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Sympathetic Cooling of Mixed Species Two-Ion Crystals for Precision Spectroscopy

Sympathetic cooling of trapped ions has become an indispensable tool for quantum information processing and precision spectroscopy. In the simplest situation a single Doppler-cooled ion sympathetically cools another ion which typically has a different mass. We analytically investigate the effect of the mass ratio of such an ion crystal on the achievable temperature limit in the presence of external heating. As an example, we show that cooling of a single Al+ with Be+, Mg+ and Ca+ ions provides similar results for heating rates typically observed in ion traps, whereas cooling ions with a larger mass perform worse. Furthermore, we present numerical simulation results of the rethermalisation dynamics after a background gas collision for the Al+/Ca+ crystal for different cooling laser configurations.

physics.atom-ph↗

Ultranarrow CPO resonance in a Λ-type atomic system

It is well known that ultranarrow electromagnetically induced transparency (EIT) resonances can be observed in atomic gases at room temperature. We report here the experimental observation of another type of ultranarrow resonances, as narrow as the EIT ones, in a Λ-system selected by light polarization in metastable 4He at room temperature. It is shown to be due to coherent population oscillations in an open two-level system (TLS). For perpendicular linearly polarized coupling and probe beams, this system can be considered as two coupled open TLSs, in which the ground state populations exhibit anti-phase oscillations. We also predict theoretically that in case of two parallel polarizations, the system would behave like a closed TLS, and the narrow resonance associated with these oscillations would disappear.

physics.atom-ph↗

Numerical Computation of Dynamically Important Excited States of Many-Body Systems

We present an extension of the time-dependent Density Matrix Renormalization Group (t-DMRG), also known as Time Evolving Block Decimation algorithm (TEBD), allowing for the computation of dynamically important excited states of one-dimensional many-body systems. We show its practical use for analyzing the dynamical properties and excitations of the Bose-Hubbard model describing ultracold atoms loaded in an optical lattice from a Bose-Einstein condensate. This allows for a deeper understanding of nonadiabaticity in experimental realizations of insulating phases.

cond-mat.quant-gas↗

Spectral Lineshape Measurements with Shot-Noise Limited Accuracy

Spectroscopy has played the key role in revealing, and thereby understanding, the structure of atoms and molecules. A central drive in this field is the pursuit of higher precision and accuracy so that ever more subtle effects might be discovered. Here, we report on laser absorption spectroscopy that operates at the conventional quantum limit imposed by photon shot-noise. Furthermore, we achieve this limit without compromising the accuracy of the measurement. We demonstrate these properties by recording an absorption profile of cesium vapor at the 2 parts-per-million level. The extremely high signal-to-noise ratio allows us to directly observe the homogeneous lineshape component of the spectral profile, even while in the presence of Doppler broadening that is a factor of 100 times wider. We can do this because we can precisely measure the spectral profile at a frequency detuning more than 200 natural linewidths from the line center. We use the power of this tool to demonstrate direct measurements of a low-intensity optically-induced broadening process that is quite distinct from the well-known power broadening phenomenon.

physics.optics↗

Hyperfine structure of excited state of muonic helium atom

The recoil, vacuum polarization and electron vertex corrections of first and second orders in the fine structure constant $α$ and the ratio of electron to muon and electron to α-particle masses are calculated in the hyperfine splitting of the $1s^{(e)}_{1/2}2s^{(μ)}_{1/2}$ state of muonic helium atom (μe ^4_2He) on the basis of a perturbation theory. We obtain total result for the muonically excited state hyperfine splitting $Δν^{hfs}=4295.66$ MHz which improves previous calculations due to the account of new corrections and more accurate treatment of the electron vertex contribution.

hep-ph↗

Observation of interspecies Li-Cs Feshbach resonances

We report on the observation of nineteen interspecies Feshbach resonances in an optically trapped ultracold Bose-Fermi mixture of ^{133}Cs and ^{6}Li in the two energetically lowest spin states. We assign the resonances to s- and p-wave molecular channels by a coupled-channels calculation, resulting in an accurate determination of LiCs ground state potentials. Fits of the resonance position based on the undressed Asymptotic Bound State model do not provide the same level of accuracy as the coupled-channels calculation. Several broad s-wave resonances provide prospects to create fermionic LiCs molecules with a large dipole moment via Feshbach association followed by stimulated Raman passage. Two of the s-wave resonances overlap with a zero crossing of the Cs scattering length which offers prospects for the investigation of polarons in an ultracold Li-Cs mixture.

cond-mat.quant-gas↗

Experimental access to higher-order Zeeman effects by precision spectroscopy of highly charged ions in a Penning trap

We present an experimental concept and setup for laser-microwave double-resonance spectroscopy of highly charged ions in a Penning trap. Such spectroscopy allows a highly precise measurement of the Zeeman splittings of fine- and hyperfine-structure levels due the magnetic field of the trap. We have performed detailed calculations of the Zeeman effect in the framework of quantum electrodynamics of bound states as present in such highly charged ions. We find that apart from the linear Zeeman effect, second- and third-order Zeeman effects also contribute to the splittings on a level of 10^-4 and 10^-8, respectively, and hence are accessible to a determination within the achievable spectroscopic resolution of the ARTEMIS experiment currently in preparation.

physics.atom-ph↗

Entanglement-assisted scheme for nondemolition detection of the presence of a single photon

In this paper, we propose a resources-optimal linear-optical scheme for quantum nondemolition detection of single-photon presence. By measuring the state of ancillary photons, the presence of a photon in signal mode is revealed with a success probability of 1/2 without any disturbance to its state. We also show how to tune the setup to perform quantum nondemolition measurement of the signal photon state, and we provide tradeoff between the extracted information and the signal state disturbance. Moreover, the optimality of resources and methods by which to increase the success probability are discussed.

quant-ph↗

Adiabatic quantum computation with Rydberg-dressed atoms

We study an architecture for implementing adiabatic quantum computation with trapped neutral atoms. Ground state atoms are dressed by laser fields in a manner conditional on the Rydberg blockade mechanism, thereby providing the requisite entangling interactions. As a benchmark we study the performance of a Quadratic Unconstrained Binary Optimization (QUBO) problem whose solution is found in the ground state spin configuration of an Ising-like model. We model a realistic architecture, including details of the atomic implementation, with qubits encoded into the clock states of 133Cs, effective B-fields implemented through stimulated Raman transitions, and atom-atom coupling achieved by excitation to the 100P3/2 Rydberg level. Including the fundamental effects of photon scattering, we find the fidelity of two-qubit implementation to be on the order of 0.99, with higher fidelities possible with improved laser sources.

quant-ph↗

High resolution photoassociation spectroscopy of the $^{6}$Li$_2$ $1^{3}Σ_{g}^{+}$ state

We present experimental observations of seven vibrational levels $v'=20-26$ of the $1^{3}Σ_{g}^{+}$ excited state of Li$_2$ molecules by the photoassociation (PA) of a degenerate Fermi gas of $^6$Li atoms. For each vibrational level, we resolve the rotational structure using a Feshbach resonance to enhance the PA rates from p-wave collisions. We also, for the first time, determine the spin-spin and spin-rotation interaction constants for this state. The absolute uncertainty of our measurements is $\pm 0.00002$ cm$^{-1}$ ($\pm 600$ kHz). We use these new data to further refine an analytic potential for this state.

physics.atom-ph↗

Hyperfine-induced effects on the linear polarization of the K$α_1$ emission from helium-like ions

The linear polarization of the characteristic photon emission from few-electron ions is studied for its sensitivity with regard to the nuclear spin and magnetic moment of the ions. Special attention is paid, in particular, to the K$α_1$ ($1s 2p_{3/2} ^{1,3}P_{1,2} \to 1s^2 ^1S_0$) decay of selected helium-like ions following the radiative electron capture into initially hydrogen-like species. Based on the density matrix theory, a unified description is developed that includes both, the many-electron and hyperfine interactions as well as the multipole-mixing effects arising from the expansion of the radiation field. It is shown that the polarization of the K$α_1$ line can be significantly affected by the mutipole mixing between the leading $M2$ and hyperfine-induced $E1$ components of $1s2p ^3P_2, F_i \to 1s^2 ^1S_0, F_f$ transitions. This $E1$-$M2$ mixing strongly depends on the nuclear properties of the considered isotopes and can be addressed experimentally at existing heavy-ion storage rings.

nucl-th↗

Universal nature and finite-range corrections in elastic atom-dimer scattering below the dimer breakup threshold

We investigate universal behavior in elastic atom-dimer scattering below the dimer breakup threshold calculating the atom-dimer effective-range function $ak\cotδ$. Using the He-He system as a reference, we solve the Schrödinger equation for a family of potentials having different values of the two-body scattering length $a$ and we compare our results to the universal zero-range form deduced by Efimov, $ak\cotδ=c_1(ka)+c_2(ka)\cot[s_0\ln(κ_*a)+ϕ(ka)]$, for selected values of the three-body parameter $κ_*$. Using the parametrization of the universal functions $c_1,c_2,ϕ$ given in the literature, a good agreement with the universal formula is obtained after introducing a particular type of finite-range corrections. Furthermore, we show that the same parametrization describes a very different system: nucleon-deuteron scattering below the deuteron breakup threshold. Our analysis confirms the universal character of the process, and relates the pole energy in the effective-range function of nucleon-deuteron scattering to the three-body parameter $κ_*$.

cond-mat.quant-gas↗

Effect of two-beam coupling in strong-field optical pump-probe experiments

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a weak probe beam experiences a greater phase shift from a strong pump beam than the pump beam induces on itself. The physical mechanism behind the enhanced phase shift is diffraction of pump light into the probe direction by a nonlinear refractive index grating produced by interference between the two beams. For an instantaneous third-order response, the effect of the grating is to simply double the probe phase shift, but when delayed nonlinearities are considered, the effect is more complex. A comprehensive treatment is given for both degenerate and nondegenerate pump-probe experiments in noble and diatomic gases. Results of numerical calculations are compared to a recent transient birefringence measurement [Loriot et al., Opt. Express 17, 13429 (2009)] and a recent spectral interferometry experiment [Wahlstrand et al., Phys. Rev. A 85, 043820 (2012)]. We also present results from two new experiments using spectrally-resolved transient birefringence with 800 nm pulses in Ar and air and degenerate chirped pulse spectral interferometry in Ar. Both experiments support the interpretation of the negative birefringence at high intensity as arising from a plasma grating.

physics.optics↗

Transfer of orbital angular momentum of light using two component slow light

We study the manipulation of slow light with an orbital angular momentum propagating in a cloud of cold atoms. Atoms are affected by four copropagating control laser beams in a double tripod configuration of the atomic energy levels involved, allowing to minimize the losses at the vortex core of the control beams. In such a situation the atomic medium is transparent for a pair of copropagating probe fields, leading to the creation of two-component (spinor) slow light. We study the interaction between the probe fields when two control beams carry optical vortices of opposite helicity. As a result, a transfer of the optical vortex takes place from the control to the probe fields without switching off and on the control beams. This feature is missing in a single tripod scheme where the optical vortex can be transferred from the control to the probe field only during either the storage or retrieval of light.

quant-ph↗

Cooperative Fluorescence from a Strongly Driven Dilute Cloud of Atoms

We investigate cooperative fluorescence in a dilute cloud of strongly driven two-level emitters. Starting from the Heisenberg equations of motion, we compute the first-order scattering corrections to the saturation of the excited-state population and to the resonance-fluorescence spectrum, which both require going beyond the state-of-the-art linear-optics approach to describe collective phenomena. A dipole blockade is observed due to long range dipole-dipole coupling that vanishes at stronger driving fields. Furthermore, we compute the inelastic component of the light scattered by a cloud of many atoms and find that the Mollow triplet is affected by cooperativity. In a lobe around the forward direction, the inelastic Mollow triplet develops a spectral asymmetry, observable under experimental conditions.

physics.atom-ph↗

Effect of screening on spectroscopic properties of Li-like ions in plasma environment

This work presents accurate {\it ab initio} investigations of various spectroscopic properties of a few Li-like ions in presence of a plasma environment within the Debye screening potential. The coupled-cluster theory in the relativistic framework has been employed to compute ionization potentials, excitation energies, electric dipole oscillator strengths, and electric quadrupole transition probabilities of Li-like C$^{3+}$, N$^{4+}$, and O$^{5+}$ ions. The unretarded Breit interaction has been implemented to increase the accuracy of the calculations. The effects of ion density and temperature on the ionization potentials, excitation energies, electric dipole oscillator strengths, and electric quadrupole transition probabilities have been investigated in the plasma environment. It is found that the plasma screening leads to a sharp decrease in the ionization potential as the screening strength increases. With increasing strength, the oscillator strengths associated with 2$s ^{2}S_{1/2}$$\rightarrow2 p ^{2}P_{1/2, 3/2}$ transitions increase, whereas the transition probabilities associated with 3$d ^2D_{3/2, 5/2}$$\rightarrow2 s ^2S_{1/2}$ transitions decrease.

physics.atom-ph↗

Λ-enhanced Sub-Doppler Cooling of Lithium Atoms in D1 Gray Molasses

Following the bichromatic sub-Doppler cooling scheme on the D1 line of 40K recently demonstrated in (Fernandes et al. 2012), we introduce a similar technique for 7Li atoms and obtain temperatures of 60 uK while capturing all of the 5x10^8 atoms present from the previous stage. We investigate the influence of the detuning between the the two cooling frequencies and observe a threefold decrease of the temperature when the Raman condition is fulfilled. We interpret this effect as arising from extra cooling due to long-lived coherences between hyperfine states. Solving the optical Bloch equations for a simplified, Λ-type three-level system we identify the presence of an efficient cooling force near the Raman condition. After transfer into a quadrupole magnetic trap, we measure a phase space density of ~10^-5. This laser cooling offers a promising route for fast evaporation of lithium atoms to quantum degeneracy in optical or magnetic traps.

physics.atom-ph↗

Quantum dynamics of an atom orbiting around an optical nanofiber

We propose a novel platform for the investigation of quantum wave packet dynamics, offering a complementary approach to existing theoretical models and experimental systems. It relies on laser-cooled neutral atoms which orbit around an optical nanofiber in an optical potential produced by a red-detuned guided light field. We show that the atomic center-of-mass motion exhibits genuine quantum effects like collapse and revival of the atomic wave packet. As distinctive advantages, our approach features a tunable dispersion relation as well as straightforward readout for the wave packet dynamics and can be implemented using existing quantum optics techniques.

quant-ph↗