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arXiv · 2207.10834

Ferroelectricity driven by magnetism in quasi-one-dimensional Ba9Fe3Se15

Jun Zhang·Xiancheng Wang·Yiqing Hao·Guangxiu Liu·Long Zhou·Daniel M. Pajerowski·Jian-Tao Wang·Jinlong Zhu·Jun Zhao·Jiulong Wang·Yifeng Zhao·Chungang Duan·Youwen Long·Chang-Jong Kang·Martha Greenblatt·Changqing Jin
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Abstract

The spin-induced ferroelectricity in quasi-1D spin chain system is little known, which could be fundamentally different from those in three-dimensional (3D) system. Here, we report the ferroelectricity driven by a tilted screw spin order and its exotic dynamic in the spin-chain compound Ba9Fe3Se15. It is found that the spin-induced polarization has already occurred and exhibits magnetoelectric coupling behavior far above the long-range spin order (LRSO) at TN = 14 K. The polarized entities grow and their dynamic responses slow down gradually with decreasing temperature and permeate the whole lattice to form 3D ferroelectricity at TN. Our results reveal that the short-range spin orders (SRSOs) in the decoupled chains play a key role for the exotic dynamic in this dimension reduced system. Ba9Fe3Se15 is the only example so far which exhibits electric polarization above LRSO temperature because of the formation of SRSOs.

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Jun Zhang, Xiancheng Wang, Yiqing Hao, Guangxiu Liu, Long Zhou, Daniel M. Pajerowski, Jian-Tao Wang, Jinlong Zhu, Jun Zhao, Jiulong Wang, Yifeng Zhao, Chungang Duan, Youwen Long, Chang-Jong Kang, Martha Greenblatt, Changqing Jin. 2022-07-22. Ferroelectricity driven by magnetism in quasi-one-dimensional Ba9Fe3Se15. https://arxiv.org/abs/2207.10834

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