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arXiv · 2310.00189

Electro-nuclear dynamics of single and double ionization of H$_2$ in ultrafast intense laser pulses

Jean-Nicolas Vigneau·Thanh-Tung Nguyen Dang·Eric Charron
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Abstract

We present an efficient method for modeling the single and double ionization dynamics of the H$_2$ molecule in ultrashort intense laser fields. This method is based on a semi-analytical approach to calculate the time-dependent single and double molecular ionization rates and on a numerical approach to describe the vibrational motion that takes place in the intermediate molecular ion H$_2^+$. This model allows for the prediction of the single and double ionization probabilities of the H$_2$ molecule to be made over a wide range of frequencies and laser intensities with limited computational time, while providing a realistic estimate of the energy of the products of the dissociative ionization and of the Coulomb explosion of the H$_2$ molecule. The effect of vibrational dynamics on ionization yields and proton kinetic energy release spectra is demonstrated and, in the case of the latter, discussed in terms of basic strong-field molecular fragmentation mechanisms.

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Jean-Nicolas Vigneau, Thanh-Tung Nguyen Dang, Eric Charron. 2023-09-29. Electro-nuclear dynamics of single and double ionization of H$_2$ in ultrafast intense laser pulses. https://doi.org/10.1021/acs.jpca.3c06525

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