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arXiv · 1412.3776

High-field magnetic resonance of spinons and magnons in a triangular lattice S=1/2 antiferromagnet Cs2CuCl4

A. I. Smirnov·T. A. Soldatov·K. Yu. Povarov·A. Ya. Shapiro
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Abstract

The electron spin resonance doublet indicating the width of the two spinon continuum in a spin-1/2 triangular-lattice Heisenberg antiferromagnet Cs2CuCl4 was studied in high magnetic field. The doublet was found to collapse in a magnetic field of a half of the saturation field. The collapse of the doublet occurs via vanishing of the high frequency component in a qualitative agreement with the theoretical prediction for the S=1/2 chain. The field of the collapse is, however, much lower than expected for the S=1/2 chain. This is proposed to be due to the destruction of frustration of interchain exchange bonds in a magnetic field, which restores the 2D character of this spin system. In the saturated phase the mode with the Larmor frequency and a much weaker mode downshifted for 119~GHz are observed. The weak mode is of exchange origin, it demonstrates a positive frequency shift at heating corresponding to the repulsion of magnons in the saturated phase.

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A. I. Smirnov, T. A. Soldatov, K. Yu. Povarov, A. Ya. Shapiro. 2014-12-11. High-field magnetic resonance of spinons and magnons in a triangular lattice S=1/2 antiferromagnet Cs2CuCl4. https://doi.org/10.1103/physrevb.91.174412

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