New technique of ion identification in Accelerator Mass Spectrometry using low-pressure TPC with GEM readout

Abstract

We have developed and successfully tested a low-pressure Time Projection Chamber (TPC) with Gas Electron Multiplier (GEM) readout for Accelerator Mass Spectrometry (AMS). AMS facility in Novosibirsk has a problem of separating isobar ions of different chemical elements that have the same atomic mass. The typical example is radioactive isotopes 10Be and 10B that are used to date geological objects at a time scale of ten million years. To solve this problem, a new ion identification technique, namely that based on measuring both ion track ranges and ion energies in low-pressure TPCs with GEM readout, has been developed. This technique is proposed to be applied in AMS for dating geological objects, namely for geochronology of Cenozoic era. In this work, we developed a new larger version of the TPC with a dedicated thin silicon nitride window for an efficient passage of ions. The TPC characteristics were studied in isobutane at low pressures using alpha particle sources. In addition, the use of GEM instead of THGEM has been shown to substantially improve the energy resolution at a nominal pressure (50 torr). Using these results and SRIM code simulations, it is shown that isobaric boron and beryllium ions can be effectively separated at AMS, providing efficient dating on a scale of ten million years. This technique will be applied in the AMS facility in Novosibirsk in the near future.