quantum mechanics cannot save the ion from micromotion-induced heating in an atom-ion collision. The results suggest that buffer gas cooling can be used to reach close to the ion's groundstate of motion and is even competitive when compared to some sub-Doppler cooling techniques such as Sisyphus cooling. Thus, buffer gas cooling is a viable alternative for ions that are not amenable to laser cooling, a result that may be of interest for studies into quantum chemistry and precision spectroscopy.

physics.atom-ph↗

arXiv2017

Quantum mechanical study of high-order harmonic generation from HeH$^{2+}$ molecule in homogeneous and plasmonic-enhanced laser Fields

High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1sσ$ (ground state) and $2pσ$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields. The electron ionization and the enhancement of HHG yield in ground and first excited states, as the initial states, is studied and a strong orientation effect for ionization of electron in $2pσ$ state is discovered, that it can be used to reach a longer lifetime for the electron in the first excited state, which is responsible for the enhancement in HHG yield, during the high harmonic emission. In order to investigate effect of plasmonic field on the cutoff position of HHG spectra, first the enhancement of laser field in a nano-antennae is calculated and then the interaction of the enhanced field with HeH$^{2+}$ molecule is studied by solving the time-dependent Schrödinger equation. According to the results, when HeH$^{2+}$ molecule, in the initial state of $2pσ$, is irradiated by plasmonic polarized laser field, with the polarization normal to the molecular axis, the HHG yield and cutoff position enhance while the excited state has a long lifetime during the HHG process.

physics.atom-ph↗

arXiv2008

Bose-Einstein condensation on an atom chip

We report an experiment of creating Bose-Einstein condensate (BEC) on an atom chip. The chip based Z-wire current and a homogeneous bias magnetic field create a tight magnetic trap, which allows for a fast production of BEC. After an 4.17s forced radio frequency evaporative cooling, a condensate with about 3000 atoms appears. And the transition temperature is about 300nK. This compact system is quite robust, allowing for versatile extensions and further studying of BEC.

physics.atom-ph↗