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arXiv · 1607.05878

Electromagnon in the Z-type hexaferrite $({\rm Ba}_{x}{\rm Sr}_{1-x})_3\rm Co_2Fe_{24}O_{41}$

Filip Kadlec·Christelle Kadlec·Jakub Vit·Fedir Borodavka·Martin Kempa·Jan Prokleska·Josef Bursik·Robert Uhrecky·Stephane Rols·Yi Sheng Chai·Kun Zhai·Young Sun·Jan Drahokoupil·Veronica Goian·Stanislav Kamba
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Abstract

We studied experimentally the high-temperature magnetoelectric $({\rm Ba}_{x}{\rm Sr}_{1-x})_3\rm Co_2Fe_{24}O_{41}$ prepared as ceramics (x = 0, 0.2) and a single crystal (x = 0.5) using inelastic neutron scattering, THz time-domain, Raman and far-infrared spectroscopies. The spectra, measured with varying temperature and magnetic field, reveal rich information about the collective spin and lattice excitations. In the ceramics, we observed an infrared-active magnon which is absent in $E^{\omega}\perp z$ polarized THz spectra of the crystal, and we assume that it is an electromagnon active in $E^{\omega} \| z$ polarized spectra. On heating from 7 to 250 K, the frequency of this electromagnon drops from 36 to 25 cm$^{-1}$ and its damping gradually increases, so it becomes overdamped at room temperature. Applying external magnetic field has a similar effect on the damping and frequency of the electromagnon, and the mode is no more observable in the THz spectra above 2 T, as the transverse-conical magnetic structure transforms into a collinear one. Raman spectra reveal another spin excitation with a slightly different frequency and much higher damping. Upon applying magnetic field higher than 3 T, in the low-frequency part of the THz spectra, a narrow excitation appears whose frequency linearly increases with magnetic field. We interpret this feature as the ferromagnetic resonance.

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Filip Kadlec, Christelle Kadlec, Jakub Vit, Fedir Borodavka, Martin Kempa, Jan Prokleska, Josef Bursik, Robert Uhrecky, Stephane Rols, Yi Sheng Chai, Kun Zhai, Young Sun, Jan Drahokoupil, Veronica Goian, Stanislav Kamba. 2016-07-20. Electromagnon in the Z-type hexaferrite $({\rm Ba}_{x}{\rm Sr}_{1-x})_3\rm Co_2Fe_{24}O_{41}$. https://doi.org/10.1103/physrevb.94.024419

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