arXiv · 1708.01991
Tunable near- to mid-infrared pump terahertz probe spectroscopy in reflection geometry
Abstract
Strong-field mid-infrared pump--terahertz (THz) probe spectroscopy has been proven as a powerful tool for light control of different orders in strongly correlated materials. We report the construction of an ultrafast broadband infrared pump--THz probe system in reflection geometry. A two-output optical parametric amplifier is used for generating mid-infrared pulses with GaSe as the nonlinear crystal. The setup is capable of pumping bulk materials at wavelengths ranging from 1.2 $\mu$m to 15 $\mu$m and beyond, and detecting the subtle, transient photoinduced changes in the reflected electric field of the THz probe at different temperatures. As a demonstration, we present 15 $\mu$m pump--THz probe measurements of a bulk EuSbTe$_{3}$ single crystal. A $0.5\%$ transient change in the reflected THz electric field can be clearly resolved. The widely tuned pumping energy could be used in mode-selective excitation experiments and applied to many strongly correlated electron systems.
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S. J. Zhang, Z. X. Wang, T. Dong, N. L. Wang. 2017-08-07. Tunable near- to mid-infrared pump terahertz probe spectroscopy in reflection geometry. https://doi.org/10.1007/s11467-017-0716-4
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