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S. Weyeneth

Publications and source records attributed to S. Weyeneth.

At least 19 recordsLinked to original sources

Oxygen Isotope Effect Resulting from Polaron-induced Superconductivity in Cuprates

The planar oxygen isotope effect coefficient measured as a function of hole doping in the Pr- and La-doped YBa2Cu3O7 (YBCO) and the Ni-doped La1.85Sr0.15CuO4 (LSCO) superconductors quantitatively and qualitatively follows the form originally proposed by Kresin and Wolf, which was derived for polarons perpendicular to the superconducting planes. Interestingly, the inverse oxygen isotope effect coefficient at the pseudogap temperature also follows the same formula. These findings allow the conclusion that the superconductivity in YBCO and LSCO results from polarons or rather bipolarons in the CuO2 plane. The original formula, proposed for the perpendicular direction only, is obviously more generally valid and accounts for the superconductivity in the CuO2 planes.

cond-mat.supr-con

Suppression of the Berezinskii-Kosterlitz-Thouless and Quantum Phase Transitions in 2D Superconductors by Finite Size Effects

We perform a detailed finite-size scaling analysis of the sheet resistance in Bi-films and the LaAlO$_{3}$/SrTiO$_{3}$ interface in the presence and absence of a magnetic field applied perpendicular to the system. Our main aim is to explore the occurrence of Berezinskii-Kosterlitz-Thouless (BKT) and quantum phase transition behavior in the presence of limited size, stemming from the finite extent of the homogeneous domains or the magnetic field. Moreover we explore the implications thereof. Above an extrapolated BKT transition temperature, modulated by the thickness $d$, gate voltage $%V_{g}$ or magnetic field $H$, we identify a temperature range where BKT behavior occurs. Its range is controlled by the relevant limiting lengths,which are set by the extent of the homogeneous domains or the magnetic field. The extrapolated BKT transition lines $T_{c}\left(d,V_{g},H\right) $ uncover compatibility with the occurrence of a quantum phase transition where $T_{c}\left( d_{c},V_{gc},H_{c}\right) =0$. However, an essential implication of the respective limiting length is that the extrapolated phase transition lines $T_{c}\left( d,V_{g},H\right) $ are unattainable. Consequently, given a finite limiting length, BKT and quantum phase transitions do not occur. Nevertheless, BKT and quantum critical behavior is observable, controlled by the extent of the relevant limiting length. Additional results and implications include: the magnetic field induced finite size effect generates a flattening out of the sheet resistance in the $T\rightarrow 0$ limit, while in zero field it exhibits a characteristic temperature dependence and vanishes at $T=0$ only. The former prediction is confirmed in both, the Bi-films and the LaAlO$_{3}$/SrTiO$_{3}$ interface, as well as in previous studies. The latter is consistent with the LaAlO$_{3}$/SrTiO$_{3}$ interface data, while the Bi-films exhibit a flattening out.

cond-mat.supr-con

L4Fe2As2Te1-xO4-yFy (L = Pr, Sm, Gd): a layered oxypnictide superconductor with Tc up to 45 K

The synthesis, structural and physical properties of iron lanthanide oxypnictide superconductors, L4Fe2As2Te1-xO4 (L = Pr, Sm, Gd), with transition temperature at ~ 25 K are reported. Single crystals have been grown at high pressure using cubic anvil technique. The crystal structure consists of layers of L2O2 tetrahedra separated by alternating layers of chains of Te and of Fe2As2 tetrahedra: -L2O2-Te-L2O2-Fe2As2-L2O2-Te-L2O2- (space group: I4/mmm, a ~ 4.0, c ~ 29.6 Å). Substitution of oxygen by fluorine increases the critical temperature, e.g. in Gd4Fe2As2Te1-xOyF4-y up to 45 K. Magnetic torque measurements reveal an anisotropy of the penetration depths of ~31.

cond-mat.supr-con

Gate voltage tuned quantum superconductor to insulator transition in an ultrathin bismuth film revisited

We explore the implications of Berezinskii-Kosterlitz-Thouless (BKT) critical behavior and variable-range hopping on the two dimensional (2D) quantum superconductor-insulator (QSI) transition driven by tuning the gate voltage. To illustrate the potential and the implications of this scenario we analyze sheet resistance data of Parendo et al. taken on a gate voltage tuned ultrathin amorphous bismuth film. The finite size scaling analysis of the BKT-transition uncovers a limiting length preventing the correlation length to diverge and to enter the critical regime deeply. Nevertheless the attained BKT critical regime reveals consistency with two parameter quantum scaling and an explicit quantum scaling function determined by the BKT correlation length. The two parameter scaling yields for the zero temperature critical exponents of the QSI-transition the estimates zn = 3/2, z = 3, and n = 1/2, revealing that hyperscaling is violated and in contrast to finite temperature disorder is relevant at zero temperature. Furthermore, zn = 3/2 is also consistent with the two variable quantum scaling form associated with a variable-range hopping controlled insulating ground state.

cond-mat.supr-con

Conventional superconductivity and hysteretic Campbell penetration depth in single crystals MgCNi$_3$

Single crystals of MgCNi$_3$, with areas sized up to 1 mm$^{2}$, were grown by the self flux method using a cubic anvil high pressure technique. The first critical field \textit{H$_{c1}$}, determined from a zero temperature extrapolation, is around 18 mT. Using the tunnel - diode resonator technique, the London penetration depth was measured with no applied \textit{dc} field and the Campbell penetration depth was measured with the external \textit{dc} fields up to 9T for two different sample orientations with respect to the direction of applied magnetic field. The absolute value of the London penetration depth, $λ(0) = 245 \pm 10$ nm was determined from the thermodynamic Rutgers formula. The superfluid density, $ρ_s=(λ(0)/λ(T))^2$ was found to follow the clean isotropic \textit{s}-wave behavior predicted by the weak - coupling BCS theory in the whole temperature range. The low - temperature behavior of the London penetration depth fits the BCS analytic form as well and produces close to the weak - coupling value of $Δ(0)/k_BT_c = 1.71$. The temperature dependence of the upper critical field, \textit{$H_{c2}$}, was found to be isotropic with a slope at \textit{T$_c$} of -2.63 T/K and \textit{H$_{c2}$}(0) $\approx$ 12.3 T at zero temperature. The Campbell penetration depth probes the vortex lattice response in the mixed state and is sensitive to the details of the pinning potential. For MgCNi$_3$, an irreversible feature has been observed in the TDR response when the sample is field-cooled and warmed versus zero-field-cooled and warmed. This feature possesses a non-monotonic field dependence and has commonly been referred to as the peak effect and is most likely related to a field - dependent non - parabolic pinning potential.

cond-mat.supr-con

High-pressure flux growth, structural, and superconducting properties of LnFeAsO (Ln = Pr, Nd, Sm) single crystals

Single crystals of the LnFeAsO (Ln1111, Ln = Pr, Nd, and Sm) family with lateral dimensions up to 1 mm were grown from NaAs and KAs flux at high pressure. The crystals are of good structural quality and become superconducting when O is partially substituted by F (PrFeAsO1-xFx and NdFeAsO1-xFx) or when Fe is substituted by Co (SmFe1-xCoxAsO). From magnetization measurements, we estimate the temperature dependence and anisotropy of the upper critical field and the critical current density of underdoped PrFeAsO0.7F0.3 crystal with Tc = 25 K. Single crystals of SmFe1-xCoxAsO with maximal Tc up to 16.3 K for x = 0.08 were grown for the first time. From transport and magnetic measurements we estimate the critical fields and their anisotropy, and find these superconducting properties to be quite comparable to the ones in SmFeAsO1-xFx with a much higher Tc of = 50 K. The magnetically measured critical current densities are as high as 109 A/m2 at 2 K up to 7 T, with indication of the usual fishtail effect. The upper critical field estimated from resistivity measurements is anisotropic with slopes of -8.7 T/K (H // ab-plane) and -1.7 T/K (H // c-axis). This anisotropy (= 5) is similar to that in other Ln1111 crystals with various higher Tc s.

cond-mat.supr-con

Quantum superconductor-insulator transition: Implications of BKT-critical behavior

We explore the implications of Berezinskii-Kosterlitz-Thouless (BKT) critical behavior on the two dimensional (2D) quantum superconductor-insulator (QSI) transition driven by the tuning parameter x. Concentrating on the sheet resistance R(x) BKT behavior implies: an explicit quantum scaling function for R(x) along the superconducting branch ending at the nonuniversal critical value R_c=R(x_c); a BKT-transition line T_c(x) that is proportional to (x-x_c)^(z*nu) where z is the dynamic and nu the exponent of the zero temperature correlation length; independent estimates of z*nu, z and nu from the x dependence of the nonuniversal parameters entering the BKT expression for the sheet resistance. To illustrate the potential and the implications of this scenario we analyze data of Bollinger et al. taken on gate voltage tuned epitaxial films of La_(2-x)Sr_xCuO_4 that are one unit cell thick. The resulting estimates z=2.35 and nu=0.63 point to a 2D-QSI critical point where hyperscaling, the proportionality between d/λ^2(0) and T_c, and the correspondence between quantum phase transitions in D and classical ones in (D+z) dimensions are violated and disorder is relevant.

cond-mat.supr-con

Superconductivity and magnetism in RbxFe2-ySe2: Impact of thermal treatment on mesoscopic phase separation

An extended study of the superconducting and normal-state properties of various as-grown and post-annealed RbxFe2-ySe2 single crystals is presented. Magnetization experiments evidence that annealing of RbxFe2-ySe2 at 413 K, well below the onset of phase separation Tp=489 K, neither changes the magnetic nor the superconducting properties of the crystals. In addition, annealing at 563 K, well above Tp, suppresses the superconducting transition temperature Tc and leads to an increase of the antiferromagnetic susceptibility accompanied by the creation of ferromagnetic impurity phases, which are developing with annealing time. However, annealing at T=488K=Tp increases Tc up to 33.3 K, sharpens the superconducting transition, increases the lower critical field, and strengthens the screening efficiency of the applied magnetic field. Resistivity measurements of the as-grown and optimally annealed samples reveal an increase of the upper critical field along both crystallographic directions as well as its anisotropy. Muon spin rotation and scanning transmission electron microscopy experiments suggest the coexistence of two phases below Tp: a magnetic majority phase of Rb2Fe4Se5 and a non-magnetic minority phase of Rb0.5Fe2Se2. Both microscopic techniques indicate that annealing the specimens just at Tp does not affect the volume fraction of the two phases, although the magnetic field distribution in the samples changes substantially. This suggests that the microstructure of the sample, caused by mesoscopic phase separation, is modified by annealing just at Tp, leading to an improvement of the superconducting properties of RbxFe2-ySe2 and an enhancement of Tc.

cond-mat.supr-con

Pressure induced ferromagnetism in antiferromagnetic Fe_1.03Te

The magnetic properties of Fe1.03Te under hydrostatic pressure up to p ~ 5.7 GPa were investigated by means of muon spin rotation, dc magnetization, and neutron depolarization measurements. With increasing pressure the antiferromagnetic ordering temperature TN decreases continuously from 70 K at ambient pressure towards higher pressures. Surprisingly, the commensurate antiferromagnetic order of FeTe enters a region of incommensurate and dynamical magnetic order before at p ~ 1.7 GPa the system turns ferromagnetic. The ferromagnetic ordering temperature TC increases with increasing pressure.

cond-mat.supr-con

Vortex lock-in transition coinciding with the 3D to 2D crossover in YBa2Cu3O7

A vortex lock-in transition was directly detected by torque magnetometry in an overdoped YBa2Cu3O7 single crystal of low anisotropy (\approx 7). The locked-in state was observed below the 3D to 2D crossover temperature Tcr = 76 K, independently of extrinsic pinning effects thanks to a high quality clean crystal and the use of a vortex shaking technique. The shape of the torque signal as a function of the angle between the applied magnetic field and the crystallographic c-axis is in very good agreement with the model developped by Feinberg and Ettouhami [Int. J. Mod. Phys. B 7, 2085 (1993)] for quasi-2D superconductors, despite the low anisotropy of the material.

cond-mat.supr-con

Magnetic-field tuned anisotropy in superconducting Rb(x)Fe(2-y)Se(2)

The anisotropic superconducting properties of a Rb(x)Fe(2-y)Se(2) single crystal with transition temperature 32 K were investigated by means of SQUID and torque magnetometry, probing the effective magnetic penetration depth and the magnetic penetration depth anisotropy. Interestingly, the anisotropy is found to be temperature independent in the superconducting state, but strongly field dependent. This unusual anisotropic behavior, together with a large zero-temperature effective magnetic penetration depth is possibly related to a superconducting state heavily biased by the coexisting antiferromagnetic phase.

cond-mat.supr-con

Study of the anisotropic magnetic order of the Eu sublattice in single crystals of EuFe_2-xCo_xAs_2 (x = 0, 0.2) by means of magnetization and magnetic torque

Here, we present a combination of magnetization and magnetic torque experiments to investigate the magnetic orders in undoped EuFe2As2 and Co doped EuFe1.8Co0.2As2 single crystals. Although at low temperatures typical results for an antiferromagnetic (AFM) state in EuFe2As2 were found, our data strongly indicate the occurrence of a canted antiferromagnetic (C-AFM) order of the Eu2+ moments between 17 K and 19 K, observed even in the lowest studied magnetic fields. However, unlike in the parent compound, no low-field and low-temperature AFM state of the Eu^2+ moments was observed in the doped EuFe1.8Co0.2As2. Only a C-AFM phase is present at low fields and low temperatures, with a reduced magnetic anisotropy as compared to the undoped system. We present and discuss for both, EuFe2As2 and EuFe1.8Co0.2As2, the experimentally deduced magnetic phase diagrams of the magnetic ordering of the Eu^2+ sublattice with respect to the temperature, the applied magnetic field, and its orientation to the crystallographic axes. It is likely that the magnetic coupling of the Eu and the Fe sublattice is strongly depending on Co doping, having detrimental influence on the magnetic phase diagrams as determined in this work. Their impact on the occurrence of superconductivity with higher Co doping is discussed.

cond-mat.supr-con

Study of the mixed state of La_{1.83}Sr_{0.17}CuO_{4} by means of muon-spin rotation and magnetization experiments in a low magnetic field

Muon-spin rotation (muSR) experiments are often used to study the magnetic field distribution in type-II superconductors in the vortex state. Based on the determination of the magnetic penetration depth it is frequently speculated---also controversially---about the order-parameter symmetry of the studied superconductors. This article reports on a combined muSR and magnetization study of the mixed state in the cuprate high-temperature superconductor La_{1.83}Sr_{0.17}CuO_{4} in a low magnetic field of 20 mT applied along the c axis of a single crystal. The macroscopic magnetization measurements reveal substantial differences for various cooling procedures. Yet, indicated changes in the vortex dynamics between different temperature regions as well as the results of the microscopic muSR experiments are virtually independent of the employed cooling cycles. Additionally, it is found that the mean magnetic flux density, locally probed by the muons, strongly increases at low temperatures. This can possibly be explained by a non-random sampling of the spatial field distribution of the vortex lattice in this cuprate superconductor caused by intensified vortex pinning.

cond-mat.supr-con

Observation of a first-order phase transition deep within the vortex-solid region of YBa2Cu3O7

We have investigated the magnetic phase diagram of a fully oxygenated detwinned YBa2Cu3O7 single crystal by means of magneto-caloric and magnetization measurements, and found thermodynamic evidence for a temperature dependent first-order phase-transition line deep within the vortex-solid region. The associated discontinuities in the entropy are apparently proportional to the magnetic flux density, which may hint at a structural transition of the vortex lattice.

cond-mat.supr-con

Interplay of composition, structure, magnetism, and superconductivity in SmFeAs1-xPxO1-y

Polycrystalline samples and single crystals of SmFeAs1-xPxO1-y were synthesized and grown employing different synthesis methods and annealing conditions. Depending on the phosphorus and oxygen content, the samples are either magnetic or superconducting. In the fully oxygenated compounds the main impact of phosphorus substitution is to suppress the Néel temperature TN of the spin density wave (SDW) state, and to strongly reduce the local magnetic field in the SDW state, as deduced from muon spin rotation measurements. On the other hand the superconducting state is observed in the oxygen deficient samples only after heat treatment under high pressure. Oxygen deficiency as a result of synthesis at high pressure brings the Sm-O layer closer to the superconducting As/P-Fe-As/P block and provides additional electron transfer. Interestingly, the structural modifications in response to this variation of the electron count are significantly different when phosphorus is partly substituting arsenic. Point contact spectra are well described with two superconducting gaps. Magnetic and resistance measurements on single crystals indicate an in-plane magnetic penetration depth of 200 nm and an anisotropy of the upper critical field slope of 4-5. PACS number(s): 74.70.Xa, 74.62.Bf, 74.25.-q, 81.20.-n

cond-mat.supr-con

Magnetic torque study of the temperature dependent anisotropy parameter in overdoped superconducting single-crystal YBa_2Cu_3O_7

An overdoped YBa2Cu3O7 single crystal was studied by SQUID and torque magnetometry in order to investigate the temperature dependence of the anisotropy parameter close to the transition temperature T_c (0.87 T_c < T < T_c). Angle dependent torque measurements were performed and analyzed with the widely used Kogan model [Phys. Rev. B 38, 7049 (1988)] as well as with an extended model by Hao and Clem [Phys. Rev. Lett. 67, 2371 (1991)], taking into account the influence of the vortex cores on the magnetization. Both approaches yield similar results, with an out-of-plane anisotropy parameter around 6.5 which slightly increases with decreasing temperature, and a temperature independent in-plane anisotropy parameter gamma_ab}= 1.12(5).

cond-mat.supr-con

Strong coupling between Eu2+ spins and Fe2As2 layers in EuFe1.9Co0.1As2 observed with NMR

A combination of x-ray diffraction, magnetization, and 75As nuclear magnetic resonance (NMR) experiments were performed on single-crystal EuFe1.9Co0.1As2. The strength of the hyperfine interaction between the 75As nuclei and the Eu^(2+) 4f states suggests a strong coupling between the Eu^(2+) moments and the Fe1.9Co0.1As2 layers. Such a strong interlayer coupling may be due to an indirect exchange interaction between the localized Eu^(2+) 4f moments, mediated by the Fe 3d conduction electrons. Magnetic susceptibility as well as 75As-NMR measurements reveal a decrease of the SDW transition temperature to T_SDW = 120 K as a result of Co doping. A change of the slope in the temperature dependence of the NMR frequency of the 75As lower-satellite line was observed at 225 K. At the same temperature also a change of the satellite line shape was found. These changes of the NMR spectra may be caused by the formation of a nematic phase below 225 K in EuFe1.9Co0.1As2.

cond-mat.supr-con

Coexistence of Magnetism and Superconductivity in the Iron-based Compound Cs_0.8(FeSe_0.98)_2

We report on muon-spin rotation/relaxation (\muSR), electrical resistivity, magnetization and differential scanning calorimetry measurements performed on a high-quality single crystal of Cs_0.8(FeSe_0.98)_2. Whereas our transport and magnetization data confirm the bulk character of the superconducting state below T_c = 28.5(2)K, the \muSR data indicate that the system is {\it magnetic} below T_N = 478.5(3)K, where a first-order transition occurs. The first-order character of the magnetic transition is confirmed by differential scanning calorimetry data. Taken all together, these data indicate in Cs_0.8(FeSe_0.98)_2 a microscopic coexistence between the superconducting phase and a strong magnetic phase. The observed ratio between T_N and T_c is the highest one reported to date for a magnetic superconductor.

cond-mat.supr-con