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Accounting for adsorption and desorption in lattice Boltzmann simulations

We report a Lattice-Boltzmann scheme that accounts for adsorption and desorption in the calculation of mesoscale dynamical properties of tracers in media of arbitrary complexity. Lattice Boltzmann simulations made it possible to solve numerically the coupled Navier-Stokes equations of fluid dynamics and Nernst-Planck equations of electrokinetics in complex, heterogeneous media. Associated to the moment propagation scheme, it became possible to extract the effective diffusion and dispersion coefficients of tracers, or solutes, of any charge, e.g. in porous media. Nevertheless, the dynamical properties of tracers depend on the tracer-surface affinity, which is not purely electrostatic, but also includes a species-specific contribution. In order to capture this important feature, we introduce specific adsorption and desorption processes in a Lattice-Boltzmann scheme through a modified moment propagation algorithm, in which tracers may adsorb and desorb from surfaces through kinetic reaction rates. The method is validated on exact results for pure diffusion and diffusion-advection in Poiseuille flows in a simple geometry. We finally illustrate the importance of taking such processes into account on the time-dependent diffusion coefficient in a more complex porous medium.

physics.flu-dyn↗

Axisymmetric multiphase lattice Boltzmann method

A lattice Boltzmann method for axisymmetric multiphase flows is presented and validated. The method is capable of accurately modeling flows with variable density. We develop the classic Shan-Chen multiphase model [ Phys. Rev. E 47 1815 (1993)] for axisymmetric flows. The model can be used to efficiently simulate single and multiphase flows. The convergence to the axisymmetric Navier-Stokes equations is demonstrated analytically by means of a Chapmann-Enskog expansion and numerically through several test cases. In particular, the model is benchmarked for its accuracy in reproducing the dynamics of the oscillations of an axially symmetric droplet and on the capillary breakup of a viscous liquid thread. Very good quantitative agreement between the numerical solutions and the analytical results is observed.

physics.comp-ph↗

Effective slip-length tensor for a flow over weakly slipping stripes

We discuss the flow past a flat heterogeneous solid surface decorated by slipping stripes. The spatially varying slip length, $b(y)$, is assumed to be small compared to the scale of the heterogeneities, $L$, but finite. For such "weakly" slipping surfaces, earlier analyses have predicted that the effective slip length is simply given by the surface-averaged slip length, which implies that the effective slip-length tensor becomes isotropic. Here we show that a different scenario is expected if the local slip length has step-like jumps at the edges of slipping heterogeneities. In this case, the next-to-leading term in an expansion of the effective slip-length tensor in powers of ${max}\,(b(y)/L)$ becomes comparable to the leading-order term, but anisotropic, even at very small $b(y)/L$. This leads to an anisotropy of the effective slip, and to its significant reduction compared to the surface-averaged value. The asymptotic formulae are tested by numerical solutions and are in agreement with results of dissipative particle dynamics simulations.

physics.flu-dyn↗

Excited Sessile Drops Dance Harmonically

In our fluid dynamics video, we demonstrate our method of visualizing and identifying various mode shapes of mechanically oscillated sessile drops. By placing metal mesh under an oscillating drop and projecting light from below, the drop's shape is visualized by the visually deformed mesh pattern seen in the top view. The observed modes are subsequently identified by their number of layers and sectors. An alternative identification associates them with spherical harmonics, as demonstrated in the tutorial. Clips of various observed modes are presented, followed by a 10-second quiz of mode identification.

physics.flu-dyn↗

Intermittent flow in yield-stress fluids slows down chaotic mixing

In this article, we present experimental results of chaotic mixing of Newtonian uids and yield stress fluids using rod-stirring protocol with rotating vessel. We show how the mixing of yield stress fluids by chaotic advection is reduced compared to the mixing of Newtonian fluids and explain our results bringing to light the relevant mechanisms: the presence of fluid that only flows intermittently, a phenomenon enhanced by the yield stress, and the importance of the peripheral region. This finding is confirmed via numerical simulations. Anomalously slow mixing is observed when the synchronization of different stirring elements leads to the repetition of slow stretching for the same fluid particles.

cond-mat.soft↗

Experimental investigation of the stability of the floating water bridge

When a high voltage is applied between two beakers filled with deionized water, a bridge of water may be formed in between exceeding the length of 2 cm when the beakers are pulled apart. We construct experiments in which the geometry and the electric field within the bridge are measured and compared with predictions of theories on the floating water bridge. A numerical simulation is used for the measurement of the electric field. Our experimental results approve that two forces of dielectric tension and surface tension are holding the bridge against gravity. These forces have the same order of magnitude. Results show that the stability can be explained by macroscopic forces, regardless of the microscopic changes in water structure.

physics.flu-dyn↗

Log-normal distribution from a process that is not multiplicative but is additive

The central limit theorem ensures that a sum of random variables tends to a Gaussian distribution as their total number tends to infinity. However, for a class of positive random variables, we find that the sum tends faster to a log-normal distribution. Although the sum tends eventually to a Gaussian distribution, the distribution of the sum is always close to a log-normal distribution rather than to any Gaussian distribution if the summands are numerous enough. This is in contrast to the current consensus that any log-normal distribution is due to a product of random variables, i.e., a multiplicative process, or equivalently to nonlinearity of the system. In fact, the log-normal distribution is also observable for a sum, i.e., an additive process that is typical of linear systems. We show conditions for such a sum, an analytical example, and an application to random scalar fields such as of turbulence.

physics.flu-dyn↗

Nonlinear electrohydrodynamics of a viscous droplet

A classic result due to G.I.Taylor is that a drop placed in a uniform electric field becomes a prolate or oblate spheroid, which is axisymmetrically aligned with the applied field. We report an instability and symmetry-breaking transition to obliquely oriented, steady and unsteady shapes in strong fields. Our experiments reveal novel droplet behaviors such as tumbling, shape oscillations, and chaotic dynamics even under creeping flow conditions. A theoretical model, which includes anisotropy in the polarization relaxation due to drop asphericity and charge convection due to drop fluidity, elucidates the interplay of interfacial flow and charging as the source of the rich nonlinear dynamics.

physics.flu-dyn↗

Bifurcations and dynamics in convection with temperature-dependent viscosity in the presence of the O(2) symmetry

We focus the study of a convection problem in a 2D setup in the presence of the O(2) symmetry. The viscosity in the fluid depends on the temperature as it changes its value abruptly in an interval around a temperature of transition. The influence of the viscosity law on the morphology of the plumes is examined for several parameter settings, and a variety of shapes ranging from spout to mushroom shaped is found. We explore the impact of the symmetry on the time evolution of this type of fluid, and find solutions which are greatly influenced by its presence: at a large aspect ratio and high Rayleigh numbers, traveling waves, heteroclinic connections and chaotic regimes are found. These solutions, which are due to the symmetry presence, have not been previously described in the context of temperature dependent viscosities. However, similarities are found with solutions described in other contexts such as flame propagation problems or convection problems with constant viscosity also under the presence of the O(2) symmetry, thus confirming the determining role of the symmetry in the dynamics.

physics.flu-dyn↗

Information Content of Turbulence

We treat a turbulent velocity field as a message in the same way as a book or a picture. All messages can be described by their entropy per symbol $h$, defined as in Shannon's theory of communication. In a turbulent flow, as the Reynolds number $Re$ increases, more correlated degrees of freedom are excited and participate in the turbulent cascade. Experiments in a turbulent soap film suggest that the spatial entropy density $h$ is a decreasing function of $Re$, namely $h \propto -\log Re$ + const. In the logistic map, also analyzed here, increasing the control parameter $r$ increases $h$. A modified logistic map with additional coupling to past iterations suggests the significance of correlations.

nlin.CD↗

Achieving tunable surface tension in the pseudopotential lattice Boltzmann modeling of multiphase flows

In this paper, we aim to address an important issue about the pseudopotential lattice Boltzmann (LB) model, which has attracted much attention as a mesoscopic model for simulating interfacial dynamics of complex fluids, but suffers from the problem that the surface tension cannot be tuned independently of the density ratio. In the literature, a multi-range potential was devised to adjust the surface tension [Sbragaglia et al., Phys. Rev. E 75, 026702 (2007)]. However, it was recently found that the density ratio of the system will be changed when the multi-range potential is employed to adjust the surface tension. A new approach is therefore proposed in the present work. The basic strategy is to add a source term to the LB equation so as to tune the surface tension of the pseudopotential LB model. The proposed approach can guarantee that the adjustment of the surface tension does not affect the mechanical stability condition of the pseudopotential LB model, and thus provides a separate control of the surface tension and the density ratio. Meanwhile, it still retains the mesoscopic feature and the computational simplicity of the pseudopotential LB model. Numerical simulations are carried out for stationary droplets, capillary waves, and droplet splashing on a thin liquid film. The numerical results demonstrate that the proposed approach is capable of achieving a tunable surface tension over a very wide range and can keep the density ratio unchanged when adjusting the surface tension.

physics.comp-ph↗

Soft beams: when capillarity induces axial compression

We study the interaction of an elastic beam with a liquid drop in the case where bending and extensional effects are both present. We use a variational approach to derive equilibrium equations and constitutive relation for the beam. This relation is shown to include a term due to surface energy in addition of the classical Young's modulus term, leading to a modification of Hooke's law. At the triple point where solid, liquid, and vapor phases meet we find that the external force applied on the beam is parallel to the liquid-vapor interface. Moreover, in the case where solid-vapor and solid-liquid interface energies do not depend on the extension state of the beam, we show that the extension in the beam is continuous at the triple point and that the wetting angle satisfy the classical Young-Dupré relation.

cond-mat.soft↗

Identification of Separation Wavenumber between Weak and Strong Turbulence Spectra for Vibrating Plate

A weakly nonlinear spectrum and a strongly nonlinear spectrum coexist in a statistically steady state of elastic wave turbulence. The analytical representation of the nonlinear frequency is obtained by evaluating the extended self-nonlinear interactions. The {\em critical\/} wavenumbers at which the nonlinear frequencies are comparable with the linear frequencies agree with the {\em separation\/} wavenumbers between the weak and strong turbulence spectra. We also confirm the validity of our analytical representation of the separation wavenumbers through comparison with the results of direct numerical simulations by changing the material parameters of a vibrating plate.

nlin.CD↗

Transient Growth of Ekman-Couette Flow

Coriolis force effects on shear flows are important in geophysical and astrophysical contexts. We here report a study on the linear stability and the transient energy growth of the plane Couette flow with system rotation perpendicular to the shear direction. External rotation causes linear instability. At small rotation rates, the onset of linear instability scales inversely with the rotation rate and the optimal transient growth in the linearly stable region is slightly enhanced, ~Re^2. The corresponding optimal initial perturbations are characterized by roll structures inclined in the streamwise direction and are twisted under external rotation. At large rotation rates, the transient growth is significantly inhibited and hence linear stability analysis is a reliable indicator for instability.

physics.flu-dyn↗

Role of roughness on the hydrodynamic homogeneous base state of inelastic spheres

A gas of inelastic rough spheres admits a spatially homogeneous base state which turns into a hydrodynamic state after a finite relaxation time. We show that this relaxation time is hardly dependent on the degree of inelasticity but increases dramatically with decreasing roughness. An accurate description of translational-rotational velocity correlations at all times is also provided. At a given inelasticity, the roughness parameter can be tuned to produce a huge distortion from the Maxwellian distribution function. The results are obtained from a Grad-like solution of the Boltzmann-Enskog equation complemented by Monte Carlo and molecular dynamics simulations.

cond-mat.soft↗

Energy flux measurement from the dissipated energy in capillary wave turbulence

We study experimentally the influence of dissipation on stationary capillary wave turbulence on the surface of a fluid by changing its viscosity. We observe that the frequency power law scaling of the capillary spectrum departs significantly from its theoretical value when the dissipation is increased. The energy dissipated by capillary waves is also measured and found to increase nonlinearly with the mean power injected within the fluid. Here, we propose an experimental estimation of the energy flux at every scale of the capillary cascade. The latter is found to be non constant through the scales. For fluids of low enough viscosity, we found that both capillary spectrum scalings with the frequency and the newly defined mean energy flux are in good agreement with wave turbulence theory. The Kolmogorov-Zakharov constant is then experimentally estimated and compared to its theoretical value.

physics.flu-dyn↗

Scaling of heat flux and energy spectrum for "very large" Prandtl number convection

Under the limit of infinite Prandtl number, we derive analytical expressions for the large-scale quantities, e.g., Péclet number Pe, Nusselt number Nu, and rms value of the temperature fluctuations $θ_\mathrm{rms}$. We complement the analytical work with direct numerical simulations, and show that $\mathrm{Nu} \sim \mathrm{Ra}^γ$ with $γ\approx (0.30-0.32)$, $\mathrm{Pe} \sim \mathrm{Ra}^η$ with $η\approx (0.57-0.61)$, and $θ_\mathrm{rms} \sim \mathrm{const}$. The Nusselt number is observed to be an intricate function of $\mathrm{Pe}$, $θ_\mathrm{rms}$, and a correlation function between the vertical velocity and temperature. Using the scaling of large-scale fields, we show that the energy spectrum $E_u(k)\sim k^{-13/3}$, which is in a very good agreement with our numerical results. The entropy spectrum $E_θ(k)$ however exhibits dual branches consisting of $k^{-2}$ and $k^0$ spectra; the $k^{-2}$ branch corresponds to the Fourier modes $\hatθ(0,0,2n)$, which are approximately $-1/(2n π)$. The scaling relations for Prandtl number beyond $10^2$ match with those for infinite Prandtl number.

physics.flu-dyn↗

Entropy and energy spectra in low-Prandtl-number convection with rotation

We present results for entropy and kinetic energy spectra computed from direct numerical simulations for low-Prandtl-number ($Pr < 1$) turbulent flow in Rayleigh-Bénard convection with uniform rotation about a vertical axis. The simulations are performed in a three-dimensional periodic box for a range of Taylor number ($ 0 \leq Ta \leq 10^8$) and reduced Rayleigh number $r = Ra/Ra_{\circ} (Ta, Pr)$ ($1.0 \times 10^2 \le r \le 5.0 \times 10^3$). The Rossby number $Ro$ varies in the range $1.34 \le Ro \le 73$. The entropy spectrum $E_θ(k)$ shows bi-splitting into two branches for lower values of wave number $k$. The entropy in the lower branch scales with $k$ as $k^{-1.4\pm 0.1}$ for $r > 10^3$ for the rotation rates considered here. The entropy in the upper branch also shows scaling behavior with $k$, but the scaling exponent decreases with increasing $Ta$ for all $r$. The energy spectrum $E_v(k)$ is also found to scale with the wave number $k$ as $k^{-1.4\pm 0.1}$ for $r > 10^3$. The scaling exponent for the energy spectrum and the lower branch of the entropy spectrum vary between $-1.7$ to $-2.4$ for lower values of $r$ ($< 10^3$). We also provide some simple arguments based on the variation of the Kolmogorov picture to support the results of simulations.

physics.flu-dyn↗