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arXiv · 1712.08511

Uniaxial and hydrostatic pressure effects in alpha-RuCl3 single crystals via thermal-expansion measurements

Mingquan He·Xiao Wang·Liran Wang·Frédéric Hardy·Thomas Wolf·Peter Adelmann·Thomas Brückel·Yixi Su·Christoph Meingast
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Abstract

We present high-resolution thermal-expansion and specific-heat measurements of single crystalline alpha-RuCl3. An extremely hysteretic structural transition expanding over 100 K is observed by thermal- expansion along both crystallographic axes, which we attribute to a change of stacking sequence of the RuCl3 layers. Three magnetic transitions are observed, which we link to the different stacking sequences. Using our data and thermodynamic relations, we derive the uniaxial and hydrostatic pressure derivatives of all three magnetic transitions. Our results demonstrate that magnetic order should be totally suppressed by very moderate pressures of 0.3 GPa to 0.9 GPa. Finally, we discuss why our results differ from recent hydrostatic pressure measurements and suggest a possible route to reaching the spin-liquid state in alpha-RuCl3.

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Mingquan He, Xiao Wang, Liran Wang, Frédéric Hardy, Thomas Wolf, Peter Adelmann, Thomas Brückel, Yixi Su, Christoph Meingast. 2017-12-22. Uniaxial and hydrostatic pressure effects in alpha-RuCl3 single crystals via thermal-expansion measurements. https://doi.org/10.1088/1361-648x/aada1e

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