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arXiv · 1207.0921

Neutron diffraction study of spin and charge ordering in SrFeO(3-delta)

M. Reehuis·C. Ulrich·A. Maljuk·Ch. Niedermayer·B. Ouladdiaf·A. Hoser·T. Hofmann·B. Keimer
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Abstract

We report a comprehensive neutron diffraction study of the crystal structure and magnetic order in a series of single-crystal and powder samples of SrFeO$_{3-\delta}$ in the vacancy range $0 \leq \delta \leq 0.23$. The data provide detailed insights into the interplay between the oxygen vacancy order and the magnetic structure of this system. In particular, a crystallographic analysis of data on Sr8Fe8O23 revealed a structural transition between the high-temperature tetragonal and a low-temperature monoclinic phase with a critical temperature T = 75 K, which originates from charge ordering on the Fe sublattice and is associated with a metal-insulator transition. Our experiments also revealed a total of seven different magnetic structures of SrFeO$_{3-\delta}$ in this range of $\delta$, only two of which (namely an incommensurate helix state in SrFeO3 and a commensurate, collinear antiferromagnetic state in Sr4Fe4O11) had been identified previously. We present a detailed refinement of some of the magnetic ordering patterns and discuss the relationship between the magneto-transport properties of SrFeO$_{3-\delta}$ samples and their phase composition and magnetic microstructure.

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M. Reehuis, C. Ulrich, A. Maljuk, Ch. Niedermayer, B. Ouladdiaf, A. Hoser, T. Hofmann, B. Keimer. 2012-07-04. Neutron diffraction study of spin and charge ordering in SrFeO(3-delta). https://doi.org/10.1103/physrevb.85.184109

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