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arXiv · 1005.4856

Disappearance of static magnetic order and evolution of spin fluctuations in Fe$_{1+δ}$Se$_{x}$Te$_{1-x}$

Zhijun Xu·Jinsheng Wen·Guangyong Xu·Qing Jie·Zhiwei Lin·Qiang Li·Songxue Chi·D. K. Singh·Genda Gu·J. M. Tranquada
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Abstract

We report neutron scattering studies on static magnetic orders and spin excitations in the Fe-based chalcogenide system Fe$_{1+δ}$Se$_{x}$Te$_{1-x}$ with different Fe and Se compositions. Short-range static magnetic order with the "bicollinear" spin configuration is found in all non-superconducting samples, with strong low-energy magnetic excitations near the $(0.5,0)$ in-plane wave-vector (using the two-Fe unit cell) for Se doping up to 45%. When the static order disappears and bulk superconductivity emerges, the spectral weight of the magnetic excitations shifts to the region of reciprocal space near the in-plane wave-vector $(0.5,0.5)$, corresponding to the "collinear" spin configuration. Our results suggest that spin fluctuations associated with the collinear magnetic structure appear to be universal in all Fe-based superconductors, and there is a strong correlation between superconductivity and the character of the magnetic order/fluctuations in

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Zhijun Xu, Jinsheng Wen, Guangyong Xu, Qing Jie, Zhiwei Lin, Qiang Li, Songxue Chi, D. K. Singh, Genda Gu, J. M. Tranquada. 2010-05-26. Disappearance of static magnetic order and evolution of spin fluctuations in Fe$_{1+δ}$Se$_{x}$Te$_{1-x}$. https://doi.org/10.1103/physrevb.82.104525

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