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arXiv · 2007.06805

Three-dimensional Ising Ferrimagnetism of Cr-Fe-Cr trimers in FeCr2Te4

Yu Liu·R. J. Koch·Zhixiang Hu·Niraj Aryal·Eli Stavitski·Xiao Tong·Klaus Attenkofer·E. S. Bozin·Weiguo Yin·C. Petrovic
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Abstract

We carried out a comprehensive study of magnetic critical behavior in single crystals of ternary chalcogenide FeCr$_2$Te$_4$ that undergoes a ferrimagnetic transition below $T_c$ $\sim$ 123 K. Detailed critical behavior analysis and scaled magnetic entropy change indicate a second-order ferrimagentic transition. Critical exponents $β= 0.30(1)$ with $T_c = 122.4(5)$ K, $γ= 1.22(1)$ with $T_c = 122.8(1)$ K, and $δ= 4.24(2)$ at $T_c$ $\sim$ 123 K suggest that the spins approach three-dimensional Ising ($β$ = 0.325, $γ$ = 1.24, and $δ$ = 4.82) model coupled with the attractive long-range interactions between spins that decay as $J(r)\approx r^{-4.88}$. Our results suggest that the ferrimagnetism in FeCr$_2$Te$_4$ is due to itinerant ferromagnetism among the antiferromagnetically coupled Cr-Fe-Cr trimers.

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Yu Liu, R. J. Koch, Zhixiang Hu, Niraj Aryal, Eli Stavitski, Xiao Tong, Klaus Attenkofer, E. S. Bozin, Weiguo Yin, C. Petrovic. 2020-08-18. Three-dimensional Ising Ferrimagnetism of Cr-Fe-Cr trimers in FeCr2Te4. https://doi.org/10.1103/physrevb.102.085158

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