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arXiv2018

Halide perovskites: Is it all about the interfaces?

Design and modification of the interfaces, always a critical issue for semiconductor devices, has become the primary tool to harness the full potential of halide perovskite (HaP)-based ones. In particular the outstanding improvements in HaP solar cell performance and stability can be primarily ascribed to a careful choice of the interfacial layout in the layer stack. In this review we describe the unique challenges and opportunities of these approaches (section A). For this purpose, we first elucidate the basic physical and chemical properties of the exposed HaP thin film and crystal surface (section B). We then lay out the energetic alignment processes to adjacent transport and buffer layers (section C) and finally elaborate on the impact of the interface formation on how well/poor a device functions. Based on those sections we then present a road map for the next steps in interfacial design principles for HaP semiconductors (section D).

physics.app-ph↗

arXiv2018

Three-dimensional nanoprinting via charged aerosol focusing

A powerful and flexible method of 3D nano-printing, based on focusing charged aerosol, has been developed. The self-consistent electric field configuration, created with a holey floating mask and used as the scaffold for printing structures, has no restriction as to sizes down to nano-scale. The electric field line is used as a writing tool. Broad material independence opens the way for producing hybrid structures that are essential for electronic devices. The method contains three modes which are complementary: controlled tip-directed 3D-growth printing, the writing mode (that can also produce 3D structures in repeating passages), and the stencil mode that produces wall-like structures of various shapes. Manipulating them gives freedom to manufacture complex 3D designs that we report. The desired morphology of the grown structures is controlled according to a simple phenomenological theory that helps organize the 2D stage motion and the 3D printing process to compete with the 3D printing provided by laser techniques in polymer based material.

physics.app-ph↗

arXiv2018

Application of the method of multiple scales to unravel energy exchange in nonlinear locally resonant metamaterials

In this paper, the effect of weak nonlinearities in 1D locally resonant metamaterials is investigated via the method of multiple scales. Commonly employed to the investigate the effect of weakly nonlinear interactions on the free wave propagation through a phononic structure or on the dynamic response of a Duffing oscillator, the method of multiple scales is here used to investigate the forced wave propagation through locally resonant metamaterials. The perturbation approach reveals that energy exchange may occur between propagative and evanescent waves induced by quadratic nonlinear local interaction.

physics.app-ph↗

arXiv2018

A Novel PN junction between Mechanically Exfoliated \b{eta}-Ga2O3 and p-GaN

Several pn junctions were constructed from mechanically exfoliated ultrawide bandgap (UWBG) beta-phase gallium oxide (\b{eta}-Ga2O3) and p-type gallium nitride (GaN). The mechanical exfoliation process, which is described in detail, is similar to that of graphene and other 2D materials. Atomic force microscopy (AFM) scans of the exfoliated \b{eta}-Ga2O3 flakes show very smooth surfaces with average roughness of 0.647 nm and transmission electron microscopy (TEM) scans reveal flat, clean interfaces between the \b{eta}-Ga2O3 flakes and p-GaN. The device showed a rectification ratio around 541.3 (V+5/V-5). Diode performance improved over the temperature range of 25°C and 200°C, leading to an unintentional donor activation energy of 135 meV. As the thickness of exfoliated \b{eta}-Ga2O3 increases, ideality factors decrease as do the diode turn on voltages, tending toward an ideal threshold voltage of 3.2 V as determined by simulation. This investigation can help increase study of novel devices between mechanically exfoliated \b{eta}-Ga2O3 and other materials.

physics.app-ph↗

arXiv2018

Ultrathin acoustic parity-time symmetric metasurface cloak

Invisibility or unhearability cloaks have been made possible by using metamaterials making light or sound flow around obstacle without the trace of reflections or shadows. Metamaterials are known for being flexible building units that can mimic a host of unusual and extreme material responses, which are essential when engineering artificial material properties to realize a coordinate transforming cloak. Bending and stretching the coordinate grid in space requires stringent material parameters, therefore, small inaccuracies and inevitable material losses become sources for unwanted scattering that are decremental to the desired effect. These obstacles further limit the possibility to achieve a robust concealment of sizeable objects from either radar or sonar detection. By using a elaborate arrangement of gain and lossy acoustic media respecting parity-time symmetry, we built an one-way unhearability cloak capable to hide objects seven times larger than acoustic wavelength. Generally speaking, our approach has no limits in terms of working frequency, shape, or size, specifically though, we demonstrate how, in principle, an object of the size of a human can be hidden from audible sound.

physics.app-ph↗

arXiv2018

My, and others', spiking memristors are true memristors: a response to R.S. Williams' question at the New Memory Paradigms: Memristive Phenomena and Neuromorphic Applications Faraday Discussion

At the Faraday Discussion, in the paper titled `Neuromorphic computation with spiking memristors: habituation, experimental instantiation of logic gates and a novel sequence-sensitive perceptron model' it was demonstrated that a large amount of computation could be done in a sequential way using memristor current spikes (d.c. response). As these spikes are found in many memristors (possibly all), this novel approach could be highly useful for fast and reproducible memristor circuits. However, questions were raised as to whether these spikes were actually due to memristance or merely capacitance in the circuit. In this longer version of the Faraday Discussion response, as much information as is available from both published and unpublished data from my lab is marshalled together. We find that the devices are likely imperfect memristors with some capacitance, and that the spikes are related to the frequency effect seen in memristor hysteresis curves, thus are an integral part of memristance.

cs.ET↗

arXiv2018

Tuning bimetallic catalysts for a selective growth of SWCNTs

Recent advances in structural control during the synthesis of SWCNTs have in common the use of bimetallic nanoparticles as catalysts, despite the fact that their exact role is not fully understood. We therefore analyze the effect of the catalyst' s chemical composition on the structure of the resulting SWCNTs by comparing three bimetallic catalysts (FeRu, CoRu and NiRu). A specific synthesis protocol is designed to impede the catalyst nanoparticle coalescence mechanisms and stabilize their diameter distributions throughout the growth. Owing to the ruthenium component which has a limited carbon solubility, tubes grow in tangential mode and their diameter is close to that of their seeding nanoparticle. By using as-synthesized SWCNTs as a channel material in field effect transistors, we show how the chemical composition of the catalysts and temperature can be used as parameters to tune the diameter distribution and semiconducting-to-metallic ratio of SWCNT samples. Finally, a phenomenological model, based on the dependence of the carbon solubility as a function of catalyst nanoparticle size and nature of the alloying elements, is proposed to interpret the results.

physics.app-ph↗

arXiv2018

Mutual synchronization of constriction-based spin Hall nano-oscillators in weak in-plane fields

We study mutual synchronization in double nanoconstriction-based spin Hall nano-oscillators (SHNOs) under weak in-plane fields ($μ_0H_\mathrm{IP}$ = 30-40 mT) and also investigate its angular dependence. We compare SHNOs with different nano-constriction spacings of 300 and 900 nm. In all devices, mutual synchronization occurs below a certain critical angle, which is higher for the 300 nm spacing than for the 900 nm spacing, reflecting the stronger coupling at shorter distances. Alongside the synchronization, we observe a strong second harmonic consistent with predictions that the synchronization may be mediated by the propagation of second harmonic spin waves. However, although Brillouin Light Scattering microscopy confirms the synchronization, it fails to detect any related increase of the second harmonic. Micromagnetic simulations instead explain the angular dependent synchronization as predominantly due to magneto-dipolar coupling between neighboring SHNOs.

physics.app-ph↗

arXiv2018

Anti-fatigue-fracture hydrogels

The emerging applications of hydrogels in devices and machines require these soft materials to maintain robustness under cyclic mechanical loads. Whereas hydrogels have been made tough to resist fracture under a single cycle of mechanical load, these toughened gels still suffer from fatigue fracture under multiple cycles of loads. The reported fatigue threshold (i.e., the minimal fracture energy at which crack propagation occurs under cyclic loads) for synthetic hydrogels is on the order of 1-100 J/m2, which is primarily associated with the energy required to fracture a single layer of polymer chains per unit area. Here, we demonstrate that the controlled introduction of crystallinity in hydrogels can significantly enhance their fatigue thresholds, since the process of fracturing crystalline domains for fatigue-crack propagation requires much higher energy than fracturing a single layer of polymer chains. The fatigue threshold of polyvinyl alcohol (PVA) with a crystallinity of 18.9 wt.% in the swollen state can exceed 1,000 J/m2. We further develop a strategy to enhance the anti-fatigue-fracture properties of PVA hydrogels, but still maintain their high water contents and low moduli by patterning highly-crystalline regions in the hydrogels. The current work not only reveals an anti-fatigue-fracture mechanism in hydrogels but also provides a practical method to design anti-fatigue-fracture hydrogels for diverse applications.

physics.app-ph↗

arXiv2019

Innovative full-field chromatic confocal microscopy using multispectral sensors

A full-field chromatic confocal microscopy using a multispectral sensor was developed for quasi-one-shot microscopic 3D surface measurement. An innovative optical configuration employs a digital micromirror device (DMD) and a multispectral sensor is used to realize chromatic confocal microscopy with full-field area scanning. In the optical design, an area-scan type chromatic dispersive objective is specially designed to achieve measuring specification. Based on an 8x chromatic dispersive objective, the FOV for one shot measurement can be reached to 1.8mm*1.3mm which is immersive to microscopic profilometry. The spectral image captured by the multispectral sensor at each pinhole position has a unique spectrum pattern corresponding to its conjugate measured depth. A normalized cross-correlation (NCC) algorithm is developed to establish a spectrum-depth response curve with its corresponding spectrum pattern sets for accurate reconstruction of the tested 3D surface profile. With real test on standard targets, the measurement repeatability for a single surface depth is less than 0.6 micrometer.

physics.optics↗

arXiv2019

Quasi one-shot full-field surface profilometry using digital diffractive-confocal imaging correlation microscope

One-shot full-field surface profilometry using digital diffractive-confocal imaging correlation microscope based on digital micromirror device is developed for one-shot microscopic 3D surface measurement. Optical configuration applies confocal microscope setup and was building on DMD to generate specific pinhole array arrangement for minimizing cross talk effect. An innovative method was invented to create normalized cross correlation depth response curve from diffraction patterns of the pinhole. Using this approach, the sub-micrometer scale depth can be detected with high accuracy and precision.

physics.optics↗

arXiv2018

Plasmonic Metamaterial Perovskite Solar Cells: Fundamental Tradeoffs, Limitations, and Opportunities

Whether dispersal of plasmonic nanoparticles (NPs) within a perovskite active layer can increase the efficiency of solar cells is a long-standing question. It is well known that inclusion of metallic NPs in an active layer can boost the surrounding near-field intensity around them owing to the dipolar localized surface plasmon resonance (LSPR, also called antenna effect), which can increase light absorption by solar cells. However, the use of plasmonic NPs in perovskite solar cells has been barely reported, and it is not known whether inserting plasmonic NPs into a perovskite active layer produces any performance advantage compared with a pure perovskite counterpart. We explore the fundamental and practical limits of plasmonic metamaterial perovskite solar cells by applying effective medium theory and a detailed balance analysis. Our results indicate that an increase in effective refractive index of perovskite through dispersed plasmonic NPs can in principle enhance the performance of solar cells.

physics.app-ph↗

arXiv2018

Quick and repeatable shear modulus measurement based on torsional resonance and torsional wave propagation using a piezoelectric torsional transducer

Shear modulus is one of the fundamental mechanical properties of materials, while its quick and accurate measurement is still a challenge. Here we proposed two methods for shear modulus measurement based on torsional resonance and torsional wave propagation using a same piezoelectric torsional transducer. Firstly, the torsional transducer was introduced which consists of two thickness poled, thickness shear (d15) piezoelectric half-rings. Secondly, the equivalent circuit of the transducer-cylindrical specimen system is derived and the shear modulus can be explicitly obtained using the torsional resonance frequency. The internal friction can also be obtained, which is calculated by using an approximate formula. Then, the principle of shear modulus and internal friction measurement based on torsional wave propagation were presented. Finally, shear modulus and internal friction measurement on four materials including 1045 steel, aluminum, quartz glass and PMMA, were conducted. Results indicate that the measured shear moduli using these two methods are very close to each other, and consistent with the reference values in literatures. The resonance method is quite convenient and highly repeatable, but is typically not suitable for long specimens where the first torsional resonance may not be visible. The wave propagation method is especially suitable for long specimens and high frequency measurement is suggested. The internal frictions measured by these two methods were also close to each other, and the simple wave attenuation method is suggested. The two shear modulus measurement methods proposed in this work are quite reliable and can be widely used in near future.

physics.app-ph↗

arXiv2018

Surface Thermal Gradients Activated by Enhanced Molecular Absorption in Mid-infrared Vertical Antenna Arrays

We investigate local heat generation by molecules at the apex of polymer-embedded vertical antennas excited at resonant mid-infrared wavelengths, exploiting the surface enhanced infrared absorption (SEIRA) effect. The embedding of vertical nanoantennas in a non-absorbing polymer creates thermal isolation between the apical hotspot, the locus of heat generation, and the heat sink represented by the substrate. Vibrational mid-infrared absorption by strongly absorbing molecules located at the antenna apex then generates nanoscale temperature gradients at the surface. We imaged the thermal gradients by using a nano-photothermal expansion microscope, and we found values up to 10 K/microm in conditions where the radiation wavelength resonates with both the molecule vibrations and the plasmonic mode of the antennas. Values up to 1000 K/microm can be foreseen at maximum quantum cascade laser power. The presented system provides a promising thermoplasmonic platform for antenna-assisted thermophoresis and resonant mid-infrared photocatalysis.

physics.app-ph↗

arXiv2018

A Worldwide Cost-based Design and Optimization of Tilted Bifacial Solar Farms

The steady decrease in the levelized cost of solar energy (LCOE) has made it increasingly cost-competitive against fossil fuels. The cost reduction is supported by a combination of material, device, and system innovations. To this end, bifacial solar farms are expected to decrease LCOE further by increasing the energy yield; but given the rapid pace of design/manufacturing innovations, a cost-inclusive optimization of bifacial solar farms has not been reported. In our worldwide study, we use a fundamentally new approach to decouple energy yield from cost considerations by parameterizing the LCOE formula in terms of "land-cost" and "module cost" to show that an interplay of these parameters defines the optimum design of bifacial farms. For ground-mounted solar panels, we observe that the panels must be oriented horizontally and packed densely for locations with high "land-cost", whereas the panels should be optimally tilted for places with high "module-cost". Compared to a monofacial farm, the modules in an optimized bifacial farm must be tilted ~15-20 degrees higher and will reduce LCOE by ~8-10% in many locations of the world. The results in this paper will guide the deployment of LCOE-minimized ground-mounted tilted bifacial farms around the world.

physics.app-ph↗

arXiv2018

Integrated all-optical manipulation of orbital angular momentum carrying modes via enhanced electro-optic Kerr effect

Mode Division Multiplexing (MDM) technique using higher order Orbital Angular Momentum (OAM) carrying modes through a channelized bandwidth provides enhanced capacity communication systems. OAM based high-dimensional Quantum Key Distribution (QKD) encrypted channels also improve transmission rate and security. All-optical mode-selective spatial distribution manipulation is a significant function in implemented MDM and QKD networks. This paper proposes a novel versatile-designed integrated optical device with Y$_{cut}$ ridge Periodically Poled Lithium Niobate (PPLN) photonic wire configuration which acts as spatial mode converter for data modulated on higher order OAM$=\pm2\hbar$ modes. It is schemed in such a way that control the phase of decomposed guided modes by enhanced electro-optic Kerr effect via phase-mismatched cascaded polarization coupling interaction in PPLN sections. The low-loss, high-purity (91 %), and low-voltage proposed device enables to operate compatible with applicable commercial modulators in OAM based MDM and QKD communication systems.

physics.app-ph↗

arXiv2018

Generalized Parity-Time Symmetry Condition for Enhanced Sensor Telemetry

Wireless sensors based on micro-machined tunable resonators are important in a variety of applications, ranging from medical diagnosis to industrial and environmental monitoring.The sensitivity of these devices is, however, often limited by their low quality (Q) factor.Here, we introduce the concept of isospectral party time reciprocal scaling (PTX) symmetry and show that it can be used to build a new family of radiofrequency wireless microsensors exhibiting ultrasensitive responses and ultrahigh resolution, which are well beyond the limitations of conventional passive sensors. We show theoretically, and demonstrate experimentally using microelectromechanical based wireless pressure sensors, that PTXsymmetric electronic systems share the same eigenfrequencies as their parity time (PT)-symmetric counterparts, but crucially have different circuit profiles and eigenmodes. This simplifies the electronic circuit design and enables further enhancements to the extrinsic Q factor of the sensors.

physics.optics↗

arXiv2018

Critical Evaluation of Organic Thin-Film Transistor Models

Thin-film transistors (TFTs) represent a wide-spread tool to determine the charge-carrier mobility of materials. Mobilities and further transistor parameters like contact resistances are commonly extracted from the electrical characteristics. However, the trust in such extracted parameters is limited, because their values depend on the extraction technique and on the underlying transistor model. We propose a technique to establish whether a chosen model is adequate to represent the transistor operation. This two-step technique analyzes the electrical measurements of a series of TFTs with different channel lengths. The first step extracts the parameters for each individual transistor by fitting the full output and transfer characteristics to the transistor model. The second step checks whether the channel-length dependence of the extracted parameters is consistent with the model. We demonstrate the merit of the technique for distinct sets of organic TFTs that differ in the semiconductor, the contacts, and the geometry. Independent of the transistor set, our technique consistently reveals that state-of-the-art transistor models fail to reproduce the correct channel-length dependence. Our technique suggests that contemporary transistor models require improvements in terms of charge-carrier-density dependence of the mobility and/or the consideration of uncompensated charges in the transistor channel.

cond-mat.mes-hall↗