Electrostatic focusing of cold and heavy molecules for the ACME electron EDM search

Abstract

The current best upper limit for electron electric dipole moment (EDM), $|d_e|<1.1\times10^{-29}\,$e$\cdot$cm ($90$% confidence), was set by the ACME collaboration in 2018. The ACME experiment uses a spin-precession measurement in a cold beam of ThO molecules to detect $d_e$. An improvement in statistical uncertainty would be possible with more efficient use of molecules from the cryogenic buffer gas beam source. Here, we demonstrate electrostatic focusing of the ThO beam with a hexapole lens. This results in a factor of $16$ enhancement in the molecular flux detectable downstream, in a beamline similar to that built for the next generation of ACME. We also demonstrate an upgraded rotational cooling scheme that increases the ground state population by $3.5$ times compared to no cooling, consistent with expectations and a factor of $1.4$ larger than previously in ACME. When combined with other demonstrated improvements, we project over an order of magnitude improvement in statistical sensitivity for the next generation ACME electron EDM search.