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arXiv · 2104.14242

Two-dimensional plasmonic polarons in n-doped monolayer MoS2

Fabio Caruso·Patrick Amsalem·Jie Ma·Areej Aljarb·Thorsten Schultz·Marios Zacharias·Vincent Tung·Norbert Koch·Claudia Draxl
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Abstract

We report experimental and theoretical evidence of strong electron-plasmon interaction in n-doped single-layer MoS2. Angle-resolved photoemission spectroscopy (ARPES) measurements reveal the emergence of distinctive signatures of polaronic coupling in the electron spectral function. Calculations based on many-body perturbation theory illustrate that electronic coupling to two-dimensional (2D) carrier plasmons provides an exhaustive explanation of the experimental spectral features and their energies. These results constitute compelling evidence of the formation of plasmon-induced polaronic quasiparticles, suggesting that highly-doped transition-metal dichalcogenides may provide a new platform to explore strong-coupling phenomena between electrons and plasmons in 2D.

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Fabio Caruso, Patrick Amsalem, Jie Ma, Areej Aljarb, Thorsten Schultz, Marios Zacharias, Vincent Tung, Norbert Koch, Claudia Draxl. 2021-04-29. Two-dimensional plasmonic polarons in n-doped monolayer MoS2. https://doi.org/10.1103/physrevb.103.205152

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