SearcharxivSearch

arXiv · 1011.4875

Diamagnetism, Nernst signal, and finite size effects in superconductors above the transition temperature

Abstract

Various superconductors, including cuprate superconductors, exhibit peculiar features above the transition temperature T_c. In particular the observation of a large diamagnetism and Nernst signal in a wide temperature window above T_c attracted considerable attention. Noting that this temperature window exceeds the fluctuation dominated regime drastically and that in these materials the spatial extent of homogeneity is limited, we explore the relevance of the zero dimensional (0D)-model, neglecting thermal fluctuations. It is shown that both, the full 0D-model as well as its Gaussian approximation, mimic the essential features of the isothermal magnetization curves in Pb nanoparticles and various cuprates remarkably well. This analysis also provides estimates for the spatial extent of the homogeneous domains giving rise to a smeared transition in zero magnetic field. The resulting estimates for the amplitude of the in-plane correlation length exhibit a doping dependence reflecting the flow to the quantum phase transition in the underdoped limit. Furthermore it is shown that the isothermal Nernst signal of a superconducting Nb_(0.15)Si_(0.85) film is fully consistent with this scenario. Accordingly, the observed diamagnetism above T_c in Pb nanoparticles, in the cuprates La_(1.91)Sr_(0.09)CuO_4 and BiSr_2Ca_2CuO_(8-d), as well as the Nernst signal in Nb_(0.15)Si_(0.85) films, are all in excellent agreement with the scaling properties emerging from the 0D-model, giving a universal perspective on the interplay between diamagnetism, Nernst signal, correlation length, and the limited spatial extent of homogeneity. Our analysis also provides evidence that singlet Cooper pairs subjected to orbital pair breaking in a 0D system are the main source of the observed diamagnetism and Nernst signal in an extended temperature window above T_c.

Explore related subjects

Keep this discovery

BibTeXRIS

T. Schneider, S. Weyeneth. 2010-11-22. Diamagnetism, Nernst signal, and finite size effects in superconductors above the transition temperature. https://doi.org/10.1103/physrevb.83.144527

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Out-of-equilibrium relaxation dynamics of the superconducting order parameter in CsV$_3$Sb$_5$

The application of a time-varying strain field drives a superconducting order parameter out of equilibrium. How the order parameter relaxes back to equilibrium depends both on the structure of the superconducting gap and on the nature of quasiparticle scattering. We report the discovery of an ultrasonic attenuation peak inside the superconducting state of the kagome superconductor CsV$_3$Sb$_5$. This peak is the natural consequence of the order parameter relaxation time matching the ultrasonic drive frequency near $T_{\rm c}$. From the measured frequency dependence of the peak, we extract a microscopic scattering time of $\tau_N = 25$ ps. This timescale is two orders of magnitude longer than the elastic scattering time as determined by resistivity measurements, but is comparable to the inelastic scattering time determined by thermal transport. Within the conventional framework of order-parameter relaxation, this implies that elastic scattering is ineffective at relaxing the superconducting condensate, consistent with a sign-preserving $s$-wave state obeying Anderson's theorem.

cond-mat.supr-con

Eight-unit-cell electronic modulations in cuprates originating from local molecular orbitals

The pair density wave (PDW) state with eight-unit-cell (8a0) periodicity has been widely regarded as the primary order in cuprates, yet its existence and origin remain subjects of intense debate. Using spectroscopic imaging scanning tunneling microscopy, we observe spatial modulations of the electronic states with approximately 8a0 periodicity in both the superconducting and insulating regimes of hole-doped Ca2CuO2Cl2 cuprate. We find that the 8a0 spatial patterns are generated by the formation of molecular orbitals by doped holes, which organize into 4a0*4a0 plaquettes as the basic unit. Our results identify the 4a0 molecular orbital as the fundamental electronic building block in cuprates, while the 8a0 PDW represents a spatial subharmonic that emerges at sufficiently high doping.

cond-mat.supr-con

Record-Breaking Elemental Superconductivity in Tetralayer Kagome Borophene

Superconductivity above the liquid-nitrogen temperature remains rare in two-dimensional elemental crystals, where strong covalent bonding often yields high phonon frequencies but insufficient electron-phonon coupling. Here, using first-principles calculations and fully anisotropic Migdal-Eliashberg theory, we predict tetralayer kagome borophene (TKB) stabilized by ABAB covalent stacking, as a liquid-nitrogen-temperature elemental superconductor. With a predicted critical temperature of 102 K, TKB sets a record-high value among previously reported elemental superconductors. Unlike known high-Tc boron-based superconductors dominated by in-plane sigma-bonding states and high-frequency in-plane B-B stretching modes, TKB realizes an out-of-plane s-pz-bonding-mediated pairing mechanism, in which interlayer s-pz bonding states at the Fermi level are strongly coupled to low-frequency out-of-plane vibrations of boron atoms. These results reveal a distinct out-of-plane pairing channel in multilayer borophene and establish covalent stacking engineering as a potential route for high-Tc superconductivity in two-dimensional materials.

cond-mat.supr-con