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arXiv · 1307.8378

Non-markovian polariton dynamics in organic strong coupling

Antoine Canaguier-Durand·Cyriaque Genet·Astrid Lambrecht·Thomas W. Ebbesen·Serge Reynaud
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Abstract

Strongly coupled organic systems are characterized by unusually large Rabi splittings, even in the vacuum state. They show the counter-intuitive feature of a lifetime of the lower polariton state longer than for all other excited states. Here we build up a new theoretical framework to understand the dynamics of such coupled system. In particular, we show that the non-Markovian character of the relaxation of the dressed organic system explains the long lifetime of the lower polariton state.

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Antoine Canaguier-Durand, Cyriaque Genet, Astrid Lambrecht, Thomas W. Ebbesen, Serge Reynaud. 2013-12-28. Non-markovian polariton dynamics in organic strong coupling. https://doi.org/10.1140/epjd%2Fe2014-50539-x

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