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Eric Charron

Publications and source records attributed to Eric Charron.

At least 19 recordsLinked to original sources

Trap-Quenched Matter-Wave Optics in Space

Dual-species atomic sources in space promise to be the testbed for a multitude of searches in quantum gas physics such as a precise test of the Universality of Free Fall (UFF), few-body physics, cold molecules and quantum bubbles. These experiments demand exquisite control over the expansion energies of both condensed ensembles as well as over their differential center-of-mass dynamics. We propose a trap-quenched collimation technique featuring in-trap excitations of collective modes compatible with state-of-the-art atom-chip setups. Using NASA's Cold Atom Laboratory aboard the International Space Station, we demonstrate it on a single-species $^{87}$Rb condensate. By controlling the center-of-mass release dynamics, we observe free expansion times up to 700 ms and measure a two-dimensional expansion energy of $k_B \cdot 78\pm 9 \;\mathrm{pK}$ in the imaging plane. A detailed model of the magnetically-induced dynamics indicates that this corresponds to a two-dimensional expansion energy of about $k_B \cdot 15^{+12}_{-5}\; \mathrm{pK}$ along two of the condensate's eigenaxes. Finally, we theoretically study this trap-quenched collimation scheme for a $^{41}$K-$^{87}$Rb mixture, predicting a simultaneous collimation that meets the expansion energy requirements for a state-of-the-art UFF test at the $10^{-15}$ accuracy level.

physics.atom-ph

Fast momentum-selective transport of Bose-Einstein condensates via controlled non-adiabatic dynamics in optical lattices

We present a detailed numerical study of a protocol for momentum-selective transport of a Bose-Einstein condensate (BEC) in a one-dimensional optical lattice, achieving narrow momentum distributions through controlled non-adiabatic dynamics. The protocol consists of non-adiabatic loading into the lattice, coherent acceleration using a symmetric trapezoidal acceleration profile, and non-adiabatic release into free space. Using the time-dependent Gross-Pitaevskii equation, we simulate the full sequence and analyze the role of non-adiabatic excitations on the final momentum distribution. We identify the intra-site breathing dynamics as the dominant mechanism governing spectral purity under fast loading conditions. By tracking the condensate's spatial width during the evolution, we demonstrate a direct correlation with the final momentum spread. A variational model based on a Gaussian ansatz quantitatively reproduces the observed dynamics and provides physical insight into the breathing mechanism. Our results reveal the existence of "magic" times, i.e., specific loading or acceleration durations synchronized with the breathing oscillation period, where quasi-monochromatic momentum distributions can be achieved even with loading times as short as 100 microseconds. In the tight-binding regime, this approach offers speedup factors of 3 to 6 compared to adiabatic protocols while maintaining high transfer fidelities, providing a practical route to coherent transport for quantum sensors operating under stringent timing constraints.

cond-mat.quant-gas

Measurement of Casimir-Polder interaction for slow atoms through a material grating

We present a method utilizing atomic diffraction patterns and statistical analysis tools to infer the Casimir-Polder interaction between Argon atoms and a silicon nitride nanograting. The quantum model that supports the data is investigated in detail, as are the roles of nanograting geometry, finite size effects, slit width opening angles, and Lennard-Jones potentials. Our findings indicate that the atom-surface potential strength parameter is C3 = 6.87 $\pm$ 1.18 meV.nm3. This value is primarily constrained by the knowledge of the nanograting geometry. The high sensitivity of our method paves the way for precise determination of the Casimir-Polder potential and exploration of new short-distance forces.

physics.atom-ph

Interferometry of Atomic Matter Waves in the Cold Atom Lab onboard the International Space Station

Ultracold atomic gases hold unique promise for space science by capitalizing on quantum advantages and extended freefall, afforded in a microgravity environment, to enable next-generation precision sensors. Atom interferometers are a class of quantum sensors which can use freely falling gases of atoms cooled to sub-photon-recoil temperatures to provide unprecedented sensitivities to accelerations, rotations, and gravitational forces, and are currently being developed for space-based applications in gravitational, earth, and planetary sciences, as well as to search for subtle forces that could signify physics beyond General Relativity and the Standard Model. NASA's Cold Atom Lab (CAL) operates onboard the International Space Station as a multi-user facility for studies of ultracold atoms and to mature quantum technologies, including atom interferometry, in persistent microgravity. In this paper, we report on path-finding experiments utilizing ultracold $^{87}$Rb atoms in the CAL atom interferometer, which was enabled by an on-orbit upgrade of the CAL science module: A three-pulse Mach-Zehnder interferometer was studied to understand limitations from the influence of ISS vibrations. Additionally, Ramsey shear-wave interferometry was used to manifest interference patterns in a single run that were observable for over 150 ms free-expansion time. Finally, the CAL atom interferometer was used to remotely measure the photon recoil from the atom interferometer laser as a demonstration of the first quantum sensor using matter-wave interferometry in space.

physics.atom-ph

Nanoscale Control over Magnetic Light-Matter Interactions

Light-matter interactions are frequently perceived as predominantly influenced by the electric optical field, with the magnetic component of light often overlooked. Nonetheless, the magnetic aspect plays a pivotal role in various optical processes, including chiral light-matter interactions, photon-avalanching, and forbidden photochemistry, underscoring the significance of manipulating magnetic processes in optical phenomena. Here, we explore the ability to control the magnetic light and matter interactions at the nanoscale. In particular, we demonstrate experimentally, using a plasmonic nanostructure, the transfer of energy from the optical magnetic field to a nanoparticle, thanks to the deep subwavelength magnetic confinement allowed by our nano-antenna. This control is made possible by the particular design of our plasmonic nanostructure, which has been optimized to spatially separate the electric and magnetic fields of the localized plasmon. Furthermore, by studying the spontaneous emission from the Lanthanide-ions doped nanoparticle, we observe that the optical field distributions are not spatially correlated with the electric and magnetic near-field quantum environments of this antenna, which seemingly contradicts the reciprocity theorem. We demonstrate that this counter-intuitive observation is in fact, the result of the different optical paths followed by the excitation and emission of the ions, which forbids a direct application of that theorem.

physics.optics

Quantum description of atomic diffraction by material nanostructures

We present a theoretical model of matter-wave diffraction through a material nanostructure. This model is based on the numerical solution of the time-dependent Schr{\"o}dinger equation, which goes beyond the standard semi-classical approach. In particular, we consider the dispersion force interaction between the atoms and the material, which is responsible for high energy variations. The effect of such forces on the quantum model is investigated, along with a comparison with the semi-classical model. In particular, for atoms at low velocity and close to the material surface, the semi-classical approach fails, while the quantum model accurately describes the expected diffraction pattern. This description is thus relevant for slow and cold atom experiments where increased precision is required, e.g. for metrological applications.

physics.atom-ph

Matter-wave collimation to picokelvin energies with scattering length and potential shape control

The sensitivity of atom interferometers depends on their ability to realize long pulse separation times and prevent loss of contrast by limiting the expansion of the atomic ensemble within the interferometer beam through matter-wave collimation. Here we investigate the impact of atomic interactions on collimation by applying a lensing protocol to a $^{39}$K Bose-Einstein condensate at different scattering lengths. Tailoring interactions, we measure energies corresponding to $340 \pm 12$ pK in one direction. Our results are supported by an accurate simulation, which allows us to extrapolate a 2D ballistic expansion energy of $438 \pm 77$ pK. Based on our findings we propose an advanced scenario, which enables 3D expansion energies below $16$ pK by implementing an additional pulsed delta-kick. Our results pave the way to realize ensembles with more than $1\times10^5$ atoms and 3D energies in the two-digit pK range in typical dipole trap setups without the need for micro-gravity or long baseline environments.

physics.atom-ph

Electro-nuclear dynamics of single and double ionization of H$_2$ in ultrafast intense laser pulses

We present an efficient method for modeling the single and double ionization dynamics of the H$_2$ molecule in ultrashort intense laser fields. This method is based on a semi-analytical approach to calculate the time-dependent single and double molecular ionization rates and on a numerical approach to describe the vibrational motion that takes place in the intermediate molecular ion H$_2^+$. This model allows for the prediction of the single and double ionization probabilities of the H$_2$ molecule to be made over a wide range of frequencies and laser intensities with limited computational time, while providing a realistic estimate of the energy of the products of the dissociative ionization and of the Coulomb explosion of the H$_2$ molecule. The effect of vibrational dynamics on ionization yields and proton kinetic energy release spectra is demonstrated and, in the case of the latter, discussed in terms of basic strong-field molecular fragmentation mechanisms.

quant-ph

A high-flux source system for matter-wave interferometry exploiting tunable interactions

Atom interferometers allow determining inertial effects to high accuracy. Quantum-projection noise as well as systematic effects impose demands on large atomic flux as well as ultra-low expansion rates. Here we report on a high-flux source of ultra-cold atoms with free expansion rates near the Heisenberg limit directly upon release from the trap. Our results are achieved in a time-averaged optical dipole trap and enabled through dynamic tuning of the atomic scattering length across two orders of magnitude interaction strength via magnetic Feshbach resonances. We demonstrate BECs with more than $6\times 10^{4}$ particles after evaporative cooling for $170$ ms and their subsequent release with a minimal expansion energy of $4.5$ nK in one direction. Based on our results we estimate the performance of an atom interferometer and compare our source system to a high performance chip-trap, as readily available for ultra-precise measurements in micro-gravity environments.

cond-mat.quant-gas

Quantum Gas Mixtures and Dual-Species Atom Interferometry in Space

The capability to reach ultracold atomic temperatures in compact instruments has recently been extended into space. Ultracold temperatures amplify quantum effects, while free-fall allows further cooling and longer interactions time with gravity - the final force without a quantum description. On Earth, these devices have produced macroscopic quantum phenomena such as Bose-Einstein condensation (BECs), superfluidity, and strongly interacting quantum gases. Quantum sensors interfering the superposition of two ultracold atomic isotopes have tested the Universality of Free Fall (UFF), a core tenet of Einstein's classical gravitational theory, at the $10^{-12}$ level. In space, cooling the elements needed to explore the rich physics of strong interactions and preparing the multiple species required for quantum tests of the UFF has remained elusive. Here, utilizing upgraded capabilities of the multi-user Cold Atom Lab (CAL) instrument within the International Space Station (ISS), we report the first simultaneous production of a dual species Bose-Einstein condensate in space (formed from $^{87}$Rb and $^{41}$K), observation of interspecies interactions, as well as the production of $^{39}$K ultracold gases. We have further achieved the first space-borne demonstration of simultaneous atom interferometry with two atomic species ($^{87}$Rb and $^{41}$K). These results are an important step towards quantum tests of UFF in space, and will allow scientists to investigate aspects of few-body physics, quantum chemistry, and fundamental physics in novel regimes without the perturbing asymmetry of gravity.

cond-mat.quant-gas

Efficient numerical description of the dynamics of interacting multispecies quantum gases

We present a highly efficient method for the numerical solution of coupled Gross-Pitaevskii equations describing the evolution dynamics of a multispecies mixture of Bose-Einstein condensates in time-dependent potentials. This method, based on a grid-scaling technique, compares favorably to a more standard but much more computationally expensive solution based on a frozen-resolution grid. It allows an accurate description of the long-time behavior of interacting, multi-species quantum mixtures including the challenging problem of long free expansions relevant for microgravity and space experiments. We demonstrate a successful comparison to experimental measurements of a binary Rb-K mixture recently performed with the payload of a sounding rocket experiment.

cond-mat.quant-gas

Full control of electric and magnetic light-matter interactions through a plasmonic nanomirror on a near-field tip

Light-matter interactions are often considered governed by the electric optical field only, leaving aside the magnetic component of light. However, the magnetic part plays a determining role in many optical processes from light and chiral-matter interactions, photon-avalanching to forbidden photochemistry, making the manipulation of magnetic processes extremely relevant. Here, by creating a standing wave using a plasmonic nanomirror we manipulate the spatial distributions of the electric and magnetic fields and their associated local density of states, allowing the selective control of the excitation and emission of electric and magnetic dipolar transitions. This control allows us to image, in 3D, the electric and magnetic nodes and anti-nodes of the fields interference pattern. It also enables us to enhance specifically photoluminescence from quantum emitters excited only by the magnetic field, and to manipulate their quantum environment by acting on the excitation fields solely, demonstrating full control of magnetic and electric light-matter interactions.

physics.optics

STE-QUEST -- Space Time Explorer and QUantum Equivalence principle Space Test: The 2022 medium-class mission concept

Space-borne quantum technologies, particularly those based on atom interferometry, are heralding a new era of strategic and robust space exploration. The unique conditions of space, characterized by low noise and low gravity environments, open up diverse possibilities for applications ranging from precise time and frequency transfer to Earth Observation and the search of new Physics. In this paper, we summarise the M-class mission proposal in response to the 2022 call in ESA's science program: Space-Time Explorer and Quantum Equivalence Principle Space Test (STE-QUEST). It consists in a satellite mission featuring a dual-species atom interferometer operating over extended durations. This mission aims to tackle three of the most fundamental questions in Physics: (i) testing the universality of free fall with an accuracy better than one part in $10^{-17}$, (ii) exploring various forms of Ultra-Light Dark Matter, and (iii) scrutinizing the foundations of Quantum Mechanics.

physics.space-ph

Strong Field Non-Franck-Condon Ionization of H$_2$: A Semi-Classical Analysis

Single ionization of H$_2$ molecules exposed to strong and short laser pulses is investigated by a semi-classical method. Three laser characteristics are considered: i) The carrier-wave frequency corresponds to wavelengths covering and bridging the two ionization regimes: From tunnel ionization (TI) at 800 nm to multiphoton ionization (MPI) at 266 nm. ii) Values of the peak intensity are chosen within a window to eliminate competing double ionization processes. iii) Particular attention is paid to the polarization of the laser field, which can be linearly or circularly polarized. The results and their interpretation concern two observables, namely the end-of-pulse total ionization probability and vibrational distribution generated in the cation H$_2^+$. The most prominent findings are an increased ionization efficiency in circular polarization and a vibrational distribution of the cation that favors lower-lying levels than those that would be populated in a vertical (Franck-Condon) ionization, leading to non Franck-Condon distributions, both in linear and circular polarizations.

physics.atom-ph

Strong-Field Molecular Ionization Beyond The Single Active Electron Approximation

The present work explores quantitative limits to the Single-Active Electron (SAE) approximation, often used to deal with strong-field ionization and subsequent attosecond dynamics. Using a time-dependent multi\-configuration approach, specifically a Time-Dependent Configuration Interaction (TDCI) method, we solve the time-dependent Schr{\"o}dinger equation (TDSE) for the two-electron dihydrogen molecule, with the possibility of tuning at will the electron-electron interaction by an adiabatic switch-on/switch-off function. We focus on signals of the single ionization of $H_2$ under a strong near-infrared (NIR) four-cycle, linearly-polarized laser pulse of varying intensity, and within a vibrationally frozen molecule model. The observables we address are post-pulse total ionization probability profiles as a function of the laser peak intensity. Three values of the internuclear distance R taken as a parameter are considered, R = R$_{eq}$ = 1.4 a.u, the equilibrium geometry of the molecule, R = 5.0 a.u for an elongated molecule and R = 10.2 a.u for a dissociating molecule. The most striking observation is the non-monotonous behavior of the ionization probability profiles at intermediate elongation distances with an instance of enhanced ionization and one of partial ionization quenching. We give an interpretation of this in terms of a Resonance-Enhanced-Multiphoton Ionization (REMPI) mechanism with interfering overlapping resonances resulting from excited electronic states.

physics.atom-ph

A space-based quantum gas laboratory at picokelvin energy scales

Ultracold quantum gases are ideal sources for high-precision space-borne sensing as proposed for Earth observation, relativistic geodesy and tests of fundamental physical laws as well as for studying new phenomena in many-body physics extended free fall. By performing experiments with the Cold Atom Lab aboard the International Space Station, we have achieved exquisite control over the quantum state of single Bose-Einstein condensates paving the way for future high-precision measurements. In particular, we have applied fast transport protocols to shuttle the atomic cloud over a millimeter distance with sub-micrometer accuracy and subsequently drastically reduced the total expansion energy to below 100 pK with matterwave lensing techniques.

cond-mat.quant-gas

Elastic and magnetoelastic properties of TbMnO3 single crystal by nanosecond time resolved acoustics and first-principles calculations

Time resolved pump and probe acoustics and first-principles calculations were employed to assess elastic properties of the TbMnO3 perovskite manganite having orthorhombic symmetry. Measuring sound velocities of bulk longitudinal and shear acoustic waves propagating along at least two different directions in the high symmetry planes (100), (010) and (001), provided a powerful mean to selectively determine the six diagonal elastic constants C11= 227 GPa, C22= 349 GPa, C33= 274 GPa, C44= 71 GPa, C55= 57 GPa, C66= 62 GPa. Among the three remaining off-diagonal ones, C23= 103 GPa was determined with a bissectrice direction. Density functional theory calculations with colinear spin-polarized provided complementary insights on their optical, elastic and magnetoelastic properties.

cond-mat.str-el

Elastic properties assessment in the multiferroic BiFeO3 by pump and probe method

We have performed elasticity measurements in the bulk multiferroic BiFeO3 (BFO) using acoustical pump and probe spectroscopy. The sound velocities of the (quasi)-longitudinal and of the two (quasi)-transverse acoustic waves along three independent directions of the (110) surface have been measured. Moreover, one surface wave and one longitudinal wave propagating perpendicular to the surface have been detected. Based on initial input values of the six independent Cij elastic constants determined by our density functional theory calculations and our eleven experimental velocities, the numerical resolution of the acoustic equations allows to determine all the Cij elastic constants of BFO. The propagation direction dependence of volume and surface waves phase velocities allows the unambiguously assignment of the waves, hence the polarization of phonons.

cond-mat.str-el