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arXiv · 1212.1001

Electric field driven destabilization of the insulating state in nominally pure LaMnO3

Rajib Nath·A. K. Raychaudhuri·Ya. M. Mukovskii·Parthasarathi Mondal·Dipten Bhattacharya·P. Mandal
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Abstract

We report an electric field driven destabilization of the insulating state in nominally pure LaMnO3 single crystal with a moderate field which leads to a resistive state transition below 300 K. The transition is between the insulating state in LaMnO3 and a high resistance bad metallic state that has a temperature independent resistivity. The transition occurs at a threshold field (Eth) which shows a steep enhancement on cooling. While at lower temperatures the transition is sharp and involves large change in resistance but it softens on heating and eventually absent above 280K. When the Mn4+ content is increased by Sr substitution up to x=0.1, the observed transition though observable in certain temperature range, softens considerably. The observation has been explained as bias driven percolation type transition between two coexisting phases, where the majority phase is a charge and orbitally ordered polaronic insulating phase and the minority phase is a bad metallic phase. The mobile fraction f of the bad metallic phase deduced from the experimental data follows an activated kinetics with the activation energy nearly equal to 200 meV and the prefactor fo is a strong function of the field that leads to a rapid enhancement of f on application of field leading to the resistive state transition. We suggest likely scenarios for such co-existing phases in nominally pure LaMnO3 that can lead to the bias driven percolation type transition.

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Rajib Nath, A. K. Raychaudhuri, Ya. M. Mukovskii, Parthasarathi Mondal, Dipten Bhattacharya, P. Mandal. 2013-03-04. Electric field driven destabilization of the insulating state in nominally pure LaMnO3. https://doi.org/10.1088/0953-8984%2F25%2F15%2F155605

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