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Incommensurate phonon anomaly and the nature of charge density waves in cuprates

While charge density wave (CDW) instabilities are ubiquitous to superconducting cuprates, the different ordering wavevectors in various cuprate families have hampered a unified description of the CDW formation mechanism. Here we investigate the temperature dependence of the low energy phonons in the canonical CDW ordered cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$. We discover that the phonon softening wavevector associated with CDW correlations becomes temperature dependent in the high-temperature precursor phase and changes from a wavevector of 0.238 reciprocal space units (r.l.u.) below the ordering transition temperature up to 0.3~r.l.u. at 300~K. This high-temperature behavior shows that "214"-type cuprates can host CDW correlations at a similar wavevector to previously reported CDW correlations in non-"214"-type cuprates such as YBa$_{2}$Cu$_{3}$O$_{6+δ}$. This indicates that cuprate CDWs may arise from the same underlying instability despite their apparently different low temperature ordering wavevectors.

cond-mat.supr-con↗

The influence of structural defects on intra-granular critical currents of bulk MgB2

Bulk MgB2 samples were prepared under different synthesis conditions and analyzed by scanning and transmission electron microscopy. The critical current densities were determined from the magnetization versus magnetic field curves of bulk and powder-dispersed-in-epoxy samples. Results show that through a slow cooling process, the oxygen dissolved in bulk MgB2 at high synthesis temperatures can segregate and form nanometer-sized coherent precipitates of Mg(B,O)2 in the MgB2 matrix. Magnetization measurements indicate that these precipitates act as effective flux pinning centers and therefore significantly improve the intra-grain critical current density and its field dependence.

cond-mat.mtrl-sci↗

Influence of the Preparation Process on Microstructure, Critical Current Density and Tc of MgB2 Powder-In-Tube Wires

MgB2 wires and tapes suffer from a limitation of the transport current densities, especially at low field, due to an unsufficient thermal stabilization caused by hot spots from a non-homogeneous microstructure, the presence of secondary phases and voids. For the preparation of MgB2 wires and tapes two different precursor routes, using MgB2 (ex-situ process) or Mg + B (in-situ process) are applied. The in-situ approach allows variation of many parameters in the wire preparation and the improvement of this approach is the central topic of this paper. We present an improved in-situ approach, the characterization of the filament microstructure, effects from stoichiometry and the corresponding superconducting properties. The transport current capability of such in-situ wires could be improved to the level of the reference ex-situ wires.

cond-mat.supr-con↗

Tunnel junctions on as-grown superconducting MgB2 thin films

We demonstrate that good superconductor/insulator/normal-metal tunnel junctions can be fabricated on as-grown superconducting MgB2 thin films. The as-grown films were prepared by coevaporation at low growth temperatures of around 280deg. The insulating barrier was formed by an Mg overlayer, which is subsequently oxidized in air. The tunneling spectra for Au/MgOx/MgB2 junctions showed a reproducible and well-defined superconducting gap (delta= ~ 2.5 meV). The resultant 2delta/ kBTc was significantly smaller than the predicted BCS value of 3.52.

cond-mat.supr-con↗

Mechanical properties of reinforced MgB2 wires

For technical application in windings of coils, transformers or motors, a reinforcement of MgB2 wires and tapes is necessary to withstand applied stresses and strains and to avoid cracks in the filaments. Therefore, the response of the superconducting transport currents on applied axial strain in different magnetic background fields was investigated for differently stainless steel reinforced MgB2 wires, by means of an axial strain rig. Increased amounts of stainless steel in the sheath caused a stronger decrease of the critical currents in fields above 3 T as a consequence of a changed irreversibility field. Heat treated wires have a quite different mechanical behaviour compared to as-cold-worked wires, but an about 10 times higher transport current level. Tape geometries, having generally higher current carrying capabilities than wires, showed much poorer mechanical properties with a less effective filament precompression from the matrix.

cond-mat.supr-con↗

Magnetic shielding in MgB2/Fe superconducting wires

Transport critical current (Ic) was measured for MgB2/Fe round wires, with magnetic field oriented perpendicular to the wire and parallel to it. Measurements were made on a wire with pure MgB2 core and another wire where MgB2 core was doped with nano-size SiC. This doping strongly improved the vortex pinning in MgB2. The field dependence of Ic was strongly improved due to the presence of the iron sheath. At 30K, Ic did not depend on the field for fields between 0.09 and 0.7T. At lower temperatures, Ic increased with the field, after initial decrease, resembling a "peak effect". This effect was extended to higher fields as the temperature went down: at 10K the peak appeared at 3.5T. This improvement was not due to mere magnetic shielding by iron, but more likely to an interaction between the iron sheath and superconductor. Improvement of vortex pinning did not affect the range of fields within which this effect was observed.

cond-mat.supr-con↗

Effects of Ion Milling on the Microwave Properties of MgB2 Films

The new superconductor MgB2 may prove useful for microwave applications at intermediate temperatures. MgB2 films with the thickness of 300 - 400 nm have surface resistance Rs less than 0.01 mOhms at a frequency (f) of 8.5 GHz and 7 K,and ~ 1.5 mOhms at 87 GHz and 4.2 K. The critical temperature (Tc) of these films is ~ 39 K when they are prepared under optimum conditions. The Rs appears to scale as f^2 up to 30 K. After surface ion-milling, a reduction of the Tc and an enhanced resistivity rho(Tc) are observed consistently at 8.5 GHz and 87 GHz along with a reduced Rs at low temperatures. The observed rho(Tc) - Tc relation and the uncorrelated behavior between rho(Tc) and Rs values measured at low temperatures are well explained in terms of the two-gap model, with the observed rho(Tc) - Tc relation attributed to the properties of the large gap, and the Rs at lower temperatures reflecting the properties of the small gap, with an enhanced small gap energy due to increased interband scattering. This study suggests that the interband scattering should be enhanced to improve the low temperature microwave properties of MgB2 films and that the ion-milling process must be performed with great care to preserve the high quality of MgB2 films.

cond-mat.supr-con↗

AC losses in type-II superconductors induced by nonuniform fluctuations of external magnetic field

Magnetic field fluctuations are inevitable in practical applications of superconductors and it is often necessary to estimate the AC losses these fluctuations induce. If the fluctuation wavelength is greater than the size of a superconductor, known estimates for an alternating uniform external magnetic field can be employed. Here we consider the opposite case and analyze, using a model critical-state problem, penetration of spatially nonuniform fluctuations into type-II superconductors. Numerical simulation is based on a variational formulation of the Bean model. The analytical solutions, found in a weak penetration limit, are used to evaluate AC losses for two types of fluctuations: the running and standing waves. It is shown that for spatially nonuniform fluctuations the losses are better characterized by the fluctuation penetration depth than by the fluctuation amplitude. The results can be used to estimate the AC losses in flywheels, electric motors, magnetic shields, etc.

cond-mat.supr-con↗

Upper Critical Fields up to 60T in Dirty Magnesium Diboride Thin Films

Upper critical fields of several magnesium diboride thin films were measured up to 28 T at the Grenoble High Magnetic Field Laboratory (GHMFL) in Grenoble and up to 60 T at the Laboratoire National des Champs Magnetiques Pulses (LNCMP) in Toulouse. The samples were prepared both by pulsed laser deposition (PLD) and hybrid physical chemical vapour deposition (HPCVD) technique; they have critical temperatures between 29 and 39 K and normal state resistivities between 5 and 250 μohmcm; one of them has been intentionally doped with carbon. The measured critical fields were exceptionally high; we obtained the record value of 52 T at 4.2 K in the parallel orientation. In contrast with the BCS predictions, no saturation in Hc2 at low temperature was observed. Furthermore, films with a wide range of resistivity values showed similar critical fields, suggesting that in a two band system resistivity and Hc2 are not trivially linked. The high Hc2 values seem to be related with the expanded c-axis. The structure of one of the samples was carefully investigated with X-ray diffraction at European Synchrotron Radiation Facility (ESRF) in Grenoble.

cond-mat.supr-con↗

A novel process to produce amorphous nano-sized B useful for MgB2 phase synthesis

In this paper we report a new synthesis route to produce boron powders characterized as being amorphous and having very fine particle size. This route has been developed to improve the performances of superconducting MgB2 powders, which can be directly synthesized from this nano-structured boron precursor by following the ex-situ or the in-situ P.I.T. method during the manufacturing of tapes, wires and cables. All the procedure steps are explained and the chemical-physical characterization of the boron powder, using x-ray diffraction (Xrd), scanning electron microscopy (SEM) and transmission electron microscopy (TEM) techniques, is reported. Furthermore, a comparison with commercial boron is given. Preliminary results of the magnetic and electrical characterization, such as the critical temperature (TC) and the transport critical current density (JC t), for the MgB2 tape are reported and compared with the tape prepared with commercial boron.

cond-mat.supr-con↗

AC Losses of Copper Stabilized Multifilament YBCO Coated Conductors

We report the data on magnetization losses and critical current of multifilament copper stabilized coated conductors. Eight centimeters long samples of copper stabilized YBa2Cu3O7-x (YBCO) coated conductors manufactured commercially were subdivided into superconducting filaments by near-IR laser micromachining. The width of the superconducting stripes was varied from 0.2 mm to 0.04 mm. Some of the samples were striated leaving superconducting bridges for current sharing between the filaments. The AC losses were measured at different sweep rates of the magnetic field up to 14 T/s. We will present the results for the hysteresis and coupling losses and discuss the means to reduce the coupling loss by changing the processing parameters of micromachining and by post-ablation treatment.

cond-mat.supr-con↗

Highly responsive Y-Ba-Cu-O thin film THz detectors with picosecond time resolution

High-temperature superconducting YBa2Cu3O7-d (YBCO) thin-film detectors with improved responsivities were developed for fast time-domain measurements in the THz frequency range. YBCO thin films of 30 nm thickness were patterned to micro- and nanobridges and embedded into planar log-spiral THz antennas. The YBCO thin-film detectors were characterized with continuous wave radiation at 0.65 THz. Responsivity values as high as 710 V/W were found for the YBCO nanobridges. Pulsed measurements in the THz frequency range were performed at the electron storage ring ANKA from the Karlsruhe Institute of Technology (KIT). Due to the high responsivities of the nanobridges no biasing was required for the detection of the coherent synchrotron radiation pulses achieving very good agreement between the measured pulse shapes and simulations.

cond-mat.supr-con↗

MOD derived pyrochlore films as buffer layer for all-chemical YBCO coated conductors

We report a detailed study performed on La2Zr2O7 (LZO) pyrochlore material grown by Metal-Organic Decomposition (MOD) method as buffer layers for YBa2Cu3O7-x (YBCO) coated conductors. High quality epitaxial LZO thin films have been obtained on single crystal (SC) and Ni-5%at.W substrates. In order to evaluate structural and morphological properties, films have been characterized by means of X-ray diffraction analyses (XRD), atomic force microscope (AFM) and scanning electron microscope (SEM). Precursors solutions and heat treatments have been studied by thermogravimetric analyses (TG-DTA-DTG) and infrared spectra (FT-IR) with the aim of optimizing the annealing process. Thin films of YBCO have been deposited by pulsed laser ablation (PLD) on this buffer layers. The best results obtained on SC showed YBCO films with critical temperature values above 90 K, high self field critical current density values (Jc > 1 MA/cm2) and high irreversibility field values (8.3 T) at 77 K together with a rather high depinning frequency vp (0.5 T, 77 K)>44 GHz as determined at microwaves. The best results on Ni-5%at.W has been obtained introducing in the heat treatment a pyrolysis process at low temperature in air in order to remove the residual organic part of the precursor solution.

cond-mat.supr-con↗

Thermal Conductivity of Industrial Nb3Sn Wires Fabricated by Various Techniques

We have developed a new experimental setup specifically designed for measuring thermal conductivity on technical superconductors in the range of temperatures from 3 to 330 K in magnetic fields up to 21 T. Three Nb3Sn wires, produced by the powder in tube technique, the bronze route and the internal tin restacked rod process, respectively, have been investigated. We show that, due to the complexity of the architecture of these wires, direct measurement of thermal conductivity is required for a correct estimation of thermal stability in superconducting magnets.

cond-mat.supr-con↗

Development of 2D Bi-SQUID Arrays with High Linearity

We develop a two-dimensional (2D) Superconducting Quantum Interference Filter (SQIF) array based on recently introduced high-linearity tri-junction bi-SQUIDs. Our bi-SQUID SQIF array design is based on a tight integration of individual bi- SQUID cells sharing inductances with adjacent cells. We provide extensive computer simulations, analysis and experimental measurements, in which we explore the phase dynamics and linearity of the array voltage response. The non-uniformity in inductances of the bi-SQUIDs produces a pronounced zero-field single antipeak in the voltage response. The anti-peak linearity and size can be optimized by varying the critical current of the additional junction of each bi-SQUID. The layout implementation of the tight 2D array integration leads to a distinct geometrical diamond shape formed by the merged dual bi-SQUID cells. Different size 2D arrays are fabricated using standard HYPRES niobium 4.5 kA/cm2 fabrication process. The measured linearity, power gain, and noise properties will be analyzed for different array sizes and the results will be compared with circuit simulations. We will discuss a design approach for the electrically small magnetic field antenna and low-noise amplifiers with high bandwidth based on these 2D bi-SQUID SQIF arrays. The results from this work will be used to design chips densely and completely covered in bi-SQUIDs that has optimized parameters such as linearity and power gain.

physics.ins-det↗

Improved nanopatterning for YBCO nanowires approaching the depairing current

An improved nanopatterning procedure has been developed to obtain YBCO nanowires with cross sections as small as 50x50 nm^2, protected by an Au capping layer. To probe the effective role of the Au protecting layer, we have measured the current-voltage characteristics and the resistive transition in temperature of the nanowires. Critical current densities up to 10^8 A/cm^2 have been achieved at T=4.2 K, approaching the theoretical depairing current limit. The resistance, measured as a function of temperature close to Tc, has been fitted with a thermal activated phase slip model, including the effect of the gold layer. The extracted values of the superconducting coherence length and of the London penetration depth give current densities consistent with the measured ones. These results cannot be achieved with same nanowires, without the Au capping layer.

cond-mat.supr-con↗

Computation of Losses in HTS Under the Action of Varying Magnetic Fields and Currents

Numerical modeling of superconductors is widely recognized as a powerful tool for interpreting experimental results, understanding physical mechanisms and predicting the performance of high-temperature superconductor (HTS) tapes, wires and devices. This is especially true for ac loss calculation, since a sufficiently low ac loss value is imperative to make these materials attractive for commercialization. In recent years, a large variety of numerical models, based on different techniques and implementations, have been proposed by researchers around the world, with the purpose of being able to estimate ac losses in HTSs quickly and accurately. This article presents a literature review of the methods for computing ac losses in HTS tapes, wires and devices. Technical superconductors have a relatively complex geometry (filaments, which might be twisted or transposed, or layers) and consist of different materials. As a result, different loss contributions exist. In this paper, we describe the ways of computing such loss contributions, which include hysteresis losses, eddy current losses, coupling losses, and losses in ferromagnetic materials. We also provide an estimation of the losses occurring in a variety of power applications.

cond-mat.supr-con↗

Microwave Response of Coaxial Cavities Made of Bulk Magnesium Diboride

We report on the microwave (mw) properties of coaxial cavities built by using bulk MgB2 superconductor prepared by reactive liquid Mg infiltration technology. We have assembled a homogeneous cavity, by using an outer MgB2 cylinder and an inner MgB2 rod, and a hybrid cavity by using an outer copper cylinder and the same MgB2 rod as inner conductor. By the analysis of the resonance curves, in the different resonant modes, we have determined the microwave surface resistance, Rs, of the MgB2 materials as a function of the temperature and the frequency, in the absence of DC magnetic fields. At T = 4.2 K and f = 2.5 GHz, by a mw pulsed technique, we have determined the quality factor of the homogeneous cavity as a function of the input power up to a maximum level of about 40 dBm (corresponding to a maximum peak magnetic field of about 100 Oe). Contrary to what occurs in many films, Rs of the MgB2 material used does not exhibit visible variations up to an input power level of about 10 dBm and varies less than a factor of 2 on further increasing the input power of 30 dB.

cond-mat.supr-con↗