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Kristen M. Parzuchowski

Publications and source records attributed to Kristen M. Parzuchowski.

6 recordsLinked to original sources

Characterization and Active Control of Position-Dependent Timing Dynamics in Superconducting Strip Detectors

Superconducting strip single-photon detectors (SSPDs) have emerged as scalable, wide-strip variants of traditional nanowire counterparts. Despite practical advantages including improved optical fill factors and enhanced signal-to-noise ratios the fundamental detection physics governing these micro-scale geometries remains largely unexplored. Here, we investigate the underlying photoresponse of a 20 um-wide tungsten silicide SSPD, demonstrating a slew-rate-corrected timing jitter of 13.2 ps at 532 nm and 20.5 ps at 1550 nm, alongside saturated internal detection efficiency up to 1550 nm. Using focused free-space optical scanning, we reveal that detector timing jitter is strongly influenced by a spatially dependent slew rate between edge and center absorption events. To mitigate this impact, we utilize a parallel superconducting rail architecture to actively redistribute supercurrent. This in-situ tuning minimizes the latency mismatch and mitigates thermally activated intrinsic dark counts, extending the device's ability to operate at higher temperatures. Finally, comparing these dynamics with time-dependent Ginzburg-Landau (TDGL) modeling elucidates the physical origins of the position-dependent photoresponse, highlighting how superconducting rails or specialized readout electronics can mitigate negative impacts on timing jitter.

physics.ins-det↗

Reaching the intrinsic performance limits of superconducting nanowire single-photon detectors up to 0.1 mm wide

Superconducting nanowire single-photon detectors (SNSPDs) combine high detection efficiency, low noise, and excellent timing resolution, making them a leading platform for photon-counting applications. However, despite decades of materials and fabrication research, detector performance has never been shown to match theoretical performance expectations. Here, we demonstrate for the first time in situ tuning of a detector from its typical, suboptimal operation, to a regime limited only by material quality, allowing the device to reach its intrinsic performance limit. Our approach is based on current-biased superconducting "rails" placed on either side of the detector that redistribute current across its width to achieve its peak performance. This technique reduces the dark count rate by ten orders of magnitude. Further, we show operation at this intrinsic performance limit for devices up to 0.1 mm wide, and also demonstrate near-unity internal detection efficiency (IDE) at a wavelength of 4um for a 20um-wide detector--a factor of 20 wider than the current state of the art. This work enables future detectors to overcome the Pearl limit for device width, paving the way for arbitrarily large detectors.

cond-mat.supr-con↗

A Liquid-Core Fiber Platform for Classical and Entangled Two-Photon Absorption Measurements

We introduce a toluene-filled fiber platform for two-photon absorption measurements. By confining both the light and molecular sample inside the 5 $μ$m hollow core of the fiber, we increase the distance over which the nonlinear light-matter interaction occurs. With only a 7.3 nL excitation volume, we measure classical two-photon absorption (C2PA) at an average laser power as low as 1.75 nW, which is a 45-fold improvement over a conventional free-space technique. We use this platform to attempt to measure entangled two-photon absorption (E2PA), a process with a limited regime where the quantum advantage is large. This regime arises due to a crossover from linear to quadratic scaling with photon flux as photon flux is increased. Recently, several teams of researchers have reported that E2PA cross-sections are much smaller than previously claimed. As a result, the linear scaling dominates at photon fluxes so low that it is extremely difficult or impossible to measure using conventional free-space techniques. In this report, we implement the first E2PA measurement using a waveguide. We see no evidence of E2PA, and we set an upper bound on the cross-section consistent with these recent reports.

quant-ph↗

Hot-Band Absorption Can Mimic Entangled Two-Photon Absorption

It has been proposed that entangled two-photon absorption (E2PA) can be observed with up to 10 orders of magnitude lower photon flux than its classical counterpart. However, there is a significant controversy regarding the magnitude of this quantum enhancement in excitation efficiency. We investigated the fluorescence signals from Rhodamine 6G and LDS798 excited with a CW laser or an entangled photon pair source at 1060 nm. We observed a signal that originates from hot-band absorption (HBA), which is one-photon absorption from thermally-populated vibrational levels of the ground electronic state. This mechanism, which has not been previously discussed in the context of E2PA, produces a signal with a linear power dependence, as would be expected for entangled two-photon excited fluorescence (E2PEF). For the typical conditions under which E2PEF measurements are performed, contributions from the HBA process could lead to a several orders-of-magnitude overestimate of the quantum advantage for excitation efficiency.

quant-ph↗

Witnessing the survival of time-energy entanglement through biological tissue and scattering media

We demonstrate the preservation of time-energy entanglement of near-IR photons through thick biological media ($\leq$1.55 mm) and tissue ($\leq$ 235 $μ$m) at room temperature. Using a Franson-type interferometer, we demonstrate interferometric contrast of over 0.9 in skim milk, 2% milk, and chicken tissue. This work supports the many proposed opportunities for nonclassical light in biological imaging and analyses from sub-shot noise measurements to entanglement-enhanced fluorescence imaging, clearly indicating that the entanglement characteristics of photons can be maintained even after propagation through thick, turbid biological samples.

quant-ph↗

Setting bounds on two-photon absorption cross-sections in common fluorophores with entangled photon pair excitation

Excitation with entangled photon pairs may lead to an increase in the efficiency of two-photon absorption at low photon flux. The corresponding process, entangled two-photon absorption (E2PA), has been investigated in numerous theoretical and experimental studies. However, significant ambiguity and inconsistency remain in the literature about the absolute values of E2PA cross-sections. Here, we use a fluorescence-based registration scheme to experimentally determine upper bounds on the cross-sections for six fluorophores. These bounds are up to four orders of magnitude lower than the smallest published cross-section. For two samples that have been studied by others, Rhodamine 6G and 9R-S, we measure upper bounds four and five orders of magnitude lower than the previously reported cross-sections.

quant-ph↗