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arXiv · 1707.01718

Graphene nanoribbons on gold: Understanding superlubricity and edge effects

Lorenzo Gigli·Nicola Manini·Andrea Benassi·Erio Tosatti·Andrea Vanossi·Roberto Guerra
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Abstract

We address the atomistic nature of the longitudinal static friction against sliding of graphene nanoribbons (GNRs) deposited on gold, a system whose structural and mechanical properties have been recently the subject of intense experimental investigation. By means of numerical simulations and modeling we show that the GNR interior is structurally lubric ("superlubric") so that the static friction is dominated by the front/tail regions of the GNR, where the residual uncompensated lateral forces arising from the interaction with the underneath gold surface opposes the free sliding. As a result of this edge pinning the static friction does not grow with the GNR length, but oscillates around a fairly constant mean value. These friction oscillations are explained in terms of the GNR-Au(111) lattice mismatch: at certain GNR lengths close to an integer number of the beat (or moire') length there is good force compensation and superlubric sliding; whereas close to half odd-integer periods there is significant pinning of the edge with larger friction. These results make qualitative contact with recent state-of-the-art atomic force microscopy experiment, as well as with the sliding of other different incommensurate systems.

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Lorenzo Gigli, Nicola Manini, Andrea Benassi, Erio Tosatti, Andrea Vanossi, Roberto Guerra. 2017-07-06. Graphene nanoribbons on gold: Understanding superlubricity and edge effects. https://arxiv.org/abs/1707.01718

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