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arXiv · 2111.05946

Hot-Band Absorption Can Mimic Entangled Two-Photon Absorption

Alexander Mikhaylov·Ryan N. Wilson·Kristen M. Parzuchowski·Michael D. Mazurek·Charles H. Camp Jr·Martin J. Stevens·Ralph Jimenez
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Abstract

It has been proposed that entangled two-photon absorption (E2PA) can be observed with up to 10 orders of magnitude lower photon flux than its classical counterpart. However, there is a significant controversy regarding the magnitude of this quantum enhancement in excitation efficiency. We investigated the fluorescence signals from Rhodamine 6G and LDS798 excited with a CW laser or an entangled photon pair source at 1060 nm. We observed a signal that originates from hot-band absorption (HBA), which is one-photon absorption from thermally-populated vibrational levels of the ground electronic state. This mechanism, which has not been previously discussed in the context of E2PA, produces a signal with a linear power dependence, as would be expected for entangled two-photon excited fluorescence (E2PEF). For the typical conditions under which E2PEF measurements are performed, contributions from the HBA process could lead to a several orders-of-magnitude overestimate of the quantum advantage for excitation efficiency.

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Alexander Mikhaylov, Ryan N. Wilson, Kristen M. Parzuchowski, Michael D. Mazurek, Charles H. Camp Jr, Martin J. Stevens, Ralph Jimenez. 2021-11-10. Hot-Band Absorption Can Mimic Entangled Two-Photon Absorption. https://arxiv.org/abs/2111.05946

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