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arXiv · 1703.04279

High quality atomically thin PtSe2 films grown by molecular beam epitaxy

Mingzhe Yan·Eryin Wang·Xue Zhou·Guangqi Zhang·Hongyun Zhang·Kenan Zhang·Wei Yao·Shuzhen Yang·Shilong Wu·Tomoki Yoshikawa·Koji Miyamoto·Taichi Okuda·Yang Wu·Pu Yu·Wenhui Duan·Shuyun Zhou
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Abstract

Atomically thin PtSe2 films have attracted extensive research interests for potential applications in high-speed electronics, spintronics and photodetectors. Obtaining high quality, single crystalline thin films with large size is critical. Here we report the first successful layer-by-layer growth of high quality PtSe2 films by molecular beam epitaxy. Atomically thin films from 1 ML to 22 ML have been grown and characterized by low-energy electron diffraction, Raman spectroscopy and X-ray photoemission spectroscopy. Moreover, a systematic thickness dependent study of the electronic structure is revealed by angle-resolved photoemission spectroscopy (ARPES), and helical spin texture is revealed by spin-ARPES. Our work provides new opportunities for growing large size single crystalline films for investigating the physical properties and potential applications of PtSe2.

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Mingzhe Yan, Eryin Wang, Xue Zhou, Guangqi Zhang, Hongyun Zhang, Kenan Zhang, Wei Yao, Shuzhen Yang, Shilong Wu, Tomoki Yoshikawa, Koji Miyamoto, Taichi Okuda, Yang Wu, Pu Yu, Wenhui Duan, Shuyun Zhou. 2017-03-15. High quality atomically thin PtSe2 films grown by molecular beam epitaxy. https://doi.org/10.1088/2053-1583%2Faa8919

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