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arXiv · 1209.6244

Identifying the Magnetoelectric Modes of Multiferroic BiFeO$_3$

Randy S. Fishman·Nobuo Furukawa·Jason T. Haraldsen·Masaaki Matsuda·Shin Miyahara
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Abstract

We have identified three of the four magnetoelectric modes of multiferroic BiFeO$_3$ measured using THz spectroscopy. Excellent agreement with the observed peaks is obtained by including the effects of easy-axis anisotropy along the direction of the electric polarization. By distorting the cycloidal spin state, anisotropy splits the $Ψ_{\pm 1}$ mode into peaks at 20 and 21.5 cm$^{-1}$ and activates the lower $Φ_{\pm 2}$ mode at 27 cm$^{-1}$ (T=200 K). An electromagnon is identified with the upper $Ψ_{\pm 1}$ mode at 21.5 cm$^{-1}$. Our results also explain recent Raman and inelastic neutron-scattering measurements.

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Randy S. Fishman, Nobuo Furukawa, Jason T. Haraldsen, Masaaki Matsuda, Shin Miyahara. 2012-09-27. Identifying the Magnetoelectric Modes of Multiferroic BiFeO$_3$. https://doi.org/10.1103/physrevb.86.220402

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