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arXiv · 1905.12448

Photoinduced nematic state in FeSe$_{0.4}$Te$_{0.6}$

Laura Fanfarillo·Damir Kopić·Andrea Sterzi·Giulia Manzoni·Alberto Crepaldi·Vladimir Tsurkan·Dorina Croitori·Joachim Deisenhofer·Fulvio Parmigiani·Massimo Capone·Federico Cilento
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Abstract

FeSe$_{x}$Te$_{1-x}$ compounds present a complex phase diagram, ranging from the nematicity of FeSe to the $(\pi, \pi)$ magnetism of FeTe. We focus on FeSe$_{0.4}$Te$_{0.6}$, where the nematic ordering is absent at equilibrium. We use a time-resolved approach based on femtosecond light pulses to study the dynamics following photoexcitation in this system. The use of polarization-dependent time- and angle-resolved photoelectron spectroscopy allows us to reveal a photoinduced nematic metastable state, whose stabilization cannot be interpreted in terms of an effective photodoping. We argue that the 1.55 eV photon-energy-pump-pulse perturbs the $C_4$ symmetry of the system triggering the realization of the nematic state. The possibility to induce nematicity using an ultra-short pulse sheds a new light on the driving force behind the nematic symmetry breaking in iron-based superconductors. Our results weaken the idea that a low-energy coupling with fluctuations is a necessary condition to stabilize the nematic order and ascribe the origin of the nematic order in iron-based superconductors to a clear tendency of those systems towards orbital differentiation due to strong electronic correlations induced by the Hund's coupling.

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Laura Fanfarillo, Damir Kopić, Andrea Sterzi, Giulia Manzoni, Alberto Crepaldi, Vladimir Tsurkan, Dorina Croitori, Joachim Deisenhofer, Fulvio Parmigiani, Massimo Capone, Federico Cilento. 2019-05-29. Photoinduced nematic state in FeSe$_{0.4}$Te$_{0.6}$. https://doi.org/10.1016/j.elspec.2021.147090

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