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arXiv2013

First-Principles Theory of Anharmonicity and the Inverse Isotope Effect in Superconducting Palladium-Hydride Compounds

Palladium hydrides display the largest isotope effect anomaly known in literature. Replacement of hydrogen with the heavier isotopes leads to higher superconducting temperatures, a behavior inconsistent with harmonic theory. Solving the self-consistent harmonic approximation by a stochastic approach, we obtain the anharmonic free energy, the thermal expansion and the superconducting properties fully ab initio. We find that the phonon spectra are strongly renormalized by anharmonicity far beyond the perturbative regime. Superconductivity is phonon mediated, but the harmonic approximation largely overestimates the superconducting critical temperatures. We explain the inverse isotope effect, obtaining a -0.38 value for the isotope coefficient in good agreement with experiments, hydrogen anharmonicity being the main responsible for the isotope anomaly.

cond-mat.supr-con↗

arXiv2018

Odd and even modes of neutron spin resonance in the bilayer iron-based superconductor CaKFe$_4$As$_4$

We report an inelastic neutron scattering study on the spin resonance in the bilayer iron-based superconductor CaKFe$_4$As$_4$. In contrast to its quasi-two-dimensional electron structure, three strongly $L$-dependent modes of spin resonance are found below $T_c=35$ K. The mode energies are below and linearly scale with the total superconducting gaps summed on the nesting hole and electron pockets, essentially in agreement with the results in cuprate and heavy fermion superconductors. This observation supports the sign-reversed Cooper pairing mechanism under multiple pairing channels and resolves the long-standing puzzles concerning the broadening and dispersive spin resonance peak in iron pnictides. More importantly, the triple resonant modes can be classified into odd and even symmetries with respect to the distance of Fe-Fe planes within the Fe-As bilayer unit. Thus, our results closely resemble those in the bilayer cuprates with nondegenerate spin excitations, suggesting that these two high-$T_c$ superconducting families share a common nature.

cond-mat.supr-con↗

arXiv2013

Muon spin rotation studies of niobium for superconducting RF applications

In this work we investigate superconducting properties of niobium samples via application of the muon spin rotation/relaxation (muSR) technique. We employ for the first time the muSR technique to study samples that are cutout from large and small grain 1.5 GHz radio frequency (RF) single cell niobium cavities. The RF test of these cavities was accompanied by full temperature mapping to characterize the RF losses in each of the samples. Results of the muSR measurements show that standard cavity surface treatments like mild baking and buffered chemical polishing (BCP) performed on the studied samples affect their surface pinning strength. We find an interesting correlation between high field RF losses and field dependence of the sample magnetic volume fraction measured via muSR. The muSR line width observed in ZF-muSR measurements matches the behavior of Nb samples doped with minute amounts of Ta or N impurities. An upper bound for the upper critical field Hc2 of these cutouts is found.

cond-mat.supr-con↗

arXiv2013

Origin of the two-dimensional electron gas at LaAlO3/SrTiO3 interfaces: The role of oxygen vacancies and electronic reconstruction

The relative importance of atomic defects and electron transfer in explaining conductivity at the crystalline LaAlO3/SrTiO3 interface has been a topic of debate. Metallic interfaces with similar electronic properties produced by amorphous oxide overlayers on SrTiO3 have called in question the original polarization catastrophe model. We resolve the issue by a comprehensive comparison of (100)-oriented SrTiO3 substrates with crystalline and amorphous overlayers of LaAlO3 of different thicknesses prepared under different oxygen pressures. For both types of overlayers, there is a critical thickness for the appearance of conductivity, but its value is always 4 unit cells (around 1.6 nm) for the oxygen-annealed crystalline case, whereas in the amorphous case, the critical thickness could be varied in the range 0.5 to 6 nm according to the deposition conditions. Subsequent ion milling of the overlayer restores the insulating state for the oxygen-annealed crystalline heterostructures but not for the amorphous ones. Oxygen post-annealing removes the oxygen vacancies, and the interfaces become insulating in the amorphous case. However, the interfaces with a crystalline overlayer remain conducting with reduced carrier density. These results demonstrate that oxygen vacancies are the dominant source of mobile carriers when the LaAlO3 overlayer is amorphous, while both oxygen vacancies and polarization catastrophe contribute to the interface conductivity in unannealed crystalline LaAlO3/SrTiO3 heterostructures, and the polarization catastrophe alone accounts for the conductivity in oxygen-annealed crystalline LaAlO3/SrTiO3 heterostructures. Furthermore, we find that the crystallinity of the LaAlO3 layer is crucial for the polarization catastrophe mechanism in the case of crystalline LaAlO3 overlayers.

cond-mat.mtrl-sci↗

arXiv2013

Correlation-enhanced electron-phonon coupling: Applications of GW and screened hybrid functional to bismuthates, chloronitrides, and other high Tc superconductors

We show that the electron-phonon coupling (EPC) in many materials can be significantly underestimated by the standard density functional theory (DFT) in the local density approximation (LDA) due to large non-local correlation effects. We present a simple yet efficient methodology to evaluate the realistic EPC going beyond LDA by using more advanced and accurate GW and screened hybrid functional DFT approaches. The corrections we propose explain the extraordinarily high superconducting temperatures that are observed in two distinct classes of compounds-the bismuthates and the transition metal chloronitrides, thus solving a thirty-year-old puzzle. Our work calls for the critically reevaluation of the EPC of certain phonon modes in many other materials such as cuprates and iron-based superconductors. The proposed methodology can be used to design new correlation-enhanced high temperature superconductors and other functional materials involving electron-phonon interaction.

cond-mat.supr-con↗

arXiv2013

Tunable coupling to a mechanical oscillator circuit using a coherent feedback network

We demonstrate a fully cryogenic microwave feedback network composed of modular superconducting devices connected by transmission lines and designed to control a mechanical oscillator coupled to one of the devices. The network features an electromechanical device and a tunable controller that coherently receives, processes and feeds back continuous microwave signals that modify the dynamics and readout of the mechanical state. While previous electromechanical systems represent some compromise between efficient control and efficient readout of the mechanical state, as set by the electromagnetic decay rate, the tunable controller produces a closed-loop network that can be dynamically and continuously tuned between both extremes much faster than the mechanical response time. We demonstrate that the microwave decay rate may be modulated by at least a factor of 10 at a rate greater than $10^4$ times the mechanical response rate. The system is easy to build and suggests that some useful functions may arise most naturally at the network-level of modular, quantum electromagnetic devices.

cond-mat.supr-con↗

arXiv2013

Gate defined wires in HgTe quantum wells: from Majorana fermions to spintronics

We introduce a promising new platform for Majorana zero-modes and various spintronics applications based on gate-defined wires in HgTe quantum wells. Due to the Dirac-like band structure for HgTe the physics of such systems differs markedly from that of conventional quantum wires. Most strikingly, we show that the subband parameters for gate-defined HgTe wires exhibit exquisite tunability: modest gate voltage variation allows one to modulate the Rashba spin-orbit energies from zero up to ~30K, and the effective g-factors from zero up to giant values exceeding 600. The large achievable spin-orbit coupling and g-factors together allow one to access Majorana modes in this setting at exceptionally low magnetic fields while maintaining robustness against disorder. As an additional benefit, gate-defined wires (in HgTe or other settings) should greatly facilitate the fabrication of networks for refined transport experiments used to detect Majoranas, as well as the realization of non-Abelian statistics and quantum information devices.

cond-mat.mes-hall↗

arXiv2002

Influence of the Preparation Process on Microstructure, Critical Current Density and Tc of MgB2 Powder-In-Tube Wires

MgB2 wires and tapes suffer from a limitation of the transport current densities, especially at low field, due to an unsufficient thermal stabilization caused by hot spots from a non-homogeneous microstructure, the presence of secondary phases and voids. For the preparation of MgB2 wires and tapes two different precursor routes, using MgB2 (ex-situ process) or Mg + B (in-situ process) are applied. The in-situ approach allows variation of many parameters in the wire preparation and the improvement of this approach is the central topic of this paper. We present an improved in-situ approach, the characterization of the filament microstructure, effects from stoichiometry and the corresponding superconducting properties. The transport current capability of such in-situ wires could be improved to the level of the reference ex-situ wires.

cond-mat.supr-con↗

arXiv2002

Tunnel junctions on as-grown superconducting MgB2 thin films

We demonstrate that good superconductor/insulator/normal-metal tunnel junctions can be fabricated on as-grown superconducting MgB2 thin films. The as-grown films were prepared by coevaporation at low growth temperatures of around 280deg. The insulating barrier was formed by an Mg overlayer, which is subsequently oxidized in air. The tunneling spectra for Au/MgOx/MgB2 junctions showed a reproducible and well-defined superconducting gap (delta= ~ 2.5 meV). The resultant 2delta/ kBTc was significantly smaller than the predicted BCS value of 3.52.

cond-mat.supr-con↗

arXiv2002

Mechanical properties of reinforced MgB2 wires

For technical application in windings of coils, transformers or motors, a reinforcement of MgB2 wires and tapes is necessary to withstand applied stresses and strains and to avoid cracks in the filaments. Therefore, the response of the superconducting transport currents on applied axial strain in different magnetic background fields was investigated for differently stainless steel reinforced MgB2 wires, by means of an axial strain rig. Increased amounts of stainless steel in the sheath caused a stronger decrease of the critical currents in fields above 3 T as a consequence of a changed irreversibility field. Heat treated wires have a quite different mechanical behaviour compared to as-cold-worked wires, but an about 10 times higher transport current level. Tape geometries, having generally higher current carrying capabilities than wires, showed much poorer mechanical properties with a less effective filament precompression from the matrix.

cond-mat.supr-con↗

arXiv2003

AC losses in type-II superconductors induced by nonuniform fluctuations of external magnetic field

Magnetic field fluctuations are inevitable in practical applications of superconductors and it is often necessary to estimate the AC losses these fluctuations induce. If the fluctuation wavelength is greater than the size of a superconductor, known estimates for an alternating uniform external magnetic field can be employed. Here we consider the opposite case and analyze, using a model critical-state problem, penetration of spatially nonuniform fluctuations into type-II superconductors. Numerical simulation is based on a variational formulation of the Bean model. The analytical solutions, found in a weak penetration limit, are used to evaluate AC losses for two types of fluctuations: the running and standing waves. It is shown that for spatially nonuniform fluctuations the losses are better characterized by the fluctuation penetration depth than by the fluctuation amplitude. The results can be used to estimate the AC losses in flywheels, electric motors, magnetic shields, etc.

cond-mat.supr-con↗

arXiv2004

Upper Critical Fields up to 60T in Dirty Magnesium Diboride Thin Films

Upper critical fields of several magnesium diboride thin films were measured up to 28 T at the Grenoble High Magnetic Field Laboratory (GHMFL) in Grenoble and up to 60 T at the Laboratoire National des Champs Magnetiques Pulses (LNCMP) in Toulouse. The samples were prepared both by pulsed laser deposition (PLD) and hybrid physical chemical vapour deposition (HPCVD) technique; they have critical temperatures between 29 and 39 K and normal state resistivities between 5 and 250 μohmcm; one of them has been intentionally doped with carbon. The measured critical fields were exceptionally high; we obtained the record value of 52 T at 4.2 K in the parallel orientation. In contrast with the BCS predictions, no saturation in Hc2 at low temperature was observed. Furthermore, films with a wide range of resistivity values showed similar critical fields, suggesting that in a two band system resistivity and Hc2 are not trivially linked. The high Hc2 values seem to be related with the expanded c-axis. The structure of one of the samples was carefully investigated with X-ray diffraction at European Synchrotron Radiation Facility (ESRF) in Grenoble.

cond-mat.supr-con↗

arXiv2012

AC Losses of Copper Stabilized Multifilament YBCO Coated Conductors

We report the data on magnetization losses and critical current of multifilament copper stabilized coated conductors. Eight centimeters long samples of copper stabilized YBa2Cu3O7-x (YBCO) coated conductors manufactured commercially were subdivided into superconducting filaments by near-IR laser micromachining. The width of the superconducting stripes was varied from 0.2 mm to 0.04 mm. Some of the samples were striated leaving superconducting bridges for current sharing between the filaments. The AC losses were measured at different sweep rates of the magnetic field up to 14 T/s. We will present the results for the hysteresis and coupling losses and discuss the means to reduce the coupling loss by changing the processing parameters of micromachining and by post-ablation treatment.

cond-mat.supr-con↗

arXiv2012

Highly responsive Y-Ba-Cu-O thin film THz detectors with picosecond time resolution

High-temperature superconducting YBa2Cu3O7-d (YBCO) thin-film detectors with improved responsivities were developed for fast time-domain measurements in the THz frequency range. YBCO thin films of 30 nm thickness were patterned to micro- and nanobridges and embedded into planar log-spiral THz antennas. The YBCO thin-film detectors were characterized with continuous wave radiation at 0.65 THz. Responsivity values as high as 710 V/W were found for the YBCO nanobridges. Pulsed measurements in the THz frequency range were performed at the electron storage ring ANKA from the Karlsruhe Institute of Technology (KIT). Due to the high responsivities of the nanobridges no biasing was required for the detection of the coherent synchrotron radiation pulses achieving very good agreement between the measured pulse shapes and simulations.

cond-mat.supr-con↗

arXiv2012

MOD derived pyrochlore films as buffer layer for all-chemical YBCO coated conductors

We report a detailed study performed on La2Zr2O7 (LZO) pyrochlore material grown by Metal-Organic Decomposition (MOD) method as buffer layers for YBa2Cu3O7-x (YBCO) coated conductors. High quality epitaxial LZO thin films have been obtained on single crystal (SC) and Ni-5%at.W substrates. In order to evaluate structural and morphological properties, films have been characterized by means of X-ray diffraction analyses (XRD), atomic force microscope (AFM) and scanning electron microscope (SEM). Precursors solutions and heat treatments have been studied by thermogravimetric analyses (TG-DTA-DTG) and infrared spectra (FT-IR) with the aim of optimizing the annealing process. Thin films of YBCO have been deposited by pulsed laser ablation (PLD) on this buffer layers. The best results obtained on SC showed YBCO films with critical temperature values above 90 K, high self field critical current density values (Jc > 1 MA/cm2) and high irreversibility field values (8.3 T) at 77 K together with a rather high depinning frequency vp (0.5 T, 77 K)>44 GHz as determined at microwaves. The best results on Ni-5%at.W has been obtained introducing in the heat treatment a pyrolysis process at low temperature in air in order to remove the residual organic part of the precursor solution.

cond-mat.supr-con↗

arXiv2013

Development of 2D Bi-SQUID Arrays with High Linearity

We develop a two-dimensional (2D) Superconducting Quantum Interference Filter (SQIF) array based on recently introduced high-linearity tri-junction bi-SQUIDs. Our bi-SQUID SQIF array design is based on a tight integration of individual bi- SQUID cells sharing inductances with adjacent cells. We provide extensive computer simulations, analysis and experimental measurements, in which we explore the phase dynamics and linearity of the array voltage response. The non-uniformity in inductances of the bi-SQUIDs produces a pronounced zero-field single antipeak in the voltage response. The anti-peak linearity and size can be optimized by varying the critical current of the additional junction of each bi-SQUID. The layout implementation of the tight 2D array integration leads to a distinct geometrical diamond shape formed by the merged dual bi-SQUID cells. Different size 2D arrays are fabricated using standard HYPRES niobium 4.5 kA/cm2 fabrication process. The measured linearity, power gain, and noise properties will be analyzed for different array sizes and the results will be compared with circuit simulations. We will discuss a design approach for the electrically small magnetic field antenna and low-noise amplifiers with high bandwidth based on these 2D bi-SQUID SQIF arrays. The results from this work will be used to design chips densely and completely covered in bi-SQUIDs that has optimized parameters such as linearity and power gain.

physics.ins-det↗

arXiv2013

Computation of Losses in HTS Under the Action of Varying Magnetic Fields and Currents

Numerical modeling of superconductors is widely recognized as a powerful tool for interpreting experimental results, understanding physical mechanisms and predicting the performance of high-temperature superconductor (HTS) tapes, wires and devices. This is especially true for ac loss calculation, since a sufficiently low ac loss value is imperative to make these materials attractive for commercialization. In recent years, a large variety of numerical models, based on different techniques and implementations, have been proposed by researchers around the world, with the purpose of being able to estimate ac losses in HTSs quickly and accurately. This article presents a literature review of the methods for computing ac losses in HTS tapes, wires and devices. Technical superconductors have a relatively complex geometry (filaments, which might be twisted or transposed, or layers) and consist of different materials. As a result, different loss contributions exist. In this paper, we describe the ways of computing such loss contributions, which include hysteresis losses, eddy current losses, coupling losses, and losses in ferromagnetic materials. We also provide an estimation of the losses occurring in a variety of power applications.

cond-mat.supr-con↗

arXiv2015

Optimization of the Superconducting Linear Magnetic Bearing of a Maglev Vehicle

Considering the need for cost/performance prediction and optimization of superconducting maglev vehicles, we develop and validate here a 3D finite element model to simulate superconducting linear magnetic bearings. Then we reduce the 3D model to a 2D model in order to decrease the computing time. This allows us to perform in a reasonable time a stochastic optimization considering the superconductor properties and the vehicle operation. We look for the permanent magnet guideway geometry that minimizes the cost and maximizes the lateral force during a displacement sequence, with a constraint on the minimum levitation force. The displacement sequence reproduces a regular maglev vehicle operation with both vertical and lateral movements. For the sake of comparison, our reference is the SupraTrans prototype bearing. The results of the optimization suggest that the bearing cost could be substantially reduced, while keeping the same performances as the initial design. Alternatively, the performances could be significantly improved for the same original cost.

cond-mat.supr-con↗