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arXiv2013

Crystals, magnetic and electronic properties of a new ThCr2Si2-type BaMn2Bi2 and K-doped compositions

This is a report on the new 122 ternary transition-metal pnictide of BaMn2Bi2, which is crystallized from bismuth flux. BaMn2Bi2 adopts ThCr2Si2-type structure (I4/mmm) with a = 4.4902(3) Å and c = 14.687(1) Å; it is antiferromagnetic with anisotropic magnetic susceptibility and semiconducting with a band gap of Eg = 6 meV. Heat capacity result confirms the insulating ground state in BaMn2Bi2 with the electronic residual Sommerfeld coefficient of γ ~ 0. The high temperature magnetization results show that magnetic ordering temperature is TN ~ 400 K. Hole-doping in BaMn2Bi2 via potassium in Ba1-xKxMn2Bi2 results in metallic behavior for x = 0.10(1), 0.32(1) and 0.36(1). With K-doping, more magnetically anisotropic behavior is observed. Although there is a downturn in electrical resistivity and low-field magnetization data below 4 K in > 30%-doped crystals, there is no sign of zero resistance or diamagnetism. This manuscript is a report on new materials of BaMn2Bi2 and Ba1-xKxMn2Bi2 (0 < x < 0.4). Results from powder X-ray diffraction, anisotropic temperature- and field-dependent magnetization, temperature-and field-dependent electrical resistivity, and heat capacity are presented.

cond-mat.supr-con↗

arXiv2006

Dynamics of rotating Bose-Einstein condensates probed by Bragg scattering

Gaseous Bose-Einstein condensates (BECs) have become an important test bed for studying the dynamics of quantized vortices. In this work we use two-photon Doppler sensitive Bragg scattering to study the rotation of sodium BECs. We analyze the microscopic flow field and present laboratory measurements of the coarse-grained velocity profile. Unlike time-of-flight imaging, Bragg scattering is sensitive to the direction of rotation and therefore to the phase of the condensate. In addition, we have non-destructively probed the vortex flow field using a sequence of two Bragg pulses.

cond-mat.other↗

arXiv2013

Monopoles, confinement and charge localization in the t-J model with dilute holes

We present a quantum field theoretic description on the t$-$J model on a square lattice with dilute holes (i.e. near half-filling), based on the compact mutual Chern-Simons gauge theory. We show that, due to the presence of non-perturbative monopole plasma configuration from the antiferromagnetic background, holons (carrying electric charge) are linearly confined and strongly localized even without extrinsic disorder taken into account. Accordingly, the translation symmetry is spontaneously broken at ground state. Such an exotic localization is distinct from Anderson localization and essentially rooted in intrinsic Mott physics of the t$-$J model. Finally, a finite-temperature phase diagram is proposed. The metal-insulator transition observed in in-plane resistivity measurement is identified to a confinement-deconfinement transition from the perspective of gauge theory. The transition is characterized by the order parameter "Polyakov-line".

cond-mat.str-el↗

arXiv2013

Minimum model and its theoretical analysis for superconducting materials with BiS$_2$ layers

We perform first principles band calculation of the newly discovered superconductor LaO$_{1-x}$F$_x$BiS$_2$, and study the lattice structure and the fluorine doping dependence of the gap between the valence and conduction bands. We find that the distance between La and S as well as the fluorine doping significantly affects the band gap. On the other hand, the four orbital model of the BiS$_2$ layer shows that the lattice structure does not affect this portion of the band. Still, the band gap can affect the carrier concentration in the case of light electron doping, which in turn should affect the transport properties.

cond-mat.supr-con↗

arXiv2013

BaFe2As2/Fe bilayers with [001]-tilt grain boundary on MgO and SrTiO3 bicrystal substrates

Co-doped BaFe2As2 (Ba-122) can be realized on both MgO and SrTiO3 bicrystal substrates with [001]-tilt grain boundary by employing Fe buffer layers. However, an additional spinel (i.e. MgAl2O4) buffer between Fe and SrTiO3 is necessary since an epitaxial, smooth surface of Fe layer can not be grown on bare SrTiO3. Both types of bicrystal films show good crystalline quality.

cond-mat.supr-con↗

arXiv2017

Heavy-Fermion Superconductivity in CeAg$_2$Si$_2$ --Interplay of Spin and Valence Fluctuations--

We present the pressure-temperature phase diagram of the antiferromagnet CeAg$_2$Si$_2$ established via resistivity and calorimetry measurements under quasi-hydrostatic conditions up to 22.5~GPa. With increasing pressure, the Néel temperature [$T_{\mathrm{N}}(p=0)=8.6$~K] slowly increases up to $T_{\mathrm{N}}=13.4$~K at 9.4~GPa and then vanishes abruptly at the magnetic critical pressure $p_{\mathrm{c}}\sim13$~GPa. For the first time, heavy fermion superconductivity is observed in CeAg$_2$Si$_2$ . Superconductivity emerges at $\sim 11$~GPa and persists over roughly 10~GPa. Partial- and bulk-transition temperatures are highest at $p=16$~GPa, with a maximal $T_{\mathrm{c}^{\rm bulk}}=1.25$~K. In the pressure region of superconductivity, Kondo and crystal-field splitting energies become comparable and resistivity exhibits clear signatures of a Ce-ion valence crossover. The crossover line is located at a rapid collapse in resistivity as function of pressure and extrapolates to a valence transition critical endpoint at critical pressure and temperature of $p_{\rm cr}\sim 17$~GPa and $T_{\rm cr}\sim-13~K$, respectively. Both critical spin and valence fluctuations may build up superconductivity in CeAg$_2$Si$_2$.

cond-mat.str-el↗

arXiv2012

Synchronization of Josephson oscillations in mesa array of BSCCO single crystal through the Josephson plasma waves in base crystal

Using mesa array of $\rm{Bi_{2}Sr_{2}CaCu_{2}O_{8}}$ single crystal was demonstrated recently as a promising route to enhance the radiation power generated by Josephson oscillations in mesas. We study the synchronization in such an array via the plasma waves in the base crystal. First, we analyze plasma oscillations inside the base crystal generated by the synchronized mesa array and the associated dissipation. We then solve the dynamic equation for superconducting phase numerically to find conditions for synchronization and to check the stability of synchronized state. We find that mesas are synchronized when the cavity resonance of mesas matches with that of the base crystal. An optimal configuration of mesa arrays is also obtained.

cond-mat.supr-con↗

arXiv2018

Interplay between charge order and superconductivity in cuprate superconductors

One of the central issues in the recent study of cuprate superconductors is the interplay of charge order with superconductivity. Here the interplay of charge order with superconductivity in cuprate superconductors is studied based on the kinetic-energy-driven superconducting (SC) mechanism by taking into account the intertwining between the pseudogap and SC gap. It is shown that the appearance of the Fermi pockets is closely associated with the emergence of the pseudogap. However, the distribution of the spectral weight of the SC-state quasiparticle spectrum on the Fermi arc, or equivalently the front side of the Fermi pocket, and back side of Fermi pocket is extremely anisotropic, where the most part of the spectral weight is located around the tips of the Fermi arcs, which in this case coincide with the hot spots on the electron Fermi surface (EFS). In particular, as charge order in the normal-state, this EFS instability drives charge order in the SC-state, with the charge-order wave vector that is well consistent with the wave vector connecting the hot spots on the straight Fermi arcs. Furthermore, this charge-order state is doping dependent, with the charge-order wave vector that decreases in magnitude with the increase of doping. Although there is a coexistence of charge order and superconductivity, this charge order antagonizes superconductivity. The results from the SC-state dynamical charge structure factor indicate the existence of a quantitative connection between the low-energy electronic structure and collective response of the electron density. The theory also shows that the pseudogap and charge order have a root in common, they and superconductivity are a natural consequence of the strong electron correlation.

cond-mat.supr-con↗

arXiv2000

Hole superconductivity from kinetic energy gain

The apparently unrelated experimental observations of optical sum rule violation[1] and of tunneling asymmetry in NIS tunneling[2] find a simple explanation within the theory of hole superconductivity. In fact, both phenomena were predicted by the theory long before they were experimentally observed[3,4]. Other experimental predictions of the theory, in particular a novel feature expected in photoemission experiments, are discussed.

cond-mat.supr-con↗

arXiv2013

Bounding the pseudogap with a line of phase transitions in YBCO cuprate superconductors

Close to optimal doping, the copper oxide superconductors show 'strange metal' behavior, suggestive of strong fluctuations associated with a quantum critical point. Such a critical point requires a line of classical phase transitions terminating at zero temperature near optimal doping inside the superconducting 'dome'. The underdoped region of the temperature-doping phase diagram from which superconductivity emerges is referred to as the 'pseudogap' because evidence exists for partial gapping of the conduction electrons, but so far there is no compelling thermodynamic evidence as to whether the pseudogap is a distinct phase or a continuous evolution of physical properties on cooling. Here we report that the pseudogap in YBCO cuprate superconductors is a distinct phase, bounded by a line of phase transitions. The doping dependence of this line is such that it terminates at zero temperature inside the superconducting dome. From this we conclude that quantum criticality drives the strange metallic behavior and therefore superconductivity in the cuprates.

cond-mat.supr-con↗

arXiv2013

Suppression of the radiative decay of atomic coherence in squeezed vacuum

Quantum fluctuations of the electromagnetic vacuum are responsible for physical effects such as the Casimir force and the radiative decay of atoms, and set fundamental limits on the sensitivity of measurements. Entanglement between photons can produce correlations that result in a reduction of these fluctuations below the vacuum level allowing measurements that surpass the standard quantum limit in sensitivity. Here we demonstrate that the radiative decay rate of an atom that is coupled to quadrature squeezed electromagnetic vacuum can be reduced below its natural linewidth. We observe a two-fold reduction of the transverse radiative decay rate of a superconducting artificial atom coupled to continuum squeezed vacuum generated by a Josephson parametric amplifier, allowing the transverse coherence time T_2 to exceed the vacuum decay limit of 2T_1. We demonstrate that the measured radiative decay dynamics can be used to tomographically reconstruct the Wigner distribution of the the itinerant squeezed state. Our results are the first confirmation of a canonical prediction of quantum optics and open the door to new studies of the quantum light-matter interaction.

quant-ph↗

arXiv2013

Exciting Andreev pairs in a superconducting atomic contact

The Josephson effect describes the flow of supercurrent in a weak link, such as a tunnel junction, nanowire, or molecule, between two superconductors. It is the basis for a variety of circuits and devices, with applications ranging from medicine to quantum information. Currently, experiments using Josephson circuits that behave like artificial atoms are revolutionizing the way we probe and exploit the laws of quantum physics. Microscopically, the supercurrent is carried by Andreev pair states, which are localized at the weak link. These states come in doublets and have energies inside the superconducting gap. Existing Josephson circuits are based on properties of just the ground state of each doublet and so far the excited states have not been directly detected. Here we establish their existence through spectroscopic measurements of superconducting atomic contacts. The spectra, which depend on the atomic configuration and on the phase difference between the superconductors, are in complete agreement with theory. Andreev doublets could be exploited to encode information in novel types of superconducting qubits.

cond-mat.mes-hall↗

arXiv2013

Heavy Solitons in a Fermionic Superfluid

Topological excitations are found throughout nature, in proteins and DNA, as dislocations in crystals, as vortices and solitons in superfluids and superconductors, and generally in the wake of symmetry-breaking phase transitions. In fermionic systems, topological defects may provide bound states for fermions that often play a crucial role for the system's transport properties. Famous examples are Andreev bound states inside vortex cores, fractionally charged solitons in relativistic quantum field theory, and the spinless charged solitons responsible for the high conductivity of polymers. However, the free motion of topological defects in electronic systems is hindered by pinning at impurities. Here we create long-lived solitons in a strongly interacting fermionic superfluid by imprinting a phase step into the superfluid wavefunction, and directly observe their oscillatory motion in the trapped superfluid. As the interactions are tuned from the regime of Bose-Einstein condensation (BEC) of tightly bound molecules towards the Bardeen-Cooper-Schrieffer (BCS) limit of long-range Cooper pairs, the effective mass of the solitons increases dramatically to more than 200 times their bare mass. This signals their filling with Andreev states and strong quantum fluctuations. For the unitary Fermi gas, the mass enhancement is more than fifty times larger than expectations from mean-field Bogoliubov-de Gennes theory. Our work paves the way towards the experimental study and control of Andreev bound states in ultracold atomic gases. In the presence of spin imbalance, the solitons created here represent one limit of the long sought-after Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state of mobile Cooper pairs.

cond-mat.quant-gas↗

arXiv2013

Realization of Deterministic Quantum Teleportation with Solid State Qubits

Transferring the state of an information carrier from a sender to a receiver is an essential primitive in both classical and quantum communication and information processing. In a quantum process known as teleportation the unknown state of a quantum bit can be relayed to a distant party using shared entanglement and classical information. Here we present experiments in a solid-state system based on superconducting quantum circuits demonstrating the teleportation of the state of a qubit at the macroscopic scale. In our experiments teleportation is realized deterministically with high efficiency and achieves a high rate of transferred qubit states. This constitutes a significant step towards the realization of repeaters for quantum communication at microwave frequencies and broadens the tool set for quantum information processing with superconducting circuits.

quant-ph↗

arXiv2013

Emergence of charge order from the vortex state of a high temperature superconductor

Evidence is mounting that charge order competes with superconductivity in high Tc cuprates. Whether this has any relationship to the pairing mechanism is unknown since neither the universality of the competition nor its microscopic nature has been established. Here using nuclear magnetic resonance, we show that, similar to La214, charge order in YBCO has maximum strength inside the superconducting dome, at doping levels p = 0.11 - 0.12.We further show that the overlap of halos of incipient charge order around vortex cores, similar to those visualised in Bi2212, can explain the threshold magnetic field at which long-range charge order emerges. These results reveal universal features of a competition in which charge order and superconductivity appear as joint instabilities of the same normal state, whose relative balance can be field-tuned in the vortex state.

cond-mat.supr-con↗

arXiv2013

Quantum Criticality in Electron-doped BaFe_{2-x}Ni_xAs_2

A quantum critical point (QCP) is a point in a system's phase diagram at which an order is completely suppressed at absolute zero temperature (T). The presence of a quantum critical point manifests itself in the finite-T physical properties, and often gives rise to new states of matter. Superconductivity in the cuprates and in heavy fermion materials is believed by many to be mediated by fluctuations associated with a quantum critical point. In the recently-discovered iron-pnictide high temperature superconductors, it is unknown whether a QCP exists or not in a carrier-doped system. Here we report transport and nuclear magnetic resonance (NMR) measurements on BaFe_{2-x}Ni_xAs_2 (0 =< x =< 0.17). We find two critical points at x_{c1} = 0.10 and x_{c2} = 0.14. The electrical resistivity follows ρ= ρ_0 + A*T^n, with n = 1 around x_{c1} and another minimal n = 1.1 at x_{c2}. By NMR measurements, we identity x_{c1} to be a magnetic QCP and suggest that x_{c2} is a new type of QCP associated with a nematic structural phase transition. Our results suggest that the superconductivity in carrier-doped pnictides is closely linked to the quantum criticality.

cond-mat.supr-con↗

arXiv2013

A Strained Organic Field-Effect-Transistor with a Gate-Tunable Superconducting Channel

In state-of-the-art silicon devices, mobility of the carrier is enhanced by the lattice strain from the back substrate. Such an extra control of device performance is significant in realizing high performance computing and should be valid for electric-field-induced superconducting devices, too. However, so far, the carrier density is the sole parameter for field-induced superconducting interfaces. Here we show an active organic superconducting field-effect-transistor whose lattice is modulated by the strain from the substrate. The soft organic lattice allows tuning of the strain by a choice of the back substrate to make an induced superconducting state accessible at low temperature with a paraelectric solid gate. An active three terminal Josephson junction device thus realized is useful both in advanced computing and in elucidating a direct connection between filling-controlled and bandwidth-controlled superconducting phases in correlated materials.

cond-mat.supr-con↗

arXiv2013

Artificially engineered superlattices of pnictide superconductor

Significant progress has been achieved in fabricating high quality bulk and thinfilm iron-based superconductors. In particular, artificial layered pnictide superlattices offer the possibility of tailoring the superconducting properties and understanding the mechanism of the superconductivity itself. For high field applications, large critical current densities (Jc) and irreversibility fields (Hirr) are indispensable along all crystal directions. On the other hand, the development of superconducting devices such as tunnel junctions requires multilayered heterostructures. Here we show that artificially engineered undoped Ba-122 / Co doped Ba-122 compositionally modulated superlattices produce ab-aligned nanoparticle arrays. These layer and self-assemble along c-axis aligned defects, and combine to produce very large Jc and Hirr enhancements over a wide angular range. We also demonstrate a structurally modulated SrTiO3 (STO) / Co doped Ba-122 superlattice with sharp interfaces. Success in superlattice fabrication involving pnictides will aid the progress of heterostructured systems exhibiting novel interfacial phenomena and device applications.

cond-mat.supr-con↗