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On-chip broadband plasmon-induced transparency based on plasmonic metal-insulator-metal waveguides

As an analogue of electromagnetically induced transparency (EIT), plasmon-induced transparency (PIT) has been realized both in plasmonic metamaterial and waveguide structures. Via near-field coupling within unit cells, PIT with broadband could be produced by plasmonic metamaterials, which, however, has not been realized in on-chip plasmonic waveguide structures. Here, we introduce broadband PIT based on a plasmonic metal-insulator-metal (MIM) waveguide system. Utilizing the direct coupling structure, PIT emerges based on an easy-fabricated structure without gap. By tuning coupling distance, the transparent window can be continuously tuned from narrow- to broadband. Such device is promising for on-chip applications on sensing, filtering and slow light over a broad frequency range.

physics.optics↗

Recent Progress and Future Prospects of 2D-based Photodetectors

Conventional semiconductors such as silicon and InGaAs based photodetectors have encountered a bottleneck in modern electronics and photonics in terms of spectral coverage, low resolution, non-transparency, non-flexibility and CMOS-incompatibility. New emerging 2D materials such as graphene, TMDs and their hybrid systems thereof, however, can circumvent all these issues benefitting from mechanically flexibility, extraordinary electronic and optical properties, as well as wafer-scale production and integration. Heterojunction-based photodiodes based on 2D materials offer ultrafast and broadband response from visible to far infrared range. Phototransistors based on 2D hybrid systems combined with other material platforms such as quantum dots, perovskites, organic materials, or plasmonic nanostructures yield ultrasensitive and broadband light detection capabilities. Notably the facile integration of 2D-photodetectors on silicon photonics or CMOS platforms paves the way towards high performance, low-cost, broadband sensing and imaging modalities.

physics.app-ph↗

Ultrasensitive all-optical thermometry using nanodiamonds with high concentration of silicon-vacancy centres and multiparametric data analysis

Nanoscale thermometry is paramount to study primary processes of heat transfer in solids and is a subject of hot debate in cell biology. Here we report ultrafast temperature sensing using all-optical thermometry exploiting synthetic nanodiamonds with silicon-vacancy (SiV) centres embedded at a high concentration. Using multi-parametric analysis of photoluminescence (PL) of these centres, we have achieved an intrinsic noise floor of about 10 mK Hz$^{-1/2}$, which is a thousand-fold increase in the readout speed in comparison to the current record values demonstrated with all-optical methods of comparable spatial-resolution and precision. Our thermometers are smaller than 250-nm across but can detect a 0.4$^\circ$C change of temperature in a measurement taking only 0.001 second. The exceptional sensitivity and simplicity of these thermometers enable a wide range of applications such as temperature monitoring and mapping within intracellular regions and in state-of-the-art solid-state electronic nanodevices.

physics.app-ph↗

Measurement of 3D bubble distribution using digital inline holography

The paper presents a hybrid bubble hologram processing approach for measuring the size and 3D distribution of bubbles over a wide range of size and shape. The proposed method consists of five major steps, including image enhancement, digital reconstruction, small bubble segmentation, large bubble/cluster segmentation, and post-processing. Two different segmentation approaches are proposed to extract the size and the location of bubbles in different size ranges from the 3D reconstructed optical field. Specifically, a small bubble is segmented based on the presence of the prominent intensity minimum in its longitudinal intensity profile, and its depth is determined by the location of the minimum. In contrast, a large bubble/cluster is segmented using a modified watershed segmentation algorithm and its depth is measured through a wavelet-based focus metric. Our processing approach also determines the inclination angle of a large bubble with respect to the hologram recording plane based on the depth variation along its edge on the plane. The accuracy of our processing approach on the measurements of bubble size, location and inclination is assessed using the synthetic bubble holograms and a 3D printed physical target. The holographic measurement technique is further implemented to capture the fluctuation of instantaneous gas leakage rate from a ventilated supercavity generated in a water tunnel experiment. Overall, our paper introduces a low cost, compact and high-resolution bubble measurement technique that can be used for characterizing low void fraction bubbly flow in a broad range of applications.

physics.app-ph↗

An integrated cryogenic optical modulator

Integrated electrical and photonic circuits (PIC) operating at cryogenic temperatures are fundamental building blocks required to achieve scalable quantum computing, and cryogenic computing technologies. Optical interconnects offer better performance and thermal insulation than electrical wires and are imperative for true quantum communication. Silicon PICs have matured for room temperature applications but their cryogenic performance is limited by the absence of efficient low temperature electro-optic (EO) modulation. While detectors and lasers perform better at low temperature, cryogenic optical switching remains an unsolved challenge. Here we demonstrate EO switching and modulation from room temperature down to 4 K by using the Pockels effect in integrated barium titanate (BaTiO3)-based devices. We report the nonlinear optical (NLO) properties of BaTiO3 in a temperature range which has previously not been explored, showing an effective Pockels coefficient of 200 pm/V at 4 K. We demonstrate the largest EO bandwidth (30 GHz) of any cryogenic switch to date, ultra-low-power tuning which is 10^9 times more efficient than thermal tuning, and high-speed data modulation at 20 Gbps. Our results demonstrate a missing component for cryogenic PICs. It removes major roadblocks for the realisation of novel cryogenic-compatible systems in the field of quantum computing and supercomputing, and for interfacing those systems with the real world at room-temperature.

physics.app-ph↗

Design for a 10 KeV Multi-Pass Transmission Electron Microscope

Multi-pass transmission electron microscopy (MPTEM) has been proposed as a way to reduce damage to radiation-sensitive materials. For the field of cryo-electron microscopy (cryo-EM), this would significantly reduce the number of projections needed to create a 3D model and would allow the imaging of lower-contrast, more heterogeneous samples. We have designed a 10 keV proof-of-concept MPTEM. The column features fast-switching gated electron mirrors which cause each electron to interrogate the sample multiple times. A linear approximation for the multi-pass contrast transfer function (CTF) is developed to explain how the resolution depends on the number of passes through the sample.

physics.app-ph↗

Gold/Parylene-C/Pentacene Capacitor under Constant-Voltage Stress

Degradation of metal-insulator-semiconductor (MIS) capacitors of gold/Parylene-C/Pentacene under constant voltage stress (CVS) was investigated to explore the electrical stability and reliability of Parylene C as a gate dielectric in flexible electronics. A stress voltage of fixed magnitude as high as 20 V, both negative and positive in polarity, was applied to each MIS capacitor at room temperature for a fixed duration as long as 10 s. The CVS effects on the capacitance-voltage curve-shift, the time-dependent leakage current, and the time-dependent dielectric breakdown were measured and analyzed. CVS is observed to induce charge in Parylene-C and its interfaces with gold and Pentacene. The net induced charge is positive and negative for, respectively, negative and positive gate bias polarity during CVS. The magnitude of the charge accumulated following positive gate CVS is significantly higher than that following negative gate bias CVS in the range of 4 to 25 nC cm$^{-2}$. In contrast, the leakage current during the negative gate stress is three orders of magnitude higher than that during the positive gate stress for the same bias stress magnitude. The charge buildup and leakage current are due to the trapping of electrons and holes near the Parylene-C/Pentacene interface as well as in the Parylene-C layer. Before the application of the CVS, a dielectric breakdown occurs at an electric field of 1.62 MV cm$^{-1}$. After the application of the CVS, the breakdown voltage decreases and the density of the trapped charges increases as the stress voltage increases in magnitude, with the polarity of the trapped charges opposite to that of the stress voltage. The magnitude and direction of the capacitance-voltage curve-shift depend on the trapping and recombination of electrons and holes in the Parylene-C layer and in the proximity of the Parylene-C/Pentacene interface during CVS.

physics.app-ph↗

Tailoring superhydrophobic ZnO nanorods on Si pyramids with enhanced visible range antireflection property

Simultaneous superhydrophobic and visible range antireflective properties are demonstrated in hydrothermally grown ZnO nanorods on chemically textured Si surfaces. A drastic transformation of Si micro pyramids from hydrophobic to superhydrophobic is observed by securing the formation of polycrystalline ZnO nanorods at surfaces, showing an increment of apparent contact angle from 102 degree to 157 degree and further explained in the light of a decrease in solid fractional surface area, according to the Cassie Baxter model. Moreover, wurtzite phase of ZnO NRs is confirmed by the X ray diffraction and Raman analysis. Such hierarchical structures further exhibit a large visible range antireflection, 5 percentage, and correlated it to the variation in aspect ratio of Si pyramids in conjunction with the formation of graded refractive index. The combined superhydrophobic and large antireflection phenomenon in the present dual scale structures is believed to be useful for Si based photovoltaic applications.

physics.app-ph↗

Effect of Ion Migration Induced Electrode Degradation on the Operational Stability of Perovskite Solar Cells

Perovskite-based solar cells are promising due to their rapidly improving efficiencies, but suffer from instability issues. Recently it has been claimed that one of the key contributors to the instability of perovskite solar cells is ion migration induced electrode degradation, which can be avoided by incorporating inorganic hole blocking layers (HBL) in the device architecture. In this work, we investigate the operational environmental stability of methylammonium lead iodide (MAPbI3) perovskite solar cells that contain either an inorganic or organic HBL, with only the former effectively blocking ions from migrating to the metal electrode. This is confirmed by X-ray photoemission spectroscopy measured on electrodes of degraded devices, where only electrodes of devices with an organic HBL show a significant iodine signal. Despite this, we show that when these devices are degraded under realistic operational conditions (i.e. constant illumination in a variety of atmospheric conditions), both types of devices exhibit nearly identical degradation behavior. These results demonstrate that contrary to prior suggestions, ion-induced electrode degradation is not the dominant factor in perovskite environmental instability under operational conditions.

physics.app-ph↗

Quantifying the Damage Induced by XPS Depth Profiling of Organic Conjugated Polymers

X-ray photoemission spectroscopy (XPS) depth profiling using monoatomic Ar+ ion etching sources is a common technique that allows for the probing of the vertical compositional profiles of a wide range of materials. In polymer-based organic photovoltaic devices, it is commonly used to study compositional variations across the interfaces of the organic active layer with charge extraction layers or electrodes, as well as the vertical phase separation within the bulk-heterojunction active layer. It is generally considered that the damage induced by the etching of organic layers is limited to the very top surface, such that the XPS signal (acquired from the top ~10 nm of the layer) remains largely unaffected, allowing for a reliable measurement of the sample composition throughout the depth profile. Herein, we investigate a range of conjugated polymers and quantify the depth of the damage induced by monoatomic etching for Ar+ ion energies ranging from 0.5 keV to 4 keV using argon gas cluster ion beam depth profiling. The results demonstrate that even when etching with the lowest available monoatomic ion energy for as little as 3 s, the damaged polymer material extends deeper into the bulk than the XPS probing depth. We show that the damaged material distorts the compositional information obtained by XPS, resulting in erroneous depth profiles. Furthermore, we propose that only gas cluster ion beam etching sources should be used for depth profiling of organic conjugated polymers, as those induce significantly less damage and maintain the compositional information throughout the entire profile.

physics.app-ph↗

Fractional Deviations in Precursor Stoichiometry Dictate the Properties, Performance and Stability of Perovskite Photovoltaic Devices

The last five years have witnessed a remarkable progress in the field of lead halide perovskite materials and devices. Examining the existing body of literature reveals staggering inconsistencies in the reported results among different research groups with a particularly wide spread in the photovoltaic performance and stability of devices. In this work we demonstrate that fractional, quite possibly unintentional, deviations in the precursor solution stoichiometry can cause significant changes in the properties of the perovskite layer as well as in the performance and stability of perovskite photovoltaic devices. We show that while the absorbance and morphology of the layers remains largely unaffected, the surface composition and energetics, crystallinity, emission efficiency, energetic disorder and storage stability are all very sensitive to the precise stoichiometry of the precursor solution. Our results elucidate the origin of the irreproducibility and inconsistencies of reported results among different groups as well as the wide spread in device performance even within individual studies. Finally, we propose a simple experimental method to identify the exact stoichiometry of the perovskite layer that researchers can employ to confirm their experiments are performed consistently without unintentional variations in precursor stoichiometry.

physics.app-ph↗

Non-volatile silicon photonic memory with more than 4-bit per cell capability

We present the first demonstration of an integrated photonic phase-change memory using GeSbTe-225 on silicon-on-insulator and demonstrate reliable multilevel operation with a single programming pulse. We also compare our results on silicon with previous demonstrations on silicon nitride. Crucially, achieving this on silicon enables tighter integration of traditional electronics with photonic memories in future, making phase-change photonic memory a viable and integrable technology.

physics.optics↗

Non-Closed Acoustic Cloak Enabled by Sequential-Step Linear Coordinate Transformations

Hitherto acoustic cloaking devices, which conceal objects externally, have depended on the objects' characteristics. Despite previous works, we design cloaking device placed neighbor an arbitrary object and makes it invisible without the need to make it enclosed. Applying sequential linear coordinate transformations, leads to a non-closed acoustic cloak (NCAC) with homogeneous materials that creates an open invisible region. We propose a non-closed carpet cloak to conceal objects on a reflecting plane. Numerical simulations verify the cloaking effect, which is completely independent of the geometry and material properties of the hidden object. Due to the simple acoustic constitutive parameters of presented structures, this work paves the way toward realization of non-closed acoustic devices, which could find applications in air born sound manipulation and underwater demands.

physics.app-ph↗

Forward and inverse acoustic scattering problems involving the mass density

This investigation is concerned with the 2D acoustic scattering problem of a plane wave propagating in a non-lossy fluid host and soliciting a linear, isotropic, macroscopically-homogeneous, lossy, flat-plane layer in which the mass density and wavespeed are different from those of the host. The focus is on the inverse problem of the retrieval of either the layer mass density or the real part of the layer wavespeed. The data is the transmitted pressure field, obtained by simulation (resolution of the forward problem) in exact, explicit form via separation of variables. Another form of this solution, which is exact and more explicit in terms of the mass-density contrast (between the host and layer), is obtained by a domain-integral method. A perturbation technique enables this solution to be cast as a series of powers of the mass density contrast, the first three terms of which are employed as the trial models in the treatment of the inverse problem. The aptitude of these models to retrieve the mass density contrast and real part of the layer wavespeed is demonstrated both theoretically and numerically. Keywords: 2D acoustics, forward scattering, inverse scattering, domain integral equation, constant mass density assumption, small density contrast, retrieval accuracy

physics.app-ph↗

Ultrathin complex oxide nanomechanical resonators

Complex oxide thin films and heterostructures exhibit a profusion of exotic phenomena, often resulting from the intricate interplay between film and substrate. Recently it has become possible to isolate epitaxially grown single-crystalline layers of these materials, enabling the study of their properties in the absence of interface effects. In this work, we create ultrathin membranes of strongly correlated materials and demonstrate top-down fabrication of nanomechanical resonators made out of \ce{SrTiO3} and \ce{SrRuO3}. Using laser interferometry, we successfully actuate and measure the motion of the nanodrum resonators. By measuring their temperature-dependent mechanical response, we observe signatures of structural phase transitions in \ce{SrTiO3}, which affect the strain and mechanical dissipation in the resonators. This approach can be extended to investigate phase transitions in a wide range of materials. Our study demonstrates the feasibility of integrating ultrathin complex oxide membranes for realizing nanoelectromechanical systems on arbitrary substrates.

physics.app-ph↗

Exploring inorganic and nontoxic double perovskites Cs$_2$AgInBr$_{6-x}$Cl$_x$ from material selection to device design in material genome approach

Halide double perovskites have recently been proposed as potential environmentally friendly alternatives to organic group and lead based hybrid halide perovskites. In particular, Cs2BiAgX6 have been synthesized and found to exhibit tunable band gaps in the visible range. However, the band gaps of these compounds are indirect, not ideal for applications in thin film photovoltaics. Here in this work we have carried out systematic modelling, using a materials genome approach in the framework of the density functional theory (DFT), to formulate a new system of solar absorption layer based on Cs2InAgX6 and its heterojunction device. Through Cl partial substitution on Br in Cs2InAgBr6 to optimize its thermodynamic stability after the calculation of ATAT proportion searching and Gibbs free energy, we have identified a series of stable cubic structured phases, with the general formula of Cs2AgInBr(6-x)Clx, as remarkable solar absorption layer to enable harvesting the solar energy. The optimized Cs2InAgBr5Cl compound is a marvellous solar absorption layer, with direct 1.92 eV bandgap and high solar absorption ability, consistent with Cs2InAgBr6 at standard room temperature (298 K). Assembling with anatase as n type TCO and Cs6Ag4In4Br18Cl4 as p type TCO fabricated by introducing Cs_Br defect, the heterojunction is integrated into PSCs based on the standard pin structure (TiO2_Cs2InAgBr5Cl_Cs6Ag4In4Br18Cl4), the lattice mismatching, microscopic function and band offset are evaluated for this well designed device.

physics.app-ph↗

Analysis, optimization, and characterization of magnetic photonic crystal structures and thin-film material layers

MPC (Magneto-Photonic Crystal) Optimisation is a feature-rich Windows software application designed to enable researchers to analyze the optical and magneto-optical spectral properties of multilayers containing gyrotropic constituents. A set of computational algorithms aimed at enabling the design optimization and optical or magneto-optical (MO) spectral analysis of 1D magnetic photonic crystals (MPC) is reported, together with its Windows software implementation. Relevant material property datasets (e.g., the optical spectra of refractive index, absorption, and gyration) of several important optical and MO materials are included, enabling easy reproduction of the previously published results from the field of MPC-based Faraday rotator development, and an effective demonstration-quality introduction of future users to the multiple features of this package. We also report on the methods and algorithms used to obtain the absorption coefficient spectral dispersion datasets for new materials, for which the film thickness, transmission spectrum, and refractive index dispersion function are known.

physics.app-ph↗

Study of tantalum and iridium as adhesion layers for Pt/LGS high temperature SAW devices

In this paper, we report on the use of tantalum and iridium as adhesion layers for platinum electrodes used in high temperature SAW devices based on langasite substrates (LGS). Unlike iridium, tantalum exhibits a great adhesive strength, and a very low mobility through the Pt film, ensuring a device lifetime of at least half an hour at 1000{\textdegree}C. The latter is limited by morphological modifications of platinum, starting by the apparition of crystallites on the surface, and followed by important terracing and breaking of the film continuity. SNMS and XRD measurements allowed us to show that these phenomena are likely intrinsic to platinum film, whatever be the nature of the adhesion layer. Finally, after having outlined a possible scenario leading to this deterioration, we consider some solutions that could replace platinum in order to increase the lifetime of LGS-based SAW devices in high temperatures conditions.

physics.app-ph↗