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arXiv2013

Nonadiabatic Effects in Ultracold Molecules via Anomalous Linear and Quadratic Zeeman Shifts

Anomalously large linear and quadratic Zeeman shifts are measured for weakly bound ultracold $^{88}$Sr$_2$ molecules near the intercombination-line asymptote. Nonadiabatic Coriolis coupling and the nature of long-range molecular potentials explain how this effect arises and scales roughly cubically with the size of the molecule. The linear shifts yield nonadiabatic mixing angles of the molecular states. The quadratic shifts are sensitive to nearby opposite $f$-parity states and exhibit fourth-order corrections, providing a stringent test of a state-of-the-art \textit{ab initio} model.

physics.atom-ph↗

arXiv2013

Imaging Cold Molecules on a Chip

We present the integrated imaging of cold molecules in a microchip environment. The on-chip de- tection is based on REMPI, which is quantum-state-selective and generally applicable. We demon- strate and characterize time-resolved spatial imaging and subsequently use it to analyze the effect of a phase-space manipulation sequence aimed at compressing the velocity distribution of a molec- ular ensemble with a view to future high-resolution spectroscopic studies. The realization of such on-chip measurements adds the final fundamental component to the molecule chip, offering a new and promising route for investigating cold molecules.

physics.atom-ph↗

arXiv2013

Accurate Atom Counting in Mesoscopic Ensembles

Many cold atom experiments rely on precise atom number detection, especially in the context of quantum-enhanced metrology where effects at the single particle level are important. Here, we investigate the limits of atom number counting via resonant fluorescence detection for mesoscopic samples of trapped atoms. We characterize the precision of these fluorescence measurements beginning from the single-atom level up to more than one thousand. By investigating the primary noise sources, we obtain single-atom resolution for atom numbers as high as 1200. This capability is an essential prerequisite for future experiments with highly entangled states of mesoscopic atomic ensembles.

physics.atom-ph↗

arXiv2013

Reaching Fermi degeneracy via universal dipolar scattering

We report on the creation of a degenerate dipolar Fermi gas of erbium atoms. We force evaporative cooling in a fully spin-polarized sample down to temperatures as low as 0.2 times the Fermi temperature. The strong magnetic dipole-dipole interaction enables elastic collisions between identical fermions even in the zero-energy limit. The measured elastic scattering cross section agrees well with the predictions from dipolar scattering theory, which follow a universal scaling law depending only on the dipole moment and on the atomic mass. Our approach to quantum degeneracy proceeds with very high cooling efficiency and provides large atomic densities, and it may be extended to various dipolar systems.

cond-mat.quant-gas↗

arXiv2014

Full counting statistics of laser excited Rydberg aggregates in a one-dimensional geometry

We experimentally study the full counting statistics of few-body Rydberg aggregates excited from a quasi-one-dimensional Rydberg gas. We measure asymmetric excitation spectra and increased second and third order statistical moments of the Rydberg number distribution, from which we determine the average aggregate size. Direct comparisons with numerical simulations reveal the presence of liquid-like spatial correlations, and indicate sequential growth of the aggregates around an initial grain. These findings demonstrate the importance of dissipative effects in strongly correlated Rydberg gases and introduce a way to study spatio-temporal correlations in strongly-interacting many-body quantum systems without imaging.

physics.atom-ph↗

arXiv2014

Adsorbate Electric Fields on a Cryogenic Atom Chip

We investigate the behaviour of electric fields originating from adsorbates deposited on a cryogenic atom chip as it is cooled from room temperature to cryogenic temperature. Using Rydberg electromagnetically induced transparency we measure the field strength versus distance from a 1 mm square of YBCO patterned onto a YSZ chip substrate. We find a localized and stable dipole field at room temperature and attribute it to a saturated layer of chemically adsorbed rubidium atoms on the YBCO. As the chip is cooled towards 83 K we observe a change in sign of the electric field as well as a transition from a localized to a delocalized dipole density. We relate these changes to the onset of physisorption on the chip surface when the van der Waals attraction overcomes the thermal desorption mechanisms. Our findings suggest that, through careful selection of substrate materials, it may be possible to reduce the electric fields caused by atomic adsorption on chips, opening up experiments to controlled Rydberg-surface coupling schemes.

physics.atom-ph↗

arXiv2014

Ultracold Heteronuclear Mixture of Ground and Excited State Atoms

We report on the realization of an ultracold mixture of lithium atoms in the ground state and ytterbium atoms in the excited metastable 3P2 state. Such a mixture can support broad magnetic Feshbach resonances which may be utilized for the production of ultracold molecules with an electronic spin degree of freedom, as well as novel Efimov trimers. We investigate the interaction properties of the mixture in the presence of an external magnetic field and find an upper limit for the background interspecies two-body inelastic decay coefficient of K'2 < 3e-12 cm^3/s for the 3P2 m_J=-1 substate. We calculate the dynamic polarizabilities of the Yb 3P2 magnetic substates for a range of wavelengths, and find good agreement with our measurements at 1064nm. Our calculations also allow the identification of magic frequencies where Yb ground and metastable states are identically trapped and the determination of the interspecies van der Waals coefficients.

physics.atom-ph↗

arXiv2014

Quantum Joule-Thomson Effect in a Saturated Homogeneous Bose Gas

We study the thermodynamics of Bose-Einstein condensation in a weakly interacting quasi-homogeneous atomic gas, prepared in an optical-box trap. We characterise the critical point for condensation and observe saturation of the thermal component in a partially condensed cloud, in agreement with Einstein's textbook picture of a purely statistical phase transition. Finally, we observe the quantum Joule-Thomson effect, namely isoenthalpic cooling of an (essentially) ideal gas. In our experiments this cooling occurs spontaneously, due to energy-independent collisions with the background gas in the vacuum chamber. We extract a Joule-Thomson coefficient $μ_{\rm JT} > 10^9$ K/bar, about ten orders of magnitude larger than observed in classical gases.

cond-mat.quant-gas↗

arXiv2014

Antiresonance phase shift in strongly coupled cavity QED

We investigate phase shifts in the strong coupling regime of single-atom cavity quantum electrodynamics (QED). On the light transmitted through the system, we observe a phase shift associated with an antiresonance and show that both its frequency and width depend solely on the atom, despite the strong coupling to the cavity. This shift is optically controllable and reaches 140 degrees - the largest ever reported for a single emitter. Our result offers a new technique for the characterization of complex integrated quantum circuits.

quant-ph↗

arXiv2014

Effective mass signatures in multiphoton pair production

Electron-positron pair production in oscillating electric fields is investigated in the nonperturbative threshold regime. Accurate numerical solutions of quantum kinetic theory for corresponding observables are presented and analyzed in terms of a proposed model for an effective mass of electrons and positrons acquired within the given strong electric field. Although this effective mass cannot provide an exact description of the collective interaction of a charged particle with the strong field, physical observables are identified which carry direct and sensitive signatures of the effective mass.

hep-ph↗

arXiv2014

Proposed Entanglement of X-ray Nuclear Polaritons as a Potential Method for Probing Matter at the Subatomic Scale

A setup for generating the special superposition of a simultaneously forward- and backward-propagating collective excitation in a nuclear sample is studied. We show that by actively manipulating the scattering channels of single x-ray quanta with the help of a normal incidence x-ray mirror, a nuclear polariton which propagates in two opposite directions can be generated. The two counterpropagating polariton branches are entangled by a single x-ray photon. The quantum nature of the nuclear excitation entanglement gives rise to a subangstrom-wavelength standing wave excitation pattern that can be used as a flexible tool to probe matter dynamically on the subatomic scale.

quant-ph↗

arXiv2014

Hyperfine structure in $^{229g}$Th$^{3+}$ as a probe of the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy

We identify a potential means to extract the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy from precision microwave spectroscopy of the $5F_{5/2,7/2}$ hyperfine manifolds in the ion $^{229g}$Th$^{3+}$. The hyperfine interaction mixes this ground fine structure doublet with states of the nuclear isomer, introducing small but observable shifts to the hyperfine sub-levels. We demonstrate how accurate atomic structure calculations may be combined with measurement of the hyperfine intervals to quantify the effects of this mixing. Further knowledge of the magnetic dipole decay rate of the isomer, as recently reported, allows an indirect determination of the nuclear excitation energy.

physics.atom-ph↗

arXiv2013

Suppressing the loss of ultracold molecules via the continuous quantum Zeno effect

We investigate theoretically the suppression of two-body losses when the on-site loss rate is larger than all other energy scales in a lattice. This work quantitatively explains the recently observed suppression of chemical reactions between two rotational states of fermionic KRb molecules confined in one-dimensional tubes with a weak lattice along the tubes [Yan et al., Nature 501, 521-525 (2013)]. New loss rate measurements performed for different lattice parameters but under controlled initial conditions allow us to show that the loss suppression is a consequence of the combined effects of lattice confinement and the continuous quantum Zeno effect. A key finding, relevant for generic strongly reactive systems, is that while a single-band theory can qualitatively describe the data, a quantitative analysis must include multiband effects. Accounting for these effects reduces the inferred molecule filling fraction by a factor of five. A rate equation can describe much of the data, but to properly reproduce the loss dynamics with a fixed filling fraction for all lattice parameters we develop a mean-field model and benchmark it with numerically exact time-dependent density matrix renormalization group calculations.

quant-ph↗

arXiv2014

Dominant Secondary Nuclear Photoexcitation with the X-ray Free Electron Laser

The new regime of resonant nuclear photoexcitation rendered possible by x-ray free electron laser beams interacting with solid state targets is investigated theoretically. Our results unexpectedly show that secondary processes coupling nuclei to the atomic shell in the created cold high-density plasma can dominate direct photoexcitation. As an example we discuss the case of $^{93m}$Mo isomer depletion for which nuclear excitation by electron capture as secondary process is shown to be orders of magnitude more efficient than the direct laser-nucleus interaction. General arguments revisiting the role of the x-ray free electron laser in nuclear experiments involving solid-state targets are further deduced.

nucl-th↗

arXiv2014

Vortices associated with the wave function of a single electron emitted in slow ion-atom collisions

We present measurements and calculations of the momentum distribution of electrons emitted during the ion-atom collision 10 keV/u $He^{2+}+He \rightarrow He^{+} + He^{2+} + e^{-}$, which show rich structures for ion scattering angles above 2 mrad arising dominantly from two-electron states. Our calculations reveal that minima in the measured distributions are zeros in the electronic probability density resulting from vortices in the electronic current.

physics.atom-ph↗

arXiv2014

Local observation of pair-condensation in a Fermi gas at unitarity

We present measurements of the local (homogeneous) density-density response function of a Fermi gas at unitarity using spatially resolved Bragg spectroscopy. By analyzing the Bragg response across one axis of the cloud we extract the response function for a uniform gas which shows a clear signature of the Bose-Einstein condensation of pairs of fermions when the local temperature drops below the superfluid transition temperature. The method we use for local measurement generalizes a scheme for obtaining the local pressure in a harmonically trapped cloud from the line density and can be adapted to provide any homogeneous parameter satisfying the local density approximation.

cond-mat.quant-gas↗

arXiv2013

New limit on Lorentz and CPT violating neutron spin interactions using a free precession 3He-129Xe co-magnetometer

We report on the search for a CPT and Lorentz invariance violating coupling of the 3He and 129Xe nuclear spins (each largely determined by a valence neutron) to background tensor fields which permeate the universe. Our experimental approach is to measure the free precession of nuclear spin polarized 3He and 129Xe atoms in a homogeneous magnetic guiding field of about 400 nT using LTC SQUIDs as low-noise magnetic flux detectors. As the laboratory reference frame rotates with respect to distant stars, we look for a sidereal modulation of the Larmor frequencies of the co-located spin samples. As a result we obtain an upper limit on the equatorial component of the background field interacting with the spin of the bound neutron bn< 6.7*10^-34 GeV (68% C.L.). Our result improves our previous limit (data measured in 2009) by a factor of 30 and the world's best limit by a factor of 5.

gr-qc↗

arXiv2014

Decoherence-assisted spectroscopy of a single Mg$^+$ ion

We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly at rest are recorded efficiently with high signal-to-noise ratios. Spectra display symmetric line shapes without stray-light background from spectroscopy probes. We employ this method on a $^{25}$Mg$^+$ ion to measure one, two, and three-photon transition frequencies from the 3S ground state to the 3P, 3D, and 4P excited states, respectively. Our results are relevant for astrophysics and searches for drifts of fundamental constants. Furthermore, the method can be extended to other transitions, isotopes, and species. The currently achieved fractional frequency uncertainty of $5 \times 10^{-9}$ is not limited by the method.

physics.atom-ph↗