Large Thermal Hall Effect in $α$-RuCl$_3$: Evidence for Heat Transport by Kitaev-Heisenberg Paramagnons

Abstract

The honeycomb Kitaev model in a magnetic field is a source of a topological quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. We present experimental results for the thermal Hall effect of the material $α$-RuCl$_{3}$ which recently emerged as a prime candidate for realizing such physics. At temperatures above long-range magnetic ordering $T\gtrsim T_N\approx8$ K, we observe with an applied magnetic field $B$ perpendicular to the honeycomb layers a sizeable positive transversal heat conductivity $κ_{xy}$ which increases linearly with $B$. Upon raising the temperature, $κ_{xy}(T)$ increases strongly, exhibits a broad maximum at around 30 K, and eventually becomes negligible at $T\gtrsim 125$ K. Remarkably, the longitudinal heat conductivity $κ_{xx}(T)$ exhibits a sizeable positive thermal magnetoresistance effect. Thus, our findings provide clear-cut evidence for longitudinal and transverse magnetic heat transport and underpin the unconventional nature of the quasiparticles in the paramagnetic phase of $α$-RuCl$_{3}$.