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Dorina Croitori

Publications and source records attributed to Dorina Croitori.

3 recordsLinked to original sources

Spatially resolving superconductivity in type-II superconductors

Superconductivity is identified by the emergence of a macroscopic zero-resistance state, typically inferred from a vanishing four-probe voltage at finite current. That inference assumes spatially uniform conduction-e.g., at least one continuous superconducting path between the current leads and voltage electrodes that sample a finite potential gradient-and can fail if the drive current bypasses the electrodes or if narrow filaments short the current contacts. Here we introduce a methodology to test these assumptions in superconductors, by using spatially resolved measurements of local variations in dc using cryogenic conductive atomic-force microscopy (cAFM). Using Fe(Se,Te) as a model system, we find that despite bulk measurements consistent with a homogeneous superconducting state, the material exhibits a heterogeneous conducting landscape: micrometre-scale superconducting regions coexist with relatively insulating areas. We further show that cAFM resolves conductance fluctuations at 20 K (> TC) that vary between repeated scans, consistent with expectations for short-lived, pre-formed Cooper pairs in the BCS-BEC crossover regime. These results establish cAFM as a practical tool to validate assumptions underlying four-probe transport and underscore the need for direct spatial probes in materials whose macroscopic response can conceal nanoscale inhomogeneity. Accurate identification of macroscopic properties is critical for materials classes like superconductors that are defined by their macroscopic properties.

cond-mat.supr-con

Photoinduced nematic state in FeSe$_{0.4}$Te$_{0.6}$

FeSe$_{x}$Te$_{1-x}$ compounds present a complex phase diagram, ranging from the nematicity of FeSe to the $(π, π)$ magnetism of FeTe. We focus on FeSe$_{0.4}$Te$_{0.6}$, where the nematic ordering is absent at equilibrium. We use a time-resolved approach based on femtosecond light pulses to study the dynamics following photoexcitation in this system. The use of polarization-dependent time- and angle-resolved photoelectron spectroscopy allows us to reveal a photoinduced nematic metastable state, whose stabilization cannot be interpreted in terms of an effective photodoping. We argue that the 1.55 eV photon-energy-pump-pulse perturbs the $C_4$ symmetry of the system triggering the realization of the nematic state. The possibility to induce nematicity using an ultra-short pulse sheds a new light on the driving force behind the nematic symmetry breaking in iron-based superconductors. Our results weaken the idea that a low-energy coupling with fluctuations is a necessary condition to stabilize the nematic order and ascribe the origin of the nematic order in iron-based superconductors to a clear tendency of those systems towards orbital differentiation due to strong electronic correlations induced by the Hund's coupling.

cond-mat.str-el

Manipulating surface magnetic order in iron telluride

Control of emergent magnetic orders in correlated electron materials promises new opportunities for applications in spintronics. For their technological exploitation, it is important to understand the role of surfaces and interfaces to other materials and their impact on the emergent magnetic orders. Here, we demonstrate for iron telluride, the nonsuperconducting parent compound of the iron chalcogenide superconductors, determination and manipulation of the surface magnetic structure by low-temperature spin-polarized scanning tunneling microscopy. Iron telluride exhibits a complex structural and magnetic phase diagram as a function of interstitial iron concentration. Several theories have been put forward to explain the different magnetic orders observed in the phase diagram, which ascribe a dominant role either to interactions mediated by itinerant electrons or to local moment interactions. Through the controlled removal of surface excess iron, we can separate the influence of the excess iron from that of the change in the lattice structure.

cond-mat.str-el