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arXiv2008

Quasi-universal finite-$T$ scaling in gapped one-dimensional quantum magnets

Temperature dependencies of gap energies and magnon lifetimes are measured in the quasi-1-dimensional S=1/2 gapped quantum magnets IPA-CuCl3 and Sul-Cu2Cl4 using inelastic neutron scattering. The results are compared to those found in literature for S=1 Haldane spin chain materials and to theoretical calculations for the O(3)- and O(N)- quantum non-linear sigma-models. It is found that when the T=0 energy gap Delta is used as the temperature scale, all experimental and theoretical curves are identical to within system-dependent but temperature-independent scaling factors of the order of unity. This quasi-universality extends over a surprising broad T range, at least up to kappa T ~ 1.5 Delta.

cond-mat.str-el↗

arXiv2009

Observation of free hole gases at ambient conditions

By studying fluctuations in the electrostatic potential of a single electrode immersed in a cold plasma, we were able to perform in situ electron spectroscopy. Electron exchange processes that occur at the surface of the electrode were triggered by the surface Auger process either using metastable molecular nitrogen or triplet helium at ambient conditions. Ongoing redox reactions were decomposed into their two fundamental half reactions and the reduction and oxidation potentials were detected. We found that redox reactions near the electrode surface are the result of binary interactions of a free electron gas with a free hole gas that occur on a femtosecond time scale. The measured lifetimes of electron-hole recombination processes and the elastic scattering rate of the hole-hole process are in fair agreement with theoretical estimates. The observed asymmetry in the energy distributions of free electron and free hole ensembles suggests that at thermal equilibrium the identity of hole differs from that of an electron vacancy.

cond-mat.str-el↗

arXiv2008

Cooperative electron-phonon interaction in molecular chains

Using a controlled analytic treatment, we derive a model that generically describes cooperative strong electron-phonon interaction (EPI) in one-band and two-band Jahn-Teller (JT) systems. The model involves a {\em next-nearest-neighbor} hopping and a nearest-neighbor repulsion. Rings with odd number of sites (o-rings) belong to a different universality class compared to rings with even number (e-rings). The e-rings, upon tuning repulsion, undergo a dramatic discontinuous transition to a {\em conducting commensurate} charge density wave (CDW) state with a period independent of filling.

cond-mat.str-el↗

arXiv2009

Thermoelectric properties of LaRh$_{1-x}$Ni$_x$O$_3$

We report measurements and analyses of resistivity, thermopower, and thermal conductivity of polycrystalline samples of perovskite LaRh$_{1-x}$Ni$_x$O$_3$. The thermopower is found to be large at 800 K (185 $μ$V/K for $x=$0.3), which is ascribed to the high-temperature stability of the low-spin state of Rh$^{3+}$/Rh$^{4+}$ ions. This clearly contrasts with the thermopower of the isostructural oxide LaCoO$_3$, which rapidly decreases above 500 K owing to the spin-state transition. The spin state of the transition-metal ions is one of the most important parameters in oxide thermoelectrics.

cond-mat.str-el↗

arXiv2007

Dynamical Symmetry Breaking of a Relativistic Model in Quasi-(1+1)-Dimensions. I. Formulation

The dynamical symmetry breaking in a quasi-(1+1)-dimensional relativistic model is investigated. The motions of particles in intrachain are described as a relativistic electron-hole gas, while the interchain hopping term is introduced as a 0th-component of vector in (1+1)-dimensions, a kind of chemical potential of the system. The gauge symmetry of the model is chosen as U(1) suitable for a possible situation of a real substance in condensed matter physics. We consider the BCS-type contact interactions for the s-wave fermion-pair condensates, while employ the nonlocal interactions of the generalized BCS framework to generate the $p$-, $d$- and $f$-wave condensations in the system. Especially we examine the dynamical generation of a Dirac mass term and superconductivity in the model. The phenomenon is interpreted as metal-insulator/metal-superconductor phase transitions.

cond-mat.supr-con↗

arXiv2008

Large magnetocaloric effect in Gd4Co3

We report a large entropy change (DeltaS) below 300 K, peaking near TC= 220 K, due to isothermal change of magnetic field, for Gd4Co3, with a refrigeration capacity higher than that of Gd. Notably, the isothermal magnetization is nonhysteretic - an important criterion for magnetic refrigeration without loss. DeltaS behavior is also compared with that of magnetoresistance.

cond-mat.str-el↗

arXiv2007

Dissipation in finite systems: Semiconductor NEMS, graphene NEMS, and metallic nanoparticles

This thesis studies three kinds of mesoscopic systems and how one of their collective degrees of freedom is affected by a dissipative environment: a)Nanoelectromechanical systems based on semiconductor materials, and how surface friction processes limit the quality factor of their vibrational eigenmodes at low temperatures, causing as well a frequency shift; b)Graphene - based nanoresonators, and several damping mechanisms limiting the quality factor of its fundamental bending (flexural) eigenmode, and c)The dissipative dynamics of the surface plasmon created in a metallic nanocluster by a laser pulse, discussing the validity and limitations of a very common theoretical model used for its description.

cond-mat.mes-hall↗

arXiv2007

Resistivity of Inhomogeneous Superconducting Wires

We study the contribution of quantum phase fluctuations in the superconducting order parameter to the low--temperature resistivity $ρ(T)$ of a dirty and inhomogeneous superconducting wire. In particular, we account for random spatial fluctuations of arbitrary size in the wire thickness. For a typical wire thickness above the critical value for superconductor--insulator transition, phase--slips processes can be treated perturbatively. We use a memory formalism approach, which underlines the role played by weak violation of conservation laws in the mechanism for generating finite resistivity. Our calculations yield an expression for $ρ(T)$ which exhibits a smooth crossover from a homogeneous to a ``granular'' limit upon increase of $T$, controlled by a ``granularity parameter'' $D$ characterizing the size of thickness fluctuations. For extremely small $D$, we recover the power--law dependence $ρ(T)\sim T^α$ obtained by unbinding of quantum phase--slips. However in the strongly inhomogeneous limit, the exponent $α$ is modified and the prefactor is {\em exponentially enhanced}. We examine the dependence of the exponent $α$ on an external magnetic field applied parallel to the wire. Finally, we show that the power--law dependence at low $T$ is consistent with a series of experimental data obtained in a variety of long and narrow samples. The values of $α$ extracted from the data, and the corresponding field dependence, are consistent with known parameters of the corresponding samples.

cond-mat.supr-con↗

arXiv2008

The Bose-Fermi Kondo model with a singular dissipative spectrum: Exact solutions and their implications

Quantum dissipation induces a critical destruction of a Kondo screened state, which is of interest in the contexts of quantum critical heavy fermion metals and magnetic nanostructures. The sub-ohmic Bose-Fermi Kondo model provides a setting to study this effect. We find that this many-body problem is exactly solvable when the spectrum of the dissipative bosonic bath, J(ω), is singular, corresponding to J(τ)=const.. We determine the local spin correlation functions, showing that the singular LONGITUDINAL fluctuations of the bosonic bath dominate over the transverse ones. Our results provide evidence that the local quantum critical solution, derived within the extended dynamical mean field approach to the Kondo lattice model, has a zero residual entropy.

cond-mat.str-el↗

arXiv2008

Density of state and non-magnetic impurity effects in electron-doped cuprates

We analyze the density of state (DOS) and a non-magnetic impurity effect in electron-doped cuprates starting from two different scenarios: the $d_{x^{2}-y^{2}}$-wave superconductivity coexisting with antiferromagnetic spin density wave (SDW) order versus $d_{x^{2}-y^{2}}$-wave superconductivity with a higher harmonic. We find that in both cases the local density of state (LDOS) exhibits two impurity-induced resonance states at low energies. We also find that for the intermediate value of the SDW gap, the DOS looks similar to that obtained from the scenario of the $d_{x^{2}-y^{2}}$-wave gap with a higher harmonic, suggesting the presence of a non-monotonic $d_{x^{2}-y^{2}}$-wave gap. However, if the SDW gap is sufficiently large the DOS looks more conventional s-wave like. This obvious difference from the DOS resulted from the $d_{x^{2}-y^{2}}$-wave gap with a higher harmonic model, could differentiate the two above scenarios and is needed to be proved in the further doping dependence of tunneling spectrum measurement.

cond-mat.str-el↗

arXiv2008

Isospin excitations of a trapped 1D gas of attractively interacting fermions

We consider a gas of fermions with a short-range attractive intercomponent interaction in a parabolic external potential and derive the conditions of the local density approximation. The obtained spectrum of quasiparticle (isospin) excitations shows equidistant low-energy levels, which is equivalent to a linear momentum dependence and is fundamentally different from the ordinary Dirac spectrum in the spatially uniform case.

cond-mat.str-el↗

arXiv2007

Effects of electron-phonon coupling in angle-resolved photoemission spectra of SrTiO3

We have studied the O 2p valence-band structure of Nb-doped SrTiO3, in which a dilute concentration of electrons are doped into the d0 band insulator, by angle-resolved photoemission spectroscopy (ARPES) measurements. We found that ARPES spectra at the valence band maxima at the M [k = (pi/a, pi/a, 0)]and R [k = (pi/a, pi/a, pi/a)] points start from ~ 3.3 eV below the Fermi level (EF), consistent with the indirect band gap of 3.3 eV and the EF position at the bottom of the conduction band. The peak position of the ARPES spectra were, however, shifted toward higher binding energies by ~ 500 meV from the 3.3 eV threshold. Because the bands at M and R have pure O 2p character, we attribute this ~ 500 meV shift to strong coupling of the oxygen p hole with optical phonons in analogy with the peak shifts observed for d-electron photoemission spectra in various transition-metal oxides.

cond-mat.mtrl-sci↗

arXiv2008

Dynamical Mean Field Theory equations on nearly real frequency axis

The Iterated Perturbation Theory (IPT) equations of the Dynamical Mean Field Theory (DMFT) for the half-filled Hubbard model, are solved on nearly real frequencies at various values of the Hubbard parameters $U$, to investigate the nature of metal-insulator transition (MIT) at finite temperatures. This method avoids the instabilities associated with the infamous Padé analytic continuation and reveals fine structures across the MIT at finite temperatures, which {\em can not be captured} by conventional methods for solving DMFT equations on Matsubara frequencies. Our method suggests that at finite temperatures, there is an abrupt decrease in the height of the quasi-particle (Kondo) peak at a critical value of $U_c$, to a non-zero but small bump which gradually suppresses as one moves deeper into the {\em bad} insulator regime. In contrast to Vollhardt and coworkers [J. Phys. Soc. Jpn. {\bf 74} (2005) 136], down to $T=0.01$ of the half-bandwidth we find no $T^*$ separating bad insulator from a true Mott insulator.

cond-mat.str-el↗

arXiv2008

A vortex dynamics approach to the Nernst effect in fluctuating superconductors

We present a new method to study the Nernst effect and diamagetism of an extreme type-II superconductor dominated by phase fluctuations. We work directly with vortex variables and our method allows us to tune vortex parameters (e.g., core energy and number of vortex species). We find that diamagnetic response and transverse thermoelectric conductivity ($α_{xy}$) persist well above the Kosterlitz-Thouless transition temperature, and become more pronounced as the vortex core energy is increased. However, they \textit{weaken} as the number of internal vortex states are increased. We find that $α_{xy}$ closely tracks the magnetization $(-M/T)$ over a wide range of parameters.

cond-mat.supr-con↗

arXiv2008

Spin density-functional theory for imbalanced interacting Fermi gases in highly elongated harmonic traps

We numerically study imbalanced two component Fermi gases with attractive interactions in highly elongated harmonic traps. An accurate parametrization formula for the ground state energy is presented for a spin-polarized attractive Gaudin-Yang model. Our studies are based on an accurate microscopic spin-density-functional theory through the Kohn-Sham scheme which employs the one-dimensional homogeneous Gaudin-Yang model with Luther-Emery-liquid ground-state correlation as a reference system. A Thomas-Fermi approximation is examined incorporating the exchange-correlation interaction. By studying the charge and spin density profiles of the system based on these methods, we gain a quantitative understanding of the role of attractive interactions and polarization on the formation of the two-shell structure, with the coexisted Fulde-Ferrell-Larkin-Ovchinnikov-type phase in the center of the trap and either the BCS superfluid phase or the normal phase at the edges of the trap. Our results are in good agreement with the recent theoretical consequences.

cond-mat.str-el↗

arXiv2008

Comment on Magnetic Monopole Excitations in Spin Ice

It has been proposed recently \cite{son} that excitations in Spin Ice can be of the form of magnetic monopoles that does not obey the Dirac Quantization Condition. It is also well known \cite{rj} that the above scenario leads to non-associativity among translation generators. It will be interesting to see how the monopole picture in Spin Ice survives in the light of the latter observation.

cond-mat.str-el↗

arXiv2008

Influence of spin and interactions on quantum dots and nano-wires

In this dissertation we use sophisticated numerical methods in order to examine ground-state (GS) properties of two types of quantum systems with electron electron interactions: A quantum dot (QD) and a nano-wire. In the first half of the work we study a system of a single level coupled to a one-dimensional wire with interacting spinless electrons, when the wire is either clean or disordered. We utilize the density-matrix renormalization-group (DMRG) method to investigate the influence of the level on several thermodynamic properties of the clean interacting wire, which can be in one of two phases: Tomonaga-Luttinger liquid and charge density wave phases. When the wire is disordered, we investigate the Friedel oscillations, exploring the difference between the two phases and comparing them to the clean non-interacting case, for which we develop an exact formula for the oscillations. In the second half of the dissertation we study two cases of an isolated two-dimensional QD. We begin by an investigation of a new numerical method, the particle-hole DMRG (PH-DMRG), which is used to calculate the GS energy of a disordered QD consisting of interacting spinless electrons. We show that this method is much more accurate than the Hartree-Fock method, and we suggest an improvement of the algorithm, which reduces the error rate by almost 30 percents. Finally we study the magnetization of a QD with spin 1/2 electrons, in the presence of spin-orbit coupling and interactions. We calculate the g-factor and the expectation values of the spin operators in the GS, and find that when the QD is occupied by an even number of electrons, the GS can have a finite magnetization.

cond-mat.str-el↗

arXiv2008

Magneto-transport and Magneto-dielectric effect in Bi-based Perovskite Manganites

The effect of cobalt and nickel substitutions for manganese on the physical properties of the perovskite manganite La1.2Bi0.8Mn2-x(Ni/Co)xO6+d, with x = 0.0-0.8, has been investigated. It is observed that the ferromagnetism is enhanced, TC being increased from 103 K for the parent compound (x = 0.0) to 178 K for Ni-phase, and to 181 K for the Co-phase (x = 0.8). Moreover, the systems remain insulating and depict relatively large values of magnetoresistance effect at low temperatures (up to 67 % at 90K and 70 kOe, for x = 0.0 phase). These phenomena are interpreted by means of electronic phase separation, where the ferromagnetic Mn4+/Ni2+ and Mn4+/Co2+ interactions reinforce the Mn3+/Mn4+ interactions by super-exchange interaction. The dielectric measurements below the magnetic transition temperatures exhibit weak magneto-dielectric effect of around 0.25% at 80K, which may be due to spin-lattice interaction.

cond-mat.mtrl-sci↗