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arXiv2014

Proposed Entanglement of X-ray Nuclear Polaritons as a Potential Method for Probing Matter at the Subatomic Scale

A setup for generating the special superposition of a simultaneously forward- and backward-propagating collective excitation in a nuclear sample is studied. We show that by actively manipulating the scattering channels of single x-ray quanta with the help of a normal incidence x-ray mirror, a nuclear polariton which propagates in two opposite directions can be generated. The two counterpropagating polariton branches are entangled by a single x-ray photon. The quantum nature of the nuclear excitation entanglement gives rise to a subangstrom-wavelength standing wave excitation pattern that can be used as a flexible tool to probe matter dynamically on the subatomic scale.

quant-ph↗

arXiv2014

Hyperfine structure in $^{229g}$Th$^{3+}$ as a probe of the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy

We identify a potential means to extract the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy from precision microwave spectroscopy of the $5F_{5/2,7/2}$ hyperfine manifolds in the ion $^{229g}$Th$^{3+}$. The hyperfine interaction mixes this ground fine structure doublet with states of the nuclear isomer, introducing small but observable shifts to the hyperfine sub-levels. We demonstrate how accurate atomic structure calculations may be combined with measurement of the hyperfine intervals to quantify the effects of this mixing. Further knowledge of the magnetic dipole decay rate of the isomer, as recently reported, allows an indirect determination of the nuclear excitation energy.

physics.atom-ph↗

arXiv2013

Suppressing the loss of ultracold molecules via the continuous quantum Zeno effect

We investigate theoretically the suppression of two-body losses when the on-site loss rate is larger than all other energy scales in a lattice. This work quantitatively explains the recently observed suppression of chemical reactions between two rotational states of fermionic KRb molecules confined in one-dimensional tubes with a weak lattice along the tubes [Yan et al., Nature 501, 521-525 (2013)]. New loss rate measurements performed for different lattice parameters but under controlled initial conditions allow us to show that the loss suppression is a consequence of the combined effects of lattice confinement and the continuous quantum Zeno effect. A key finding, relevant for generic strongly reactive systems, is that while a single-band theory can qualitatively describe the data, a quantitative analysis must include multiband effects. Accounting for these effects reduces the inferred molecule filling fraction by a factor of five. A rate equation can describe much of the data, but to properly reproduce the loss dynamics with a fixed filling fraction for all lattice parameters we develop a mean-field model and benchmark it with numerically exact time-dependent density matrix renormalization group calculations.

quant-ph↗

arXiv2014

Dominant Secondary Nuclear Photoexcitation with the X-ray Free Electron Laser

The new regime of resonant nuclear photoexcitation rendered possible by x-ray free electron laser beams interacting with solid state targets is investigated theoretically. Our results unexpectedly show that secondary processes coupling nuclei to the atomic shell in the created cold high-density plasma can dominate direct photoexcitation. As an example we discuss the case of $^{93m}$Mo isomer depletion for which nuclear excitation by electron capture as secondary process is shown to be orders of magnitude more efficient than the direct laser-nucleus interaction. General arguments revisiting the role of the x-ray free electron laser in nuclear experiments involving solid-state targets are further deduced.

nucl-th↗

arXiv2014

Vortices associated with the wave function of a single electron emitted in slow ion-atom collisions

We present measurements and calculations of the momentum distribution of electrons emitted during the ion-atom collision 10 keV/u $He^{2+}+He \rightarrow He^{+} + He^{2+} + e^{-}$, which show rich structures for ion scattering angles above 2 mrad arising dominantly from two-electron states. Our calculations reveal that minima in the measured distributions are zeros in the electronic probability density resulting from vortices in the electronic current.

physics.atom-ph↗

arXiv2014

Local observation of pair-condensation in a Fermi gas at unitarity

We present measurements of the local (homogeneous) density-density response function of a Fermi gas at unitarity using spatially resolved Bragg spectroscopy. By analyzing the Bragg response across one axis of the cloud we extract the response function for a uniform gas which shows a clear signature of the Bose-Einstein condensation of pairs of fermions when the local temperature drops below the superfluid transition temperature. The method we use for local measurement generalizes a scheme for obtaining the local pressure in a harmonically trapped cloud from the line density and can be adapted to provide any homogeneous parameter satisfying the local density approximation.

cond-mat.quant-gas↗

arXiv2013

New limit on Lorentz and CPT violating neutron spin interactions using a free precession 3He-129Xe co-magnetometer

We report on the search for a CPT and Lorentz invariance violating coupling of the 3He and 129Xe nuclear spins (each largely determined by a valence neutron) to background tensor fields which permeate the universe. Our experimental approach is to measure the free precession of nuclear spin polarized 3He and 129Xe atoms in a homogeneous magnetic guiding field of about 400 nT using LTC SQUIDs as low-noise magnetic flux detectors. As the laboratory reference frame rotates with respect to distant stars, we look for a sidereal modulation of the Larmor frequencies of the co-located spin samples. As a result we obtain an upper limit on the equatorial component of the background field interacting with the spin of the bound neutron bn< 6.7*10^-34 GeV (68% C.L.). Our result improves our previous limit (data measured in 2009) by a factor of 30 and the world's best limit by a factor of 5.

gr-qc↗

arXiv2014

Decoherence-assisted spectroscopy of a single Mg$^+$ ion

We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly at rest are recorded efficiently with high signal-to-noise ratios. Spectra display symmetric line shapes without stray-light background from spectroscopy probes. We employ this method on a $^{25}$Mg$^+$ ion to measure one, two, and three-photon transition frequencies from the 3S ground state to the 3P, 3D, and 4P excited states, respectively. Our results are relevant for astrophysics and searches for drifts of fundamental constants. Furthermore, the method can be extended to other transitions, isotopes, and species. The currently achieved fractional frequency uncertainty of $5 \times 10^{-9}$ is not limited by the method.

physics.atom-ph↗

arXiv2014

Controlling magnetic Feshbach resonances in polar open-shell molecules with non-resonant light

Magnetically tunable Feshbach resonances for polar paramagnetic ground-state diatomics are too narrow to allow for magnetoassociation starting from trapped, ultracold atoms. We show that non-resonant light can be used to engineer the Feshbach resonances in their position and width. For non-resonant field strengths of the order of $10^9\,$W/cm$^2$, we find the width to be increased by three orders of magnitude, reaching a few Gauss. This opens the way for producing ultracold molecules with sizeable electric and magnetic dipole moments and thus for many-body quantum simulations with such particles.

physics.atom-ph↗

arXiv2013

Shifts of a resonance line in a dense atomic sample

We study the collective response of a dense atomic sample to light essentially exactly using classical-electrodynamics simulations. In a homogeneously broadened atomic sample there is no overt Lorentz-Lorenz local field shift of the resonance, nor a collective Lamb shift. However, addition of inhomogeneous broadening restores the usual mean-field phenomenology.

physics.atom-ph↗

arXiv2018

Long-term monitoring of the internal energy distribution of isolated cluster systems

A method is presented to monitor the internal energy distribution of cluster anions via delayed electron detachment by pulsed photoexcitation and demonstrated on Co$_4{}^-$ in an electrostatic ion beam trap. In cryogenic operation, we calibrate the detachment delay to internal energy. By laser frequency scans, at room temperature, we reconstruct the time-dependent internal energy distribution of the clusters. The mean energies of ensembles from a cold and a hot ion source both approach thermal equilibrium. Our data yield a radiative emission law and the absorptivity of the cluster for thermal radiation.

physics.atm-clus↗

arXiv2018

Experimental demonstration of shaken lattice interferometry

We experimentally demonstrate a shaken lattice interferometer. Atoms are trapped in the ground Bloch state of a red-detuned optical lattice. Using a closed-loop optimization protocol based on the dCRAB algorithm, we phase-modulate (shake) the lattice to transform the atom momentum state. In this way, we implement an atom beamsplitter and build five interferometers of varying interrogation times $T_I$. The sensitivity of shaken lattice interferometry is shown to scale as $T_I^2$, consistent with simulation [1]. Finally, we show that we can measure the sign of an applied signal and optimize the interferometer in the presence of a bias signal. [1] C. A. Weidner, H. Yu, R. Kosloff, and D. Z. Anderson, Phys. Rev. A 95, 043624 (2017).

quant-ph↗

arXiv2018

Dissociation energy of the hydrogen molecule at 10$^{-9}$ accuracy

The ionization energy of ortho-H$_2$ has been determined to be $E^\mathrm{o}_\mathrm{I}(\mathrm{H}_2)/(hc)=124\,357.238\,062(25)$ cm$^{-1}$ from measurements of the GK(1,1)--X(0,1) interval by Doppler-free two-photon spectroscopy using a narrow band 179-nm laser source and the ionization energy of the GK(1,1) state by continuous-wave near-infrared laser spectroscopy. $E^\mathrm{o}_\mathrm{I}$(H$_2$) was used to derive the dissociation energy of H$_2$, $D^{N=1}_{0}$(H$_2$), at $35\,999.582\,894(25)$ cm$^{-1}$ with a precision that is more than one order of magnitude better than all previous results. The new result challenges calculations of this quantity and represents a benchmark value for future relativistic and QED calculations of molecular energies.

physics.chem-ph↗

arXiv2017

Magnetically-Trapped Molecules Efficiently Loaded from a Molecular MOT

We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$ $μ$K. Next, we optically pump the molecules into a strongly-trapped sublevel. This two-step process reliably transfers $64\%$ of the molecules initially trapped in the MOT into the magnetic trap, comparable to similar atomic experiments. Once loaded, the magnetic trap is compressed by increasing the magnetic field gradient. Finally, we demonstrate a magnetic trap lifetime of over $1$ s. This opens a promising new path to the study of ultracold molecular collisions, and potentially the production of quantum-degenerate molecular gases.

physics.atom-ph↗

arXiv2018

Nuclear-spin comagnetometer based on a liquid of identical molecules

Atomic comagnetometers are used in searches for anomalous spin-dependent interactions. Magnetic field gradients are one of the major sources of systematic errors in such experiments. Here we describe a comagnetometer based on the nuclear spins within an ensemble of identical molecules. The dependence of the measured spin-precession frequency ratio on the first-order magnetic field gradient is suppressed by over an order of magnitude compared to a comagnetometer based on overlapping ensembles of different molecules. Our single-species comagnetometer is shown to be capable of measuring the hypothetical spin-dependent gravitational energy of nuclei at the $10^{-17}$ eV level, comparable to the most stringent existing constraints. Combined with techniques for enhancing the signal such as parahydrogen-induced polarization, this method of comagnetometry offers the potential to improve constraints on spin-gravity coupling of nucleons by several orders of magnitude.

physics.atom-ph↗

arXiv2018

Efimov Physics in Quenched Unitary Bose Gases

We study the impact of three-body physics in quenched unitary Bose gases, focusing on the role of the Efimov effect. Using a local density model, we solve the three-body problem and determine three-body decay rates at unitary, finding density-dependent, log-periodic Efimov oscillations, violating the expected continuous scale-invariance in the system. We find that the breakdown of continuous scale-invariance, due to Efimov physics, manifests also in the earliest stages of evolution after the interaction quench to unitarity, where we find the growth of a substantial population of Efimov states for densities in which the interparticle distance is comparable to the size of an Efimov state. This agrees with the early-time dynamical growth of three-body correlations at unitarity [Colussi {\em et al}., Phys. Rev. Lett. 120, 100401 (2018)]. By varying the sweep rate away from unitarity, we also find a departure from the usual Landau-Zener analysis for state transfer when the system is allowed to evolve at unitarity and develop correlations.

physics.atom-ph↗

arXiv2021

Fast Preparation and Detection of a Rydberg Qubit using Atomic Ensembles

We demonstrate a new approach for fast preparation, manipulation, and collective readout of an atomic Rydberg-state qubit. By making use of Rydberg blockade inside a small atomic ensemble, we prepare a single qubit within 3~$μ$s with a success probability of $F_p=0.93 \pm 0.02$, rotate it, and read out its state in $6$ $μs$ with a single-shot fidelity of $F_d=0.92 \pm 0.04$. The ensemble-assisted detection is $10^3$ times faster than imaging of a single atom with the same optical resolution, and enables fast repeated non-destructive measurement. We observe qubit coherence times of 15~$μ$s, much longer than the $π$ rotation time of 90~ns. Potential applications ranging from faster quantum information processing in atom arrays to efficient implementation of quantum error correction are discussed.

quant-ph↗

arXiv2021

Two-photon resonance fluorescence of two interacting non-identical quantum emitters

We study a system of two interacting, non-indentical quantum emitters driven by a coherent field. We focus on the particular condition of two-photon resonance and obtain analytical expressions for the stationary density matrix of the system and observables of the fluorescent emission. Importantly, our expressions are valid for the general situation of non-identical emitters with different transition energies. Our results allow us to determine the regime of parameters in which coherent two-photon excitation, enabled by the coherent coupling between emitters, is dominant over competing, first-order processes. Using the formalism of quantum parameter estimation, we show that the features imprinted by the two-photon dynamics into the spectrum of resonance fluorescence are particularly sensitive to changes in the distance between emitters, making two-photon excitation the optimal driving regime for the estimation of inter-emitter distance. This can be exploited for applications such as superresolution imaging of point-like sources.

quant-ph↗