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arXiv2013

Nonlinear dissipative dynamics of a two-component atomic condensate coupling with a continuum

We investigate the nonlinear dissipative coherence bifurcation and population dynamics of a two-component atomic Bose-Einstein condensate coupling with a continuum. The coupling between the two-component condensates and the continuum brings effective dissipations to the two-component condensates. The steady states and the coherence bifurcation depend on both dissipation and the nonlinear interaction between condensed atoms. The coherence among condensed atoms may be even enhanced by the effective dissipations. The combination of dissipation and nonlinearity allows one to control the switching between different self-trapped states or the switching between a self-trapped state and a non-self-trapped state.

cond-mat.quant-gas↗

arXiv2017

Current algebra, statistical mechanics and quantum models

Results obtained in the past for free boson systems at zero and nonzero temperature are revisited to clarify the physical meaning of current algebra reducible functionals which are associated to systems with density fluctuations, leading to observable effects on phase transitions. To use current algebra as a tool for the formulation of quantum statistical mechanics amounts to the construction of unitary representations of diffeomorphism groups. Two mathematical equivalent procedures exist for this purpose. One searches for quasi-invariant measures on configuration spaces, the other for a cyclic vector in Hilbert space. Here, one argues that the second approach is closer to the physical intuition when modelling complex systems. An example of application of the current algebra methodology to the pairing phenomenon in two-dimensional fermion systems is discussed.

quant-ph↗

arXiv2013

Detection system for forward emitted photons at the Experimental Storage Ring at GSI

A single photon counting system has been developed for efficient detection of forward emitted fluorescence photons at the Experimental Storage Ring (ESR) at GSI. The system employs a movable parabolic mirror with a central slit that can be positioned around the ion beam and a selected low noise photomultiplier for detection of the collected photons. Compared to the previously used system of mirror segments installed inside the ESR the collection efficiency for forward-emitted photons is improved by more than a factor of 5. No adverse effects on the stored ion beam have been observed during operation besides a small drop in the ion current of about 5% during movement of the mirror into the beam position. The new detection system has been used in the LIBELLE experiment at ESR and enabled for the first time the detection of the ground-state hyperfine M1 transition in lithium-like bismuth (209Bi80+) in a laser-spectroscopy measurement.

physics.atom-ph↗

arXiv2013

Analytical eigenstates for the quantum Rabi model

We develop a method to find analytical solutions for the eigenstates of the quantum Rabi model. These include symmetric, anti-symmetric and asymmetric analytic solutions given in terms of the confluent Heun functions. Both regular and exceptional solutions are given in a unified form. In addition, the analytic conditions for determining the energy spectrum are obtained. Our results show that conditions proposed by Braak [Phys. Rev. Lett. \textbf{107}, 100401 (2011)] are a type of sufficiency condition for determining the regular solutions. The well-known Judd isolated exact solutions appear naturally as truncations of the confluent Heun functions.

quant-ph↗

arXiv2014

Harmonic inversion analysis of exceptional points in resonance spectra

The spectra of, e.g. open quantum systems are typically given as the superposition of resonances with a Lorentzian line shape, where each resonance is related to a simple pole in the complex energy domain. However, at exceptional points two or more resonances are degenerate and the resulting non-Lorentzian line shapes are related to higher order poles in the complex energy domain. In the Fourier-transform time domain an $n$-th order exceptional point is characterised by a non-exponentially decaying time signal given as the product of an exponential function and a polynomial of degree $n-1$. The complex positions and amplitudes of the non-degenerate resonances can be determined with high accuracy by application of the nonlinear harmonic inversion method to the real-valued resonance spectra. We extend the harmonic inversion method to include the analysis of exceptional points. The technique yields, in the energy domain, the amplitudes of the higher order poles contributing to the spectra, and, in the time domain, the coefficients of the polynomial characterising the non-exponential decay of the time signal. The extended harmonic inversion method is demonstrated on two examples, viz. the analysis of exceptional points in resonance spectra of the hydrogen atom in crossed magnetic and electric fields, and an exceptional point occurring in the dynamics of a single particle in a time-dependent harmonic trap.

nlin.CD↗

arXiv2013

I$_{2}$ molecule for neutrino mass spectroscopy: ab initio calculation of spectral rate

It has recently been argued that atoms and molecules may become good targets of determining neutrino parameters still undetermined, if atomic/molecular process is enhanced by a new kind of coherence. We compute photon energy spectrum rate arising from coherent radiative neutrino pair emission processes of metastable excited states of I$_2$ and its iso-valent molecules, $|Av \rangle \rightarrow |Xv' \rangle + γ+ ν_iν_j$ and $|A'v \rangle \rightarrow |Xv' \rangle + γ+ ν_iν_j$ with $γ$ an IR photon and $ν_{i(j)}$ $i(j)-$th neutrino mass eigenstates, and show how fundamental neutrino parameters may be determined. Energies of electronically excited states of I$_2$, including the effect of spin-orbit couplings were calculated by the multiconfigurational second order perturbation (CASPT2) method. Summation over many vibrational levels of intermediate states is fully incorporated. Unlike atomic candidate of a much larger energy difference such as Xe, I$_2$ transitions from a vibrational level $A(v=0)$ to $X(v' = 24)$ give an opportunity of determination of the mass type (Majorana vs Dirac distinction) and determination of Majorana CPV (charge-conjugation parity violating) phases, although the rate is much smaller.

hep-ph↗

arXiv2026

Quantum simulation with Rydberg ions in a Penning trap

Quantum simulation of interacting many-body spin systems is routinely performed with cold trapped ions, and systems with hundreds of spins have been studied in one and two dimensions. In the most common realizations of these platforms, spin degrees of freedom are encoded in low-lying electronic levels, and interactions among the spins are mediated through crystal vibrations. Here we propose a new approach which enables the quantum simulation of two-dimensional spin systems with interaction strengths that are increased by orders of magnitude. This, together with the unprecedented longevity of trapped ions, opens an avenue for the exploration of phenomena that take place on long timescales, e.g., slow and collective relaxation in frustrated and kinetically constrained systems. Our platform makes use of the strong dipolar interactions among electronic Rydberg states and planar confinement provided by a Penning trap. We investigate how the strong electric and magnetic fields that form this trap affect the properties of the Rydberg states and show that spin-spin interaction strengths on the order of MHz are achievable under experimentally realistic conditions. As a brief illustration of the capabilities of this quantum simulator, we study the entanglement in a frustrated spin system realized by three ions.

quant-ph↗

arXiv2021

Electron-loss-to-continuum cusp in collisions of U$^{89+}$ with N$_{2}$ and Xe

We study the electron-loss-to-continuum (ELC) cusp experimentally and theoretically by comparing the ionization of U$^{89+}$ projectiles in collisions with N$_2$ and Xe targets, at a beam energy of 75.91 MeV/u. The coincidence measurement between the singly ionized projectile and the energy of the emitted electron is used to compare the shape of the ELC cusp at weak and strong perturbations. A significant energy shift for the centroid of the electron cusp is observed for the heavy target of Xe as compared to the light target of N$_2$. Our results provide a stringent test for fully relativistic calculations of double-differential cross sections performed in the first-order approximation and in the continuum-distorted-wave approach.

physics.atom-ph↗

arXiv2021

Structure and electron dynamics of planetary states of Sr below the Sr$^+$ $7d$ and $8p$ thresholds

In a combined experimental and theoretical study we investigate the $7dnl$ and $8pnl$ ($n\ge 11$, $l=9-12$) doubly-excited planetary states of Sr. The experimental spectrum was obtained using a five-photon resonant excitation scheme. The method of configuration interaction with exterior complex scaling was used to compute the energy-level structure and dynamics of the two highly excited electrons from first principles. Good quantitative agreement was obtained with the spectra we recorded, and the theoretical calculations shed light on their complex structure and the signatures of electron correlations therein. The two-electron probability densities we calculated reveal the strongly-correlated angular motion of the two electrons in the $7dnl$ and $8pnl$ planetary states, and confirm quantitatively the predictions of the frozen-planet approximation describing electron dynamics as the polarization of the fast inner electron by the electric field of the outer "frozen" electron.

physics.atom-ph↗

arXiv2021

Electron affinity of oganesson

The electron affinity (EA) of superheavy element Og is calculated by the use of the relativistic Fock-space coupled cluster (FSCC) and configuration interaction methods. The FSCC cluster operator expansion included single, double, and triple excitations treated in a non-perturbative manner. The Gaunt and retardation electron-electron interactions are taken into account. Both methods yield the results that are in agreement with each other. The quantum electrodynamics correction to EA is evaluated using the model Lamb-shift operator approach. The electron affinity of Og is obtained to be 0.076(4) eV.

physics.atom-ph↗

arXiv2021

Implementation of a time-dependent multiconfiguration self-consistent-field method for coupled electron-nuclear dynamics in diatomic molecules driven by intense laser pulses

We present an implementation of a time-dependent multiconfiguration self-consistent-field (TD-MCSCF) method [R. Anzaki et al., Phys. Chem. Chem. Phys. 19, 22008 (2017)] with the full configuration interaction expansion for coupled electron-nuclear dynamics in diatomic molecules subject to a strong laser field. In this method, the total wave function is expressed as a superposition of different configurations constructed from time-dependent electronic Slater determinants and time-dependent orthonormal nuclear basis functions. The primitive basis functions of nuclei and electrons are strictly independent of each other without invoking the Born-Oppenheimer approximation. Our implementation treats the electronic motion in its full dimensionality on curvilinear coordinates, while the nuclear wave function is propagated on a one-dimensional stretching coordinate with rotational nuclear motion neglected. We apply the present implementation to high-harmonic generation and dissociative ionization of a hydrogen molecule and discuss the role of electron-nuclear correlation.

physics.atom-ph↗

arXiv2022

High harmonics from backscattering of delocalized electrons

It is shown that electron backscattering can enhance high-harmonic generation in periodic systems with broken translational symmetry. Paradigmatically, we derive for a finite chain of atoms the harmonic cutoff due to electrons backscattered from the edges of the chain and demonstrate a maximum in the harmonic yield if twice the quiver amplitude of the driven electrons equals the chain length. For an intuitive understanding of our quantum results we develop a refined semiclassical trajectory model with finite electron-hole separation after tunneling. We demonstrate that the same "tunnel exit" also holds for interband harmonics in conventional periodic solid-state systems.

physics.atom-ph↗

arXiv2024

Atomic clock interferometry using optical tweezers

Clock interferometry refers to the coherent splitting of a clock into two different paths and recombining in a way that reveals the proper time difference between them. Unlike the comparison of two separate clocks, this approach allows testing how non-flat spacetime influences quantum coherence. Atomic clocks are currently the most accurate time keeping devices. Here we propose using optical tweezers to implement clock interferometry. Our proposed clock interferometer employs an alkaline-earth-like atom held in an optical trap at the magic wavelength. Through a combination of adiabatic, tweezer-based, splitting and recombining schemes and a modified Ramsey sequence on the clock states, we achieve a linear sensitivity to the gravitational time dilation. Moreover, the measurement of the time dilation is insensitive to relative fluctuations in the intensity of the tweezer beams. We analyze the tweezer clock interferometer and show that it is feasible with current technological capabilities. The proposed interferometer could test the effect of gravitational redshift on quantum coherence, and implement the quantum twin paradox.

quant-ph↗

arXiv2024

Role of spontaneously generated coherence (SGC) in laser cooling of atoms

The well-known sub-Doppler polarization gradient cooling in type-I transition ($F_e=F_g+1$) is caused by red-detuned lasers. On the other hand, in type-II transition ($F_e\le F_g$), sub-Doppler cooling takes place through blue-detuned lasers. This opposite behavior for the two types of transitions is due to SGC. In the absence of SGC, both types of transitions show blue-detuned cooling. In this work, we experimentally and theoretically demonstrate blue-detuned cooling for both types of transitions in $^{\textrm{87}}$Rb. For completeness, we compare the temperatures in various configurations.

physics.atom-ph↗

arXiv2011

Spectroscopy of diagnostically-important magnetic-dipole lines in highly-charged 3d$^n$ ions of tungsten

An electron beam ion trap (EBIT) is used to measure extreme ultraviolet spectra between 10 nm and 25 nm from highly-charged ions of tungsten with an open 3d shell (W XLVIII through W LVI). We found that almost all strong lines are due to the forbidden magnetic-dipole (M1) transitions within $3d^n$ ground configurations. A total of 37 spectral lines are identified for the first time using detailed collisional-radiative (CR) modeling of the EBIT spectra. A new level-merging scheme for compactification of rate equations is described. The CR simulations for Maxwellian plasmas show that several line ratios involving these M1 lines can be used to reliably diagnose temperature and density in hot fusion devices.

physics.atom-ph↗

arXiv2011

Repulsive long-range forces between anisotropic atoms and dielectrics

We investigate long-range forces between atoms with anisotropic electric polarizability interacting with dielectrics having anisotropic permittivity in the weak-coupling approximation. Unstable configurations in which the force between the objects is repulsive are constructed. Such configurations exist for three anisotropic atoms as well as for an anisotropic atom above a dielectric plate with a hole whose permittivity is anisotropic. Apart from the absolute magnitude of the force, the dependence on the configuration is qualitatively the same as for metallic objects for which the anisotropy is a purely geometric effect. In the weak limit closed analytic expressions for rather complicated configurations are obtained. The non-monotonic dependence of the interaction energy on separation is related to the fact that the electromagnetic Green's dyadic is not positive definite. The analysis in the weak limit is found to also semi-quantitatively explain the dependence of Casimir forces on the orientation of anisotropic dielectrics observed experimentally. Contrary to the scalar case, irreducible electromagnetic three-body energies can change sign. We trace this to the fact that the electromagnetic Green's dyadic is not positive definite.

physics.atom-ph↗

arXiv2012

Observation of a rotational transition in trapped and sympathetically cooled molecular ions

We demonstrate rotational excitation of molecular ions that are sympathetically cooled by laser-cooled atomic ions to a temperature as low as ca. 10 mK. The molecular hydrogen ions HD+ and the fundamental rotational transition $(v=0,\, N=0)\rightarrow(v'=0,\, N'=1)$ at 1.3 THz, the most fundamental dipole-allowed rotational transition of any molecule, are used as a test case. This transition is here observed for the first time directly. Rotational laser cooling was employed in order to increase the signal, and resonance-enhanced multiphoton dissociation was used as detection method. The black-body-radiation-induced rotational excitation is also observed. The extension of the method to other molecular species is briefly discussed.

quant-ph↗

arXiv2011

Conversion of bright magneto-optical resonances into dark at fixed laser frequency for D2 excitation of atomic rubidium

Nonlinear magneto-optical resonances on the hyperfine transitions belonging to the D2 line of rubidium were changed from bright to dark resonances by changing the laser power density of the single exciting laser field or by changing the vapor temperature in the cell. In one set of experiments atoms were excited by linearly polarized light from an extended cavity diode laser with polarization vector perpendicular to the light's propagation direction and magnetic field, and laser induced fluorescence (LIF) was observed along the direction of the magnetic field, which was scanned. A low-contrast bright resonance was observed at low laser power densities when the laser was tuned to the Fg=2 --> Fe=3 transition of Rb-87 and near to the Fg=3 --> Fe=4 transition of Rb-85. The bright resonance became dark as the laser power density was increased above 0.6mW/cm2 or 0.8 mW/cm2, respectively. When the Fg=2 --> Fe=3 transition of Rb-87 was excited with circularly polarized light in a second set of experiments, a bright resonance was observed, which became dark when the temperature was increased to around 50C. The experimental observations at room temperature could be reproduced with good agreement by calculations based on a theoretical model, although the theoretical model was not able to describe measurements at elevated temperatures, where reabsorption was thought to play a decisive role. The model was derived from the optical Bloch equations and included all nearby hyperfine components, averaging over the Doppler profile, mixing of magnetic sublevels in the external magnetic field, and a treatment of the coherence properties of the exciting radiation field.

physics.atom-ph↗